☆ 4.8 Review

Polymer Semiconductors: Synthesis, Processing, and Applications

CHEMICAL REVIEWS (2023)

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Editorial Material Polymer Science

Where porous polymers can make a difference

Robert T. Woodward et al.

EXPRESS POLYMER LETTERS (2023)

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Article Chemistry, Physical

Conjugated Polymers in Solution: A Physical Perspective

Yu-Chun Xu et al.

Summary: Excellent progress has been made in the optoelectronic properties of conjugated polymers by controlling solution-state aggregation. However, it is still challenging to fully understand the complex aggregation process and microstructures of conjugated polymers due to their wide variety and complex structures. This Perspective focuses on discussing the chain conformations, aggregation, and factors influencing solution-state aggregation and microstructures. Strategies to regulate solid-state microstructures and obtain high-performance polymer-based devices from solution-state aggregation are also summarized.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2023)

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Review Polymer Science

Controlling morphology and microstructure of conjugated polymers via solution-state aggregation

Ze-Fan Yao et al.

Summary: This review focuses on the formation, behavior, and evolution of solution-state aggregation of conjugated polymers, exploring their influence on the solid-state morphology and microstructure, and ultimately elucidating the relationship between microstructure and properties of conjugated polymers.

PROGRESS IN POLYMER SCIENCE (2023)

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Article Chemistry, Multidisciplinary

Density of States Engineering of n-Doped Conjugated Polymers for High Charge Transport Performances

Xin-Yi Wang et al.

Summary: The density of states (DOS) distribution of conjugated polymers was engineered by tailoring the solvent used for film preparation, leading to enhanced electrical performances.

ADVANCED MATERIALS (2023)

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Review Chemistry, Multidisciplinary

Characterization Techniques of Polymer Aging: From Beginning to End

Rui Tian et al.

Summary: This review provides an overview of the characterization strategies for the different stages of polymer aging, including the generation of radicals, variation of functional groups, chain scission, formation of low-molecular products, and deterioration in macro-performances. The structure-property relationship and lifetime prediction for aged polymers are highlighted. This review is expected to be valuable for researchers in materials science and chemistry.

CHEMICAL REVIEWS (2023)

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Article Chemistry, Multidisciplinary

Highly Conductive and Solution-Processable n-Doped Transparent Organic Conductor

Zhifan Ke et al.

Summary: The study introduces a solution-processable n-doped organic conductor synthesized through copper-catalyzed cascade reactions. The resulting polymer ink demonstrates excellent stability and endurance under different storage temperatures. The optimized n-doped thin-film transparent conductor shows promising electrical and optical properties, comparable to indium tin oxide, and exhibits exceptional durability under accelerated weathering conditions. Additionally, the n-doped polymer film can serve as an electrode material with high volumetric capacity and enable record-high coloration efficiency in dual-polymer electrochromic devices when paired with p-doped PEDOT:PSS.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2023)

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Article Multidisciplinary Sciences

High n-type and p-type conductivities and power factors achieved in a single conjugated polymer

Zi-Di Yu et al.

Summary: The charge transport properties of conjugated polymers are often limited by energetic disorder. Recently, amorphous conjugated polymers with planar backbone conformations and low energetic disorder have been investigated. However, there is a lack of strategy to finely tune the interchain Tr-Tr contacts of these polymers. In this study, excellent conductivity and thermoelectric performance were achieved in polymers based on thiophene-fused benzodifurandione oligo(p-phenylene-vinylene) by reducing the crystallization rate of side chains and controlling the degree of interchain pi-pi contacts.

SCIENCE ADVANCES (2023)

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Article Chemistry, Multidisciplinary

Highly Conductive and Solution-Processable n-Doped Transparent Organic Conductor

Zhifan Ke et al.

Summary: We report a solution-processable n-doped organic conductor from copper-catalyzed cascade reactions in the air, showing oxidative polymerization and reductive doping in one pot. The resulting polymer ink is stable over 20 days and can withstand storage temperatures from -20 to 65 ?. The optimized n-doped thin-film transparent conductor exhibits a low sheet resistance of 45 omega/sq and a high transmittance (T550 > 80%). It also demonstrates excellent durability under accelerated weathering tests (85 ?/85% RH) and can function as an electrode material with high volumetric capacity when paired with p-doped PEDOT:PSS.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2023)

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Article Polymer Science

Revealing the effect of oligo(ethylene glycol) side chains on n-doping process in FBDPPV-based polymers

Xin-Yi Wang et al.

Summary: The study suggests that solution-state aggregation plays a dominant role in the charge transport and morphology of OEG-substituted polymer, which impacts the doping efficiency and conductivity. Suitable solution-state aggregation is crucial for achieving high doping efficiency and conductivity in doped polymer systems.

JOURNAL OF POLYMER SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Tuning Conjugated Polymer Chain Packing for Stretchable Semiconductors

Jie Xu et al.

Summary: A method of modifying the packing structure of polymer semiconductors using a molecular additive DOP is reported in this study, which improves the mechanical stretchability of polymers without affecting their charge-carrier transport properties.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Conjugated Polymer Mesocrystals with Structural and Optoelectronic Coherence and Anisotropy in Three Dimensions

Liyang Yu et al.

Summary: Semiconducting mesocrystalline bulk polymer specimens with near-intrinsic properties were successfully demonstrated using channel-die pressing method. The persistent mesocrystalline arrangement at macroscopic scales allowed reliable evaluation of electronic charge-transport anisotropy along all three crystallographic axes, with high mobilities found along the pi-stacking. The versatile approach showed promise as a straightforward, readily scalable method to fabricate bulk semiconducting polymer structures with properties typically only accessible by the tedious growth of single crystals.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Influence of Molecular Weight on the Organic Electrochemical Transistor Performance of Ladder-Type Conjugated Polymers

Han-Yan Wu et al.

Summary: Fine-tuning the molecular weight of rigid, ladder-type polymers can significantly enhance the performance of n-type OECTs, achieving record-high geometry-normalized transconductance, electron mobility, and volumetric capacitance. This improvement is attributed to more efficient intermolecular charge transport in high-molecular-weight polymers. Additionally, complementary inverters based on OECTs have demonstrated remarkable voltage gains and ultralow power consumption, making them among the best sub-1 V inverters reported to date.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Unraveling the Molar Mass Dependence of Shearing-Induced Aggregation Structure of a High-Mobility Polymer Semiconductor

Zhongli Wang et al.

Summary: This study investigates the aggregation structure of a high-mobility conjugated copolymer and demonstrates its dependence on the molar mass. The researchers were able to prepare a highly aligned and ordered film using the ordered packing of the aggregated structure in solution, leading to a reliable hole mobility in organic thin-film transistors. The results provide insights into the microstructure control of high-performance electronic devices.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Regulation of High Miscibility for Efficient Charge-Transport in n-Doped Conjugated Polymers

Qi-Yi Li et al.

Summary: This study presents a strategy for achieving efficient charge transport and high doping compatibility in n-doped conjugated polymers. By using disorder side-chains, the issue of compatibility is addressed, allowing for the accommodation of molecular dopants without compromising the original chain packing and charge transport channels.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Review Chemistry, Multidisciplinary

Molecular Design Strategies toward Improvement of Charge Injection and Ionic Conduction in Organic Mixed Ionic-Electronic Conductors for Organic Electrochemical Transistors

Nadzeya A. Kukhta et al.

Summary: This review focuses on recent material developments and current challenges in mixed conductors for bioelectronic applications. It also highlights the fundamental operation principles of the OECT and the current bioelectronic applications of OMIECs, as well as potential strategies for mitigating challenges in OECT channel materials.

CHEMICAL REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Doping Approaches for Organic Semiconductors

Alberto D. Scaccabarozzi et al.

Summary: This article reviews the important advances in organic semiconductor doping and its applications. It discusses the relevant physical processes, established mechanisms, and newly proposed theories. It also provides a comprehensive summary of the most widely studied dopants to date, with a particular focus on the chemical strategies for synthesizing molecules with improved functionality. The article further explores the processing routes for doped organic films and the important relationships between doping, processing, and nanostructure. Lastly, it highlights how doping can enhance the operating characteristics of various organic devices.

CHEMICAL REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Molecular Approach to Engineer Two-Dimensional Devices for CMOS and beyond-CMOS Applications

Yuda Zhao et al.

Summary: This paper provides a review of the recent research progress in the functionalization of two-dimensional materials (2DMs). By covalently or noncovalently functionalizing 2DMs with molecules, more efficient charge injection and transport can be achieved, along with stimuli-responsive functionality. The authors introduce the relevant properties of 2DMs, molecules, and molecular switches, and discuss the physical and chemical strategies for synthesizing 2DM/molecule hybrid systems.

CHEMICAL REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Organic Bioelectronics for In Vitro Systems

Charalampos Pitsalidis et al.

Summary: Bioelectronics have significantly improved clinical diagnostics and precision medicine by enabling bidirectional interfacing with biology and expanding applications to in vitro systems. Conjugated polymers have shown advancements in interfacing with biological tissue in vitro, aiming to develop next generation systems.

CHEMICAL REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Semiconducting Polymers for Neural Applications

Ivan B. Dimov et al.

Summary: Research on electronically interfacing with the nervous system has been ongoing for decades, and has gained more attention in recent years with high-profile initiatives and commercial endeavors. The incorporation of semiconducting polymers in devices that communicate with the nervous system has been a significant development, improving the performance of the tissue-device interface and increasing biocompatibility.

CHEMICAL REVIEWS (2022)

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Article Multidisciplinary Sciences

Organic electrochemical neurons and synapses with ion mediated spiking

Padinhare Cholakkal Harikesh et al.

Summary: This study presents the development of organic electrochemical neurons (OECNs) with ion-modulated spiking, based on all-printed complementary organic electrochemical transistors. The OECNs demonstrate facile bio-integration with Venus Flytrap, showing potential for integration with biological signaling systems. The integration of artificial neuromorphic devices with biological systems is of fundamental importance for future brain-machine interfaces, prosthetics, and intelligent soft robotics.

NATURE COMMUNICATIONS (2022)

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Review Chemistry, Multidisciplinary

High-resolution transmission electron microscopy of beam-sensitive halide perovskites

Biao Yuan et al.

Summary: This paper reviews the development of halide perovskites and discusses the challenges in observing their microstructures under electron-beam microscopy. It proposes a better methodology for image interpretation and suggests that this approach may also benefit imaging of other beam-sensitive materials.

CHEM (2022)

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Review Chemistry, Physical

Molecular packing and film morphology control in organic electrochemical transistors

Min Zhu et al.

Summary: Organic electrochemical transistors (OECTs) based on conjugated polymers have gained significant interest in flexible bioelectronics due to their high transconductance, low operating voltage, and good biocompatibility. The performance of OECTs is influenced by the mixed ionic and electronic transport properties of organic semiconductors, which in turn are determined by molecular packing and film morphology. While efforts have been made on new polymer structures, the relationship among chemical structure, molecular packing, film morphology, and OECT performance is still not fully explored.

MOLECULAR SYSTEMS DESIGN & ENGINEERING (2022)

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Article Chemistry, Physical

Tandem Organic Solar Cell with 20.2% Efficiency

Zhong Zheng et al.

Summary: A advanced interconnecting layer for tandem organic solar cell is developed in this study. By controlling the O-2 flux during evaporation, efficient electron extraction and low Schottky barrier are obtained, enabling effective charge recombination between two subcells. The tandem cell with the interconnecting layer shows a high efficiency of 20.27%.

JOULE (2022)

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Review Polymer Science

Resonant soft X-ray scattering in polymer science

Brian A. Collins et al.

Summary: Resonant soft X-ray scattering (RSoXS) is an emerging technique used to probe the structure of polymers and other molecules, offering unique chemical and bond-orientation sensitivity. Through years of development, it has evolved from a niche technique for organic electronic thin films to a mature tool applicable to various polymeric and molecular systems.

JOURNAL OF POLYMER SCIENCE (2022)

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Review Polymer Science

Extrusion 3D printing of conjugated polymers

Alex Chortos

Summary: Conjugated polymers are utilized in various applications such as biointerfaces, actuators, and energy storage, benefiting from their ability to transport ions and electronic currents in 3D structures. Extrusion-based 3D printing is a versatile approach compatible with multimaterial fabrication processes, allowing for the fabrication of conjugated polymers with different properties by adjusting ink designs. This review summarizes the progress in 3D printed conjugated polymers using three extrusion printing processes and discusses strategies for modifying ink rheology and conductivity for direct ink writing.

JOURNAL OF POLYMER SCIENCE (2022)

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Review Chemistry, Multidisciplinary

Two-Dimensional Field-Effect Transistor Sensors: The Road toward Commercialization

Changhao Dai et al.

Summary: This review summarizes the latest advances of 2D-materials-based FET sensors, including materials, operating principles, fabrication technologies, applications, and commercialization. The advantages of 2D materials include label-free detection, fast response, easy operation, and integration capability. The commercialization of these sensors still faces challenges but there are solutions and commercial prototypes emerging.

CHEMICAL REVIEWS (2022)

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Article Chemistry, Physical

Side Chain Engineering: Achieving Stretch-Induced Molecular Orientation and Enhanced Mobility in Polymer Semiconductors

Yafei Ding et al.

Summary: In this study, a side chain engineering strategy was developed to enhance the molecular orientation and charge transport of polymer semiconductors during stretching. Increasing the length of silicon chains improved the charge mobility and stretchability of the material.

CHEMISTRY OF MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Molecular Design of Stretchable Polymer Semiconductors: CurrentProgress and Future Directions

Yu Zheng et al.

Summary: Stretchable polymer semiconductors have rapidly advanced in recent years, allowing them to retain their electrical functionalities under repeated mechanical deformations. They have achieved charge-carrier mobilities on par with flexible polymer semiconductors and even surpassed amorphous silicon. This is due to molecular design concepts that enable multiple strain energy-dissipation mechanisms while maintaining efficient charge-transport pathways.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Polymer Science

Understanding Solution State Conformation and Aggregate Structure of Conjugated Polymers via Small Angle X-ray Scattering

Justin J. Kwok et al.

Summary: In this study, an in-depth small-angle X-ray scattering (SAXS) analysis was performed to reveal the solution state structure and aggregation behavior of donor-acceptor (D-A) conjugated polymers. By modeling and fitting the SAXS profiles, information about conformation and multiscale aggregation was extracted, and the physical origin of observed but unaddressed or misinterpreted features in scattering patterns was clarified. Additionally, the findings from SAXS were corroborated with electron microscopy observation, further confirming the accuracy of the conclusions. These results are important for understanding and controlling the morphology and electronic performance of D-A polymers.

MACROMOLECULES (2022)

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Article Multidisciplinary Sciences

High-brightness all-polymer stretchable LED with charge-trapping dilution

Zhitao Zhang et al.

Summary: Researchers have developed stretchable all-polymer-based light-emitting diodes with high brightness, current efficiency, and stretchability. The stretchable LEDs can be colored red, green, and blue, and are capable of on-skin wireless powering and real-time displaying of pulse signals. This advancement is significant for the development of high-performance stretchable displays.

NATURE (2022)

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Article Chemistry, Physical

Single-junction organic solar cells with over 19% efficiency enabled by a refined double-fibril network morphology

Lei Zhu et al.

Summary: Morphological control of donor and acceptor domains is crucial for efficient organic photovoltaics, and this study demonstrates a double-fibril network strategy to achieve a high power conversion efficiency of 19.3%.

NATURE MATERIALS (2022)

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Review Polymer Science

Progress of Conjugated Polymers as Emerging Thermoelectric Materials

Suhao Wang et al.

Summary: Thanks to the combined efforts of scientists in various research fields, there have been significant advancements in the past decade in the application of conjugated polymers as thermoelectric materials. However, there is a lack of systematic evaluations on the impact of molecular design on thermoelectric properties. A comprehensive understanding of the relationship between molecular structure and thermoelectric properties will facilitate the rational design of next-generation thermoelectric polymers.

PROGRESS IN POLYMER SCIENCE (2022)

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Article Multidisciplinary Sciences

Chiral emergence in multistep hierarchical assembly of achiral conjugated polymers

Kyung Sun Park et al.

Summary: By studying the assembly process of achiral conjugated polymers, the authors discovered the emergence of chirality and the formation of hierarchical helical structures. This study has significant implications for the development of chiral (opto)electronics.

NATURE COMMUNICATIONS (2022)

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Article Multidisciplinary Sciences

Seeing structural evolution of organic molecular nano-crystallites using 4D scanning confocal electron diffraction (4D-SCED)

Mingjian Wu et al.

Summary: This study introduces a method called 4D-SCED, which enables in situ observation of the evolution of organic molecular nanocrystals. The method records high-resolution diffraction patterns with lower dose, and has been successfully applied to the active layer in organic solar cells.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Multidisciplinary

Not All Aggregates Are Made the Same: Distinct Structures of Solution Aggregates Drastically Modulate Assembly Pathways, Morphology, and Electronic Properties of Conjugated Polymers

Zhuang Xu et al.

Summary: The structures of solution aggregates of conjugated polymers are modulated by tuning the solvent selectivity, which leads to three distinct assembly pathways. It is demonstrated that amorphous solution aggregates result in significantly improved alignment and reduced disorder in the solid state, leading to enhanced thin-film performance.

ADVANCED MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Polymer Photoelectrodes for Solar Fuel Production: Progress and Challenges

Madasamy Thangamuthu et al.

Summary: Polymer photoelectrodes, composed of earth-abundant elements, offer economic sustainability and easily tunable electronic structure for practical applications.

CHEMICAL REVIEWS (2022)

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Review Chemistry, Multidisciplinary

Renewed Prospects for Organic Photovoltaics

Guichuan Zhang et al.

Summary: Organic photovoltaics (OPVs) have undergone three stages of development, including optimizing bulk heterojunctions, improving donor-acceptor match, and developing non-fullerene acceptors (NFAs). NFAs have resulted in higher power conversion efficiencies (PCEs) surpassing 15% due to reduced energy losses and increased quantum efficiencies. The review provides an update on recent progress in OPV technology, including novel NFAs and donors, understanding structure-property relationships, and commercialization challenges.

CHEMICAL REVIEWS (2022)

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Article Multidisciplinary Sciences

A solution-processed n-type conducting polymer with ultrahigh conductivity

Haoran Tang et al.

Summary: This research introduces a facilely synthesized highly conductive n-type polymer with breakthrough conductivity and solution processability. By improving doping efficiency, the polymer achieves a doping level of almost 0.9 charges per repeating unit. Further investigations demonstrate the coherent charge-transport properties and existence of metallic state. The benchmark performances in electrochemical transistors and thermoelectric generators are also demonstrated.

NATURE (2022)

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Review Chemistry, Multidisciplinary

Temperature Induced Aggregation of Organic Semiconductors

Baocai Du et al.

Summary: This review summarizes the temperature-induced aggregation behaviors of organic semiconductors at different processing stages, and discusses the influences of different aggregation states on optoelectronic properties.

CHEMISTRY-A EUROPEAN JOURNAL (2021)

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Review Chemistry, Multidisciplinary

Polymerized Small-Molecule Acceptors for High-Performance All-Polymer Solar Cells

Zhi-Guo Zhang et al.

Summary: All-polymer solar cells have attracted significant research interest due to their good film formation, stable morphology, and mechanical flexibility. The strategy of polymerizing small-molecule acceptors to construct new-generation polymer acceptors has significantly increased the power conversion efficiency, but current challenges and future prospects still need to be addressed.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Systematic Investigation of Solution-State Aggregation Effect on Electrical Conductivity in Doped Conjugated Polymers

Yang-Yang Zhou et al.

Summary: This study developed four isoindigo-based conjugated polymers to investigate the relationship between solution-state aggregation, molecular doping process, and charge transport properties. The characterization revealed that one of the polymers, IIDDT-C3, exhibited the highest electrical conductivity due to its well-differentiated aggregate sizes and excellent aggregate connectivity in solutions.

CCS CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Dipeptide Nanostructure Assembly and Dynamics via in Situ Liquid-Phase Electron Microscopy

Karthikeyan Gnanasekaran et al.

Summary: This study reports the in situ growth of FF nanotubes examined via liquid-cell transmission electron microscopy (LCTEM), revealing the growth mechanism and structure formation process. The radial growth profile of the nanotubes was observed in real-time, with direct observation of the increase in diameter. Post-mortem techniques were used to verify and evaluate the performance of peptides and the assemblies they form.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Amphipathic Side Chain of a Conjugated Polymer Optimizes Dopant Location toward Efficient N-Type Organic Thermoelectrics

Jian Liu et al.

Summary: The use of amphipathic side chains in an n-type donor-acceptor copolymer selectively increases the Seebeck coefficient and improves the power factor by a factor of approximately 5. The alkyl spacer reduces energetic disorder, controls dopant sites, and minimizes the adverse influence of counterions. This molecular strategy optimizes the Seebeck coefficient and offers a new approach to improving n-type polymeric thermoelectrics by optimizing dopant location.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Persistent Conjugated Backbone and Disordered Lamellar Packing Impart Polymers with Efficient n-Doping and High Conductivities

Yang Lu et al.

Summary: A simple solution-based co-deposition method has been reported to achieve high conductivity n-doped polymers. These polymers exhibit surprising structural tolerance and excellent miscibility with commonly used n-dopants, allowing high concentrations and high mobility of charge carriers simultaneously, resulting in excellent electrical conductivity and thermoelectric performance.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Thermally Activated n-Doping of Organic Semiconductors Achieved by N-Heterocyclic Carbene Based Dopant

Yi-Fan Ding et al.

Summary: The article introduces a thermally activated n-dopant DMImC with excellent stability, which has been successfully used for doping organic semiconductors, achieving high electrical conductivity.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Efficient n-Doping of Polymeric Semiconductors through Controlling the Dynamics of Solution-State Polymer Aggregates

Miao Xiong et al.

Summary: The miscibility issue in n-doped polymeric semiconductors can be overcome by modulating the solution-state aggregates of conjugated polymers, leading to high doping efficiency and charge-carrier mobility. This method can also be applied to improve the doping efficiency of other polymer systems with different aggregation tendencies.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

When Assembly Meets Processing: Tuning Multiscale Morphology of Printed Conjugated Polymers for Controlled Charge Transport

Kyung Sun Park et al.

Summary: Conjugated polymers are emerging as an attractive class of semiconductors for next-generation electronics due to their low cost, high-throughput solution processability, mechanical flexibility, self-healing properties, and ability to interface with biological systems. Studies in the past four decades have contributed to a thorough understanding of conjugated polymers, with assembly and crystallization behavior being key factors influencing electronic performance. However, the complex solution processing environment and rapid kinetics make it challenging to fully understand the assembly process.

CHEMISTRY OF MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Organic Photovoltaics: Understanding the Preaggregation of Polymer Donors in Solution and Its Morphological Impact

Tonghui Wang et al.

Summary: This study uses thermodynamic analysis, molecular dynamics simulations, and density functional theory calculations to establish the χ value as a useful figure of merit for evaluating the extent of polymer aggregation in solution, and explores how intermolecular interactions between polymers and solvents contribute to the variations in χ values. By examining four representative polymer donors in solution, the research provides a detailed description of the relationships among intermolecular interactions, polymer solution aggregation, and morphological features of the active layers with χ as a robust bridge.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Cyano-Functionalized Bithiophene Imide-Based n-Type Polymer Semiconductors: Synthesis, Structure-Property Correlations, and Thermoelectric Performance

Kui Feng et al.

Summary: In this study, a series of novel acceptor building blocks, CNI, CNTI, and CNDTI, were successfully developed by introducing strong electron-withdrawing cyano functionality on BTI and its derivatives. Based on these novel building blocks, high-performance n-type polymers with deep-positioned LUMOs were synthesized, showing excellent stability and doping efficiency. These polymers exhibit the highest electrical conductivity of 23.3 S m-1 and a power factor of up to 10 mu W m-1 K-2, which are among the highest values reported for solution-processed molecularly n-doped polymers.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Review Polymer Science

Multicomponent Polymerization for π-Conjugated Polymers

Ki-Young Yoon et al.

Summary: Multicomponent polymerization is an efficient method for synthesizing complex pi-conjugated polymers from simple building blocks. This feature article outlines several strategies for multicomponent polymerization and discusses the challenges and outlooks in the field.

MACROMOLECULAR RAPID COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

A tied Fermi liquid to Luttinger liquid model for nonlinear transport in conducting polymers

Jiawei Wang et al.

Summary: In this study, the nonlinear charge transport in conducting polymers was investigated by varying the crystalline degrees of samples. A heterogeneous-resistive-network model based on the link between Fermi liquids and Luttinger liquids was proposed to explain the nonlinear transport behaviors. The model was supported by precise electrical and microstructural characterizations, providing new insights into microstructure-correlated charge transport in organic solids.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Approaching Crystal Structure and High Electron Mobility in Conjugated Polymer Crystals

Ze-Fan Yao et al.

Summary: Conjugated polymers often have both crystallized and amorphous regions in the solid state, making it challenging to accurately determine their precise microstructures. This study obtained crystals of two typical conjugated polymers through a controlled self-assembly process, allowing for the determination of crystal structures using X-ray techniques and molecular simulations. The highly oriented polymer chains in the crystals exhibit higher mobilities and lower hopping energy barriers compared to spin-coated thin films.

ADVANCED MATERIALS (2021)

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Article Physics, Applied

3D structure-property correlations of electronic and energy materials by tomographic atomic force microscopy

Jingfeng Song et al.

Summary: The tomographic atomic force microscopy technique has shown great potential in the 3D nanocharacterization of energy and electronic materials, offering new avenues for investigating fundamental and applied phenomena in a broader range of functional materials.

APPLIED PHYSICS LETTERS (2021)

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Article Polymer Science

Role of Molecular Weight in Microstructural Transition and Its Correlation to the Mechanical and Electrical Properties of P(NDI2OD-T2) Thin Films

Kefeng Zhao et al.

Summary: The study investigated the effects of molecular weight on the behavior, microstructures, charge carrier mobility, and mechanical properties of donor-acceptor conjugated polymers. It was found that different molecular weights of P(NDI2OD-T2) led to varying states in solution and distinct impacts on film microstructures and electrical performances.

MACROMOLECULES (2021)

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Article Polymer Science

Optimizing the Crystallization Behavior and Film Morphology of Donor-Acceptor Conjugated Semiconducting Polymers by Side-Chain-Solvent Interaction in Nonpolar Solvents

Hongxiang Li et al.

Summary: By regulating the interaction between the polymer side chain and solvent, the film formation process and morphology were effectively controlled, maintaining highly ordered aggregates in the drop-casting film. This precise adjustment of the solution state played a crucial role in optimizing device performance.

MACROMOLECULES (2021)

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Article Multidisciplinary Sciences

High-frequency and intrinsically stretchable polymer diodes

Naoji Matsuhisa et al.

Summary: This paper presents an intrinsically stretchable diode based on stretchable organic and nanomaterials, capable of operating at a frequency as high as 13.56 megahertz. This advancement enables enhanced functionalities and capabilities for skin-like wearable electronics.

NATURE (2021)

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Article Polymer Science

Nucleation and Growth of P(NDI2OD-T2) Nanowires via Side Chain Ordering and Backbone Planarization

Kefeng Zhao et al.

Summary: By controlling the side chain ordering and backbone planarization processes, we successfully prepared P(NDI2OD-T2) conjugated polymer nanowires. This method allows the nucleation pathway to be controlled using selective solvents, thereby altering the final film morphology.

MACROMOLECULES (2021)

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Article Multidisciplinary Sciences

Approaching disorder-tolerant semiconducting polymers

Xinwen Yan et al.

Summary: By carefully designing the structure of conjugated polymers, their tolerance to disorder induced by doping can be increased, leading to better n-doping efficiency and higher electrical conductivity.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Molecular design revitalizes the low-cost PTV-polymer for highly efficient organic solar cells

Junzhen Ren et al.

Summary: In this study, a new ester substituted poly(thiophene vinylene) derivative, PTVT-T, was successfully synthesized with commercially available raw materials. PTVT-T showed excellent compatibility with fullerene- and NF-based acceptors, exhibiting high efficiency in OSCs. With a power conversion efficiency of 16.20% in a PTVT-T:BTP-eC9-based device, this work demonstrates the huge potential of PTVT-T for the future commercialization of OSCs.

NATIONAL SCIENCE REVIEW (2021)

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Article Chemistry, Multidisciplinary

Alignment of linear polymeric grains for highly stable N-type thin-film transistors

Yingying Jiang et al.

Summary: The study finds that polyacrylonitrile can significantly affect the sizes of pre-aggregates of polymers in solutions and stabilize electron mobility over a wide range of temperatures. The linear-grain morphology of the film contributed to reducing the holes and grain boundaries in the transport paths of carriers.

CHEM (2021)

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Article Polymer Science

Unraveling the Unconventional Order of a High-Mobility Indacenodithiophene-Benzothiadiazole Copolymer

Camila Cendra et al.

Summary: This study demonstrates the use of low-dose transmission electron microscopy to investigate the nanoscale and mesoscale organization of a new donor-acceptor copolymer. The analysis revealed the presence of nanocrystallites and short-range order within the material, providing insights into its rich mesoscale organization.

ACS MACRO LETTERS (2021)

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Review Chemistry, Multidisciplinary

4D-STEM of Beam-Sensitive Materials

Karen C. Bustillo et al.

Summary: 4DS-TEM, also known as scanning electron nanobeam diffraction, is a powerful approach to elucidate structure in soft materials that are challenging to image in transmission electron microscopes. By careful control of experimental parameters, beam damage to samples can be minimized, leading to high-quality structural images.

ACCOUNTS OF CHEMICAL RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Molecular Weight Engineering in High-Performance Ambipolar Emissive Mesopolymers

Xiaofei Guo et al.

Summary: This study demonstrates the potential of mesopolymers with high solubility, free of structural defects, and tunable molecular weights in organic optoelectronics, particularly in the construction of organic light emitting transistors with strong emission and ambipolar carrier mobility.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Achieving over 10 % Efficiency in Poly(3-hexylthiophene)-based Organic Solar Cells via Solid Additives

Chenyi Yang et al.

Summary: This study aimed to improve the performance of P3HT-based organic solar cells by using solid and solvent additives. The solid additive (SA4) resulted in a more ordered molecular packing and phase separation, leading to a higher power conversion efficiency (PCE) of over 10% for the first time in P3HT-based OSCs.

CHEMSUSCHEM (2021)

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Article Multidisciplinary Sciences

Determining the three-dimensional atomic structure of an amorphous solid

Yao Yang et al.

Summary: This study developed an atomic electron tomography reconstruction method to experimentally determine the 3D atomic positions of an amorphous solid, successfully characterizing the short- and medium-range order of the 3D atomic arrangement. The research identified four types of crystal-like medium-range order and provided direct experimental evidence to support the efficient cluster packing model for metallic glasses.

NATURE (2021)

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Review Physics, Multidisciplinary

Multi-level aggregation of conjugated small molecules and polymers: from morphology control to physical insights

Qi-Yi Li et al.

Summary: The article focuses on the aggregation of conjugated small molecules and polymers and their impact on optoelectronic properties, emphasizing the importance of aggregation and the relationship between multi-scale structures and properties. The whole process from molecules to devices is subdivided into several parts, summarizing the progress and challenges of the relationship between optoelectronic properties and multi-level aggregation.

REPORTS ON PROGRESS IN PHYSICS (2021)

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Article Multidisciplinary Sciences

A high-conductivity n-type polymeric ink for printed electronics

Chi-Yuan Yang et al.

Summary: The team reported an alcohol-based, high-performance, and stable n-type conductive ink with high electrical conductivity and stability, which is of great significance for the realization of high-performance organic electronic devices.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Multidisciplinary

Achieving Efficient n-Doping of Conjugated Polymers by Molecular Dopants

Yang Lu et al.

Summary: Molecular doping is a central proposition in organic electronics, involving intermolecular charge transfer between organic conjugated materials and molecular dopants. While there is a focus on improving p-doping efficiency and electrical conductivity, the development of n-type molecular doping lags behind. Efficient p- and n-type molecular doping are both essential for organic electronic devices, emphasizing the need to achieve efficient n-doping in conjugated polymers.

ACCOUNTS OF CHEMICAL RESEARCH (2021)

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Review Chemistry, Multidisciplinary

Cryogenic Electron Microscopy for Energy Materials

Zewen Zhang et al.

Summary: The development of clean energy technologies, such as high energy density batteries and high efficiency solar cells, relies on a deep understanding of key materials and processes at atomic and molecular levels. Cryogenic electron microscopy (cryo-EM) is emerging as a powerful tool to investigate sensitive materials in energy science, providing opportunities for breakthroughs and discoveries. Low-temperature methods can protect and stabilize reactive components, offering insights into materials design and practical applications in energy research.

ACCOUNTS OF CHEMICAL RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Single-Junction Organic Photovoltaic Cell with 19% Efficiency

Yong Cui et al.

Summary: By combining material design and ternary blending strategy, a maximum power conversion efficiency of 19.0% is achieved in single-junction OPV cells. Optimized active layer structure significantly improves the photovoltaic parameters, enhancing the performance and PCE values of the cells.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

Metalloporphyrin-based D-A type conjugated organic polymer nanotube for efficient photocatalytic degradation

Jun Han et al.

Summary: A series of porphyrin-based D-A type conjugated organic polymer nanotubes were synthesized via acid-catalyzed Schiff base reaction. Among them, CuTAPP-BT showed superior photocatalytic activity and recyclability for BPA degradation.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Polymer Science

Evolution of Chain Dynamics and Oxidation States with Increasing Chain Length for a Donor-Acceptor-Conjugated Oligomer Series

Saadia Chaudhry et al.

Summary: This study investigates the effects of chain length on the properties of donor-acceptor conjugated organic materials by synthesizing oligomers and polymers with varying chain lengths. It reveals a convergence limit between small molecule and polymer behavior at around 15 units, highlighting the synergy between chain length and oxidation state properties. The study also demonstrates the importance of chain length in influencing material properties and property transitions as a function of chain length.

MACROMOLECULES (2021)

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Article Polymer Science

Controllable Transformation between the Kinetically and Thermodynamically Stable Aggregates in a Solution of Conjugated Polymers

Li Ding et al.

Summary: The study focused on unraveling the energy landscape of conjugated polymers during aggregation and investigating the energetic and structural information of the thermodynamically and kinetically stable aggregates. Through rational molecular design and thermodynamic control, stable aggregates of NDI-based polymers were obtained. The analysis of energetic and structural information provided insights into the relations among the structure, morphology, and properties of conjugated polymers at the molecular level.

MACROMOLECULES (2021)

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Article Materials Science, Multidisciplinary

py4DSTEM: A Software Package for Four-Dimensional Scanning Transmission Electron Microscopy Data Analysis

Benjamin H. Savitzky et al.

Summary: STEM enables imaging, diffraction, and spectroscopy of materials at various length scales, producing rich 4D-STEM datasets. The py4DSTEM analysis toolkit, written in Python, aims to extract material properties through complex analysis pipelines, with the goal of improving standards in electron microscopy data and methods.

MICROSCOPY AND MICROANALYSIS (2021)

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Article Multidisciplinary Sciences

Monolithic optical microlithography of high-density elastic circuits

Yu-Qing Zheng et al.

Summary: This study presents a monolithic optical microlithographic process that directly micro-patterns a set of elastic electronic materials by sequential ultraviolet light-triggered solubility modulation. The experimental results show the ability to fabricate transistors with a channel length of 2 micrometers at high density, as well as the fabrication of multiple elastic circuits.

SCIENCE (2021)

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Article Multidisciplinary Sciences

A design strategy for high mobility stretchable polymer semiconductors

Jaewan Mun et al.

Summary: This study presents a simple and universal strategy to achieve intrinsically stretchable semiconducting polymers with controlled multi-scale ordering, improving their stretchability and mechanical reversibility. By incorporating two types of co-monomer units, overall crystallinity and longer-range orders are reduced while maintaining high mobility, leading to improved mechanical properties. The proposed molecular design concept is observed to be applicable to various conjugated polymer systems, resulting in enhanced mechanical properties.

NATURE COMMUNICATIONS (2021)

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Article Multidisciplinary Sciences

Ultrafast, sensitive, and portable detection of COVID-19 IgG using flexible organic electrochemical transistors

Hong Liu et al.

Summary: A rapid, low-cost, and portable SARS-CoV-2 IgG detection platform based on OECTs was reported, with remote control via mobile phone. By optimizing ion concentrations and pH values, specific detection of the virus was achieved in minutes, showing promise in the diagnosis and prognosis of COVID-19.

SCIENCE ADVANCES (2021)

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Article Multidisciplinary Sciences

Small-angle X-ray and neutron scattering

Cy M. Jeffries et al.

Summary: Small-angle scattering (SAS) is a technique used to probe the structural organization of matter and quantify its response to changes in external conditions. By analyzing SAS data, information about length scale distributions of material components can be obtained. This method is widely used in structural biology as well as in the soft-matter and hard-matter sciences.

NATURE REVIEWS METHODS PRIMERS (2021)

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Article Chemistry, Multidisciplinary

Building crystal structures of conjugated polymers through X-ray diffraction and molecular modeling

Ze-Fan Yao et al.

Summary: This study establishes possible crystal structures of eight typical conjugated polymers and models their packing structures based on synchrotron X-ray diffractions and molecular simulations. The crystal structures serve as a new platform to predict the packing structures of more related polymer systems, extending the molecular scope. The polymer crystal structure database enables the prediction of multiscale microstructures and charge transport properties of conjugated polymers before experiments, eliminating trial-and-error approaches and accelerating the design of high-performance conjugated polymers.

SMARTMAT (2021)

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Article Chemistry, Multidisciplinary

Influence of solution-state aggregation on conjugated polymer crystallization in thin films and microwire crystals

Yu-Qing Zheng et al.

Summary: This study systematically investigated the effect of side chain engineering on solution-state aggregation, crystallization, and charge transport in BDOPV-based conjugated polymers. The results demonstrate that subtle differences in side chain chemical structures significantly influence the organization of intermolecular displacements and crystalline domain sizes in microwires and thin films. Furthermore, it was found that far branched side chains lead to larger polymer aggregates in solution and larger crystalline domains in solid films, ultimately increasing electron mobility with values surpassing 10 cm(2) V-1 s(-1).

GIANT (2021)

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Article Chemistry, Multidisciplinary

High-performance polymer field-effect transistors: from the perspective of multi-level microstructures

Ze-Fan Yao et al.

Summary: The multi-level microstructure of conjugated polymers plays a critical role in determining the performance of FETs. Controlling molecular structures, solution-state aggregation, and polymer crystal structures is essential for developing high-performance polymer FETs. By tuning polymer hierarchical microstructures, guidelines can be provided for the advancement of polymer electronics.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Engineering the Interfacial Materials of Organic Field-Effect Transistors for Efficient Charge Transport

Deyang Ji et al.

Summary: Efficient charge transport in OFETs is crucial for constructing high-performance devices and further understanding the intrinsic properties of organic semiconductor materials. Research on interface materials and related interface engineering offers a promising approach for optimizing charge transport capabilities.

ACCOUNTS OF MATERIALS RESEARCH (2021)

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Review Chemistry, Physical

Organic mixed ionic-electronic conductors

Bryan D. Paulsen et al.

NATURE MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A High-Performance Solution-Processed Organic Photodetector for Near-Infrared Sensing

Jianfei Huang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Controlling the Microstructure of Conjugated Polymers in High-Mobility Monolayer Transistors via the Dissolution Temperature

Mengmeng Li et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Organic Semiconducting Materials Based on BDOPV: Structures, Properties, and Applications

Li Ding et al.

CHINESE JOURNAL OF CHEMISTRY (2020)

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Article Chemistry, Multidisciplinary

Graphene Liquid Cells Assembled through Loop-Assisted Transfer Method and Located with Correlated Light-Electron Microscopy

Pauline M. G. van Deursen et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Benzo[1,2-b:4,5-c′]Dithiophene-4,8-Dione-Based Polymer Donor Achieving an Efficiency Over 16%

Pengjie Chao et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Molecular Semiconductors for Logic Operations: Dead-End or Bright Future?

Guillaume Schweicher et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Imaging Beam-Sensitive Materials by Electron Microscopy

Qiaoli Chen et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Solution-Processed Transparent Electrodes for Emerging Thin-Film Solar Cells

Yaokang Zhang et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Covalent Organic Frameworks: Design, Synthesis, and Functions

Keyu Geng et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Physical

Origin of the High Donor Acceptor Composition Tolerance in Device Performance and Mechanical Robustness of All-Polymer Solar Cells

Jin-Woo Lee et al.

CHEMISTRY OF MATERIALS (2020)

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Article Polymer Science

Closing the Stability-Performance Gap in Organic Thermoelectrics by Adjusting the Partial to Integer Charge Transfer Ratio

Osnat Zapata-Arteaga et al.

MACROMOLECULES (2020)

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Review Nanoscience & Nanotechnology

Scalable fabrication and coating methods for perovskite solar cells and solar modules

Nam-Gyu Park et al.

NATURE REVIEWS MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Distannylated Bithiophene Imide: Enabling High-Performance n-Type Polymer Semiconductors with an Acceptor-Acceptor Backbone

Yongqiang Shi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Multidisciplinary

Electrically Conductive Metal-Organic Frameworks

Lilia S. Xie et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Conformation Control of Conjugated Polymers

Zi-Di Yu et al.

CHEMISTRY-A EUROPEAN JOURNAL (2020)

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Article Multidisciplinary Sciences

18% Efficiency organic solar cells

Qishi Liu et al.

SCIENCE BULLETIN (2020)

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Article Polymer Science

Impact of Molecular Weight on the Mechanical and Electrical Properties of a High-Mobility Diketopyrrolopyrrole-Based Conjugated Polymer

Dandan Pei et al.

MACROMOLECULES (2020)

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Article Nanoscience & Nanotechnology

Achieving High Alignment of Conjugated Polymers by Controlled Dip-Coating

Qi-Yi Li et al.

ADVANCED ELECTRONIC MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Progress in Stability of Organic Solar Cells

Duan Leiping et al.

ADVANCED SCIENCE (2020)

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Editorial Material Multidisciplinary Sciences

Polymer-based bioelectronics go self-powered

Peiyun Li et al.

SCIENCE BULLETIN (2020)

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Review Chemistry, Physical

Charge transport in high-mobility conjugated polymers and molecular semiconductors

Simone Fratini et al.

NATURE MATERIALS (2020)

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Article Chemistry, Multidisciplinary

In Situ Grazing-Incidence Wide-Angle Scattering Reveals Mechanisms for Phase Distribution and Disorientation in 2D Halide Perovskite Films

Justin M. Hoffman et al.

ADVANCED MATERIALS (2020)

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Review Chemistry, Multidisciplinary

The Bulk Heterojunction in Organic Photovoltaic, Photodetector, and Photocatalytic Applications

Andrew Wadsworth et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Ordered Solid-State Microstructures of Conjugated Polymers Arising from Solution-State Aggregation

Ze-Fan Yao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

High-Performance n-Type Polymer Semiconductors: Applications, Recent Development, and Challenges

Huiliang Sun et al.

CHEM (2020)

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Article Chemistry, Multidisciplinary

The Critical Role of Dopant Cations in Electrical Conductivity and Thermoelectric Performance of n-Doped Polymers

Yang Lu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Multidisciplinary Sciences

A thermally activated and highly miscible dopant for n-type organic thermoelectrics

Chi-Yuan Yang et al.

NATURE COMMUNICATIONS (2020)

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Article Polymer Science

Elucidating the Influence of Side-Chain Circular Distribution on the Crack Onset Strain and Hole Mobility of Near-Amorphous Indacenodithiophene Copolymers

Parker J. W. Sommerville et al.

MACROMOLECULES (2020)

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Article Polymer Science

Chain Conformation and Aggregation Structure Formation of a High Charge Mobility DPP-Based Donor-Acceptor Conjugated Polymer

Chang Liu et al.

MACROMOLECULES (2020)

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Article Multidisciplinary Sciences

Random terpolymer based on thiophene-thiazolothiazole unit enabling efficient non-fullerene organic solar cells

Jingnan Wu et al.

NATURE COMMUNICATIONS (2020)

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Review Materials Science, Multidisciplinary

Meniscus-guided coating of organic crystalline thin films for high-performance organic field-effect transistors

Zhengjun Lu et al.

JOURNAL OF MATERIALS CHEMISTRY C (2020)

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Article Polymer Science

Precise tracking and modulating aggregation structures of conjugated copolymers in solutions

Zi-Yuan Wang et al.

POLYMER CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Advances in Conjugated Microporous Polymers

Jet-Sing M. Lee et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Organic field-effect transistor-based flexible sensors

Saravanan Yuvaraja et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Review Physics, Multidisciplinary

A review of non-fullerene polymer solar cells: from device physics to morphology control

Robert S. Gurney et al.

REPORTS ON PROGRESS IN PHYSICS (2019)

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Article Multidisciplinary Sciences

Printed subthreshold organic transistors operating at high gain and ultralow power

Chen Jiang et al.

SCIENCE (2019)

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Review Nanoscience & Nanotechnology

Recent Advances in n-Type Thermoelectric Nanocomposites

Junhui Tang et al.

ADVANCED ELECTRONIC MATERIALS (2019)

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Review Nanoscience & Nanotechnology

Advances in n-Type Organic Thermoelectric Materials and Devices

Yimeng Sun et al.

ADVANCED ELECTRONIC MATERIALS (2019)

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Article Nanoscience & Nanotechnology

Progress in Nickel-Coordinated Polymers as Intrinsically Conducting n-Type Thermoelectric Materials

Akanksha K. Menon et al.

ADVANCED ELECTRONIC MATERIALS (2019)

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Review Nanoscience & Nanotechnology

Thermoelectric Properties of PEDOT:PSS

Zeng Fan et al.

ADVANCED ELECTRONIC MATERIALS (2019)

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Article Chemistry, Multidisciplinary

A Multiparameter Pressure-Temperature-Humidity Sensor Based on Mixed Ionic-Electronic Cellulose Aerogels

Shaobo Han et al.

ADVANCED SCIENCE (2019)

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Article Chemistry, Multidisciplinary

An Evolvable Organic Electrochemical Transistor for Neuromorphic Applications

Jennifer Y. Gerasimov et al.

ADVANCED SCIENCE (2019)

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Article Multidisciplinary Sciences

Internal ion-gated organic electrochemical transistor: A building block for integrated bioelectronics

George D. Spyropoulos et al.

SCIENCE ADVANCES (2019)

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Article Chemistry, Physical

From Isotropic to Anisotropic Conductivities in P(NDI2OD-T2) by (Electro-)Chemical Doping Strategies

Yannic M. Gross et al.

CHEMISTRY OF MATERIALS (2019)

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Article Chemistry, Physical

Importance of Critical Molecular Weight of Semicrystalline n-Type Polymers for Mechanically Robust, Efficient Electroactive Thin Films

Joonhyeong Choi et al.

CHEMISTRY OF MATERIALS (2019)

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Review Materials Science, Multidisciplinary

Four-Dimensional Scanning Transmission Electron Microscopy (4D-STEM): From Scanning Nanodiffraction to Ptychography and Beyond

Colin Ophus

MICROSCOPY AND MICROANALYSIS (2019)

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Article Chemistry, Physical

Multi-scale ordering in highly stretchable polymer semiconducting films

Jie Xu et al.

NATURE MATERIALS (2019)

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Article Chemistry, Physical

Bringing Conducting Polymers to High Order: Toward Conductivities beyond 105 S cm-1 and Thermoelectric Power Factors of 2 mW m-1 K-2

Vishnu Vijayakumar et al.

ADVANCED ENERGY MATERIALS (2019)

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Article Chemistry, Physical

Understanding the Effects of Molecular Dopant on n-Type Organic Thermoelectric Properties

Hio-Ieng Un et al.

ADVANCED ENERGY MATERIALS (2019)

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Article Nanoscience & Nanotechnology

Diffusion-Limited Crystallization: A Rationale for the Thermal Stability of Non-Fullerene Solar Cells

Liyang Yu et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Review Chemistry, Multidisciplinary

In Situ Transmission Electron Microscopy for Energy Materials and Devices

Zheng Fan et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Rigid Coplanar Polymers for Stable n-Type Polymer Thermoelectrics

Yang Lu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Review Chemistry, Physical

Strategies To Enhance the Conductivity of n-Type Polymer Thermoelectric Materials

Yang Lu et al.

CHEMISTRY OF MATERIALS (2019)

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Article Chemistry, Physical

Diffraction imaging of nanocrystalline structures in organic semiconductor molecular thin films

Ouliana Panova et al.

NATURE MATERIALS (2019)

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Article Multidisciplinary Sciences

Impact of polymorphism on the optoelectronic properties of a low-bandgap semiconducting polymer

Mengmeng Li et al.

NATURE COMMUNICATIONS (2019)

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Review Chemistry, Multidisciplinary

The Effects of Side Chains on the Charge Mobilities and Functionalities of Semiconducting Conjugated Polymers beyond Solubilities

Yizhou Yang et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Physical

Influence of Acceptor Type and Polymer Molecular Weight on the Mechanical Properties of Polymer Solar Cells

Joonhyeong Choi et al.

CHEMISTRY OF MATERIALS (2019)

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Article Chemistry, Physical

Dopant-Induced Ordering of Amorphous Regions in Regiorandom P3HT

Patrick Y. Yee et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

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Review Chemistry, Multidisciplinary

Recent Efforts in Understanding and Improving the Nonideal Behaviors of Organic Field-Effect Transistors

Hio-leng Un et al.

ADVANCED SCIENCE (2019)

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Article Multidisciplinary Sciences

Tuning conformation, assembly, and charge transport properties of conjugated polymers by printing flow

Kyung Sun Park et al.

SCIENCE ADVANCES (2019)

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Article Chemistry, Multidisciplinary

Selenium-Substituted Diketopyrrolopyrrole Polymer for High-Performance p-Type Organic Thermoelectric Materials

Jiamin Ding et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Wafer-Scale Fabrication of High-Performance n-Type Polymer Monolayer Transistors Using a Multi-Level Self-Assembly Strategy

Ze-Fan Yao et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Fast Deposition of Aligning Edge-On Polymers for High-Mobility Ambipolar Transistors

Yingying Jiang et al.

ADVANCED MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Pyrazine-Flanked Diketopyrrolopyrrole (DPP): A New Polymer Building Block for High-Performance n-Type Organic Thermoelectrics

Xinwen Yan et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Nanoscience & Nanotechnology

Control of Crystallite Orientation in Diketopyrrolopyrrole-Based Semiconducting Polymers via Tuning of Intermolecular Interactions

Sung Yun Son et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Multidisciplinary

Kinetically Controlled Crystallization in Conjugated Polymer Films for High-Performance Organic Field-Effect Transistors

Yeon-Ju Kim et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Conjugated Donor-Acceptor Terpolymers Toward High-Efficiency Polymer Solar Cells

Dongfeng Dang et al.

ADVANCED MATERIALS (2019)

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Article Energy & Fuels

Fluorine Substituted Bithiophene Imide-Based n-Type Polymer Semiconductor for High-Performance Organic Thin-Film Transistors and All-Polymer Solar Cells

Huiliang Sun et al.

SOLAR RRL (2019)

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Article Chemistry, Physical

Single-Junction Organic Solar Cell with over 15% Efficiency Using Fused-Ring Acceptor with Electron-Deficient Core

Jun Yuan et al.

JOULE (2019)

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Article Polymer Science

Controlling aggregate formation in conjugated polymers by spin-coating below the critical temperature of the disorder-order transition

Markus Reichenberger et al.

JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS (2018)

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Review Chemistry, Physical

High Performance Thermoelectric Materials: Progress and Their Applications

Lei Yang et al.

ADVANCED ENERGY MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Enhancing Molecular n-Type Doping of Donor-Acceptor Copolymers by Tailoring Side Chains

Jian Liu et al.

ADVANCED MATERIALS (2018)

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Thiazole Imide-Based All-Acceptor Homopolymer: Achieving High-Performance Unipolar Electron Transport in Organic Thin-Film Transistors

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Engineered doping of organic semiconductors for enhanced thermoelectric efficiency

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Microstructure formation in molecular and polymer semiconductors assisted by nucleation agents

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Characterization of the morphology of solution-processed bulk heterojunction organic photovoltaics

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n-Doping of Organic Electronic Materials using Air-Stable Organometallics

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High-efficiency solution processable polymer photovoltaic cells by self-organization of polymer blends

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2005)

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MACROMOLECULAR RAPID COMMUNICATIONS (2005)

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Article Polymer Science

Dependence of regioregular poly(3-hexylthiophene) film morphology and field-effect mobility on molecular weight

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Effect of mesoscale crystalline structure on the field-effect mobility of regioregular poly(3-hexyl thiophene) in thin-film transistors

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MACROMOLECULES (2005)

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Enhancement of field-effect mobility due to surface-mediated molecular ordering in regioregular polythiophene thin film transistors

DH Kim et al.

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Article Chemistry, Physical

Control of carrier density by self-assembled monolayers in organic field-effect transistors

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NATURE MATERIALS (2004)

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High-performance semiconducting polythiophenes for organic thin-film transistors

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2004)

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Linear ladder-type π-conjugated polymers composed of fused thiophene ring systems

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MACROMOLECULES (2004)

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Chain-growth polymerization for poly(3-hexylthiophene) with a defined molecular weight and a low polydispersity

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Threshold voltage shift in organic field effect transistors by dipole monolayers on the gate insulator

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Enhanced mobility of poly(3-hexylthiophene) transistors by spin-coating from high-boiling-point solvents

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CHEMISTRY OF MATERIALS (2004)

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Review Chemistry, Multidisciplinary

Charge-transfer and energy-transfer processes in π-conjugated oligomers and polymers:: A molecular picture

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Chain growth mechanism for regioregular nickel-initiated cross-coupling polymerizations

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High electron mobility in ladder polymer field-effect transistors

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2003)

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The influence of mechanical rubbing on the field-effect mobility in polyhexylthiophene

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Polymer thin-film transistors with chemically modified dielectric interfaces

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APPLIED PHYSICS LETTERS (2002)

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Enhancement of electrical conductivity of poly(3,4-ethylenedioxythiophene)/poly(4-styrenesulfonate) by a change of solvents

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