4.7 Article

Chemically Fueled Dissipative Cross-Linking of Protein Hydrogels Mediated by Protein Unfolding

相关参考文献

注意:仅列出部分参考文献,下载原文获取全部文献信息。
Article Chemistry, Multidisciplinary

Tuning Protein Hydrogel Mechanics through Modulation of Nanoscale Unfolding and Entanglement in Postgelation Relaxation

Matt D. G. Hughes et al.

Summary: Globular folded proteins, as versatile nanoscale building blocks, can be used to create biomaterials with adjustable unfolding and entanglement behavior, which is beneficial for applications requiring responsive and dynamic modulation of mechanical properties and biological function.

ACS NANO (2022)

Article Chemistry, Multidisciplinary

Programming Dissipation Systems by DNA Timer for Temporally Regulating Enzyme Catalysis and Nanostructure Assembly

Zhaohui Qin et al.

Summary: This study demonstrates a DNA-based artificial dissipative system with a molecular timer, which allows for dynamic enzyme catalysis and DNA nanostructure disassembly. This provides a useful tool for the development of artificial reaction networks and intelligent nanostructures.

ACS NANO (2022)

Article Chemistry, Multidisciplinary

Biocatalytic cascades and intercommunicated biocatalytic cascades in microcapsule systems

Pu Zhang et al.

Summary: Biomolecule-loaded microcapsules with nucleic acid-functionalized hydrogel can enhance biocatalytic reactions. By controlling the assembly and connection of microcapsules, cascaded reactions with different enzymes can be achieved.

CHEMICAL SCIENCE (2022)

Article Chemistry, Multidisciplinary

Chemically Fueled Volume Phase Transition of Polyacid Microgels

Jonas Heckel et al.

Summary: This study introduces chemically fueled transient volume phase transitions for PMAA microgels, demonstrating controlled system behavior as a function of pH and fuel amount. Additionally, the technology showcased potential applications in transient encapsulation and time-programmed release.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

Article Nanoscience & Nanotechnology

Understanding Design Rules for Optimizing the Interface between Immobilized Enzymes and Random Copolymer Brushes

Hector Sanchez-Moran et al.

Summary: "The long-term goal of biotechnology is to develop design rules for stabilizing enzymes when immobilized to materials. By investigating the stabilization of lipases immobilized on PEGMA and SBMA copolymer brush surfaces, it was found that the stability of the lipases at elevated temperatures depended on the fraction of PEGMA in the brush layer. This understanding can lead to the rational tuning of enzyme-material interfaces for reliable ruggedization of enzymes under extreme conditions."

ACS APPLIED MATERIALS & INTERFACES (2021)

Article Chemistry, Multidisciplinary

Control of Nanoscale In Situ Protein Unfolding Defines Network Architecture and Mechanics of Protein Hydrogels

Matt D. G. Hughes et al.

Summary: This study demonstrates the critical role of protein unfolding in defining the architecture and mechanics of a photochemically cross-linked native protein network by controlling the force lability of bovine serum albumin. The nanoscale structure of proteins significantly affects network architecture and mechanics, highlighting the importance of in situ unfolding through nanoscale (un)stapling.

ACS NANO (2021)

Article Chemistry, Multidisciplinary

Chemically Fueled Three-State Chiroptical Switching Supramolecular Gel with Temporal Control

Enzo Olivieri et al.

Summary: The study introduces a fueling method using trichloroacetic acid to create dissipative gelating materials that can switch between different acid/base states. The system is robust and resilient, with the chiral nature of amino acid gelator contributing to chiroptical switching properties.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

Article Multidisciplinary Sciences

Transmembrane transport in inorganic colloidal cell-mimics

Zhe Xu et al.

Summary: The research team has created non-biological capsules that can capture, concentrate, store, and release microscopic payloads as needed. This design uses hollow colloids as cell-membrane mimics with a well-defined single pore, allowing for mass production and offering a blueprint for developing smart materials, micro-machinery, and artificial cell mimics.

NATURE (2021)

Article Chemistry, Multidisciplinary

Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures

Tong Bian et al.

Summary: The use of small molecules with electric charges can effectively induce attractive interactions between oppositely charged nanoparticles in water, guiding their assembly into colloidal crystals. This approach offers a facile way to fabricate, manipulate, and investigate nanostructured materials in aqueous environments.

NATURE CHEMISTRY (2021)

Article Chemistry, Multidisciplinary

Chemically Fueled Block Copolymer Self-Assembly into Transient Nanoreactors**

Michaela A. Wuerbser et al.

Summary: Researchers designed a diblock copolymer that self-assembles into transient micelles when combined with a fuel-driven chemical reaction cycle, allowing for localized increase in hydrophobic reagent concentration and functioning as a transient nanoreactor.

CHEMSYSTEMSCHEM (2021)

Article Chemistry, Multidisciplinary

Accelerated Ripening in Chemically Fueled Emulsions**

Marta Tena-Solsona et al.

Summary: Chemically fueled emulsions are vital solutions with droplets that can self-divide and play important roles in biology. Theoretical studies have shown various intriguing properties, but lack experimental validation. New research reveals that the growth dynamics of droplets in these emulsions are regulated by the kinetics of the fuel-driven reaction cycle.

CHEMSYSTEMSCHEM (2021)

Article Physics, Multidisciplinary

Universality of dissipative self-assembly from quantum dots to human cells

Ghaith Makey et al.

NATURE PHYSICS (2020)

Article Chemistry, Multidisciplinary

Regulating Chemically Fueled Peptide Assemblies by Molecular Design

Kun Dai et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

Article Biochemistry & Molecular Biology

Effects of Protein Unfolding on Aggregation and Gelation in Lysozyme Solutions

Shakiba Nikfarjam et al.

BIOMOLECULES (2020)

Article Chemistry, Multidisciplinary

Redox Chemical-Fueled Dissipative Self-Assembly of Active Materials

William A. Ogden et al.

CHEMSYSTEMSCHEM (2020)

Article Chemistry, Multidisciplinary

Dynamic Vesicles Formed By Dissipative Self-Assembly

Caren Wanzke et al.

CHEMSYSTEMSCHEM (2020)

Review Chemistry, Multidisciplinary

Dissipative Self-Assembly of Peptides

Marta Tena-Solsona et al.

ISRAEL JOURNAL OF CHEMISTRY (2019)

Article Chemistry, Multidisciplinary

Pathway Dependence in the Fuel-Driven Dissipative Self-Assembly of Nanoparticles

Raphael K. Groetsch et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

Article Multidisciplinary Sciences

Programmable dynamic steady states in ATP-driven nonequilibrium DNA systems

Laura Heinen et al.

SCIENCE ADVANCES (2019)

Article Chemistry, Physical

Irreversible Nature of Mesoscopic Aggregates in Lysozyme Solutions

S. Nikfarjam et al.

COLLOID JOURNAL (2019)

Article Chemistry, Physical

On Protein Folding in Crowded Conditions

David Gomez et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

Article Chemistry, Multidisciplinary

Chemically fueled covalent crosslinking of polymer materials

Borui Zhang et al.

CHEMICAL COMMUNICATIONS (2019)

Article Multidisciplinary Sciences

Self-selection of dissipative assemblies driven by primitive chemical reaction networks

Marta Tena-Solsona et al.

NATURE COMMUNICATIONS (2018)

Article Nanoscience & Nanotechnology

Energy consumption in chemical fuel-driven self-assembly

Giulio Ragazzon et al.

NATURE NANOTECHNOLOGY (2018)

Article Materials Science, Biomaterials

Metal Chelation Dynamically Regulates the Mechanical Properties of Engineered Protein Hydrogels

Na Kong et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2017)

Article Materials Science, Biomaterials

Metal Chelation Dynamically Regulates the Mechanical Properties of Engineered Protein Hydrogels

Na Kong et al.

ACS BIOMATERIALS SCIENCE & ENGINEERING (2017)

Article Chemistry, Multidisciplinary

Fuel-Mediated Transient Clustering of Colloidal Building Blocks

Bas G. P. van Ravensteijn et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

Article Chemistry, Multidisciplinary

Adenosine-Phosphate-Fueled, Temporally Programmed Supramolecular Polymers with Multiple Transient States

Shikha Dhiman et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

Article Multidisciplinary Sciences

Non-equilibrium steady states in supramolecular polymerization

Alessandro Sorrenti et al.

NATURE COMMUNICATIONS (2017)

Article Polymer Science

Pulsating Polymer Micelles via ATP-Fueled Dissipative Self-Assembly

Xiang Hao et al.

ACS MACRO LETTERS (2017)

Article Chemistry, Multidisciplinary

4D Biofabrication Using Shape-Morphing Hydrogels

Alina Kirillova et al.

ADVANCED MATERIALS (2017)

Review Chemistry, Multidisciplinary

Non-equilibrium assembly of microtubules: from molecules to autonomous chemical robots

H. Hess et al.

CHEMICAL SOCIETY REVIEWS (2017)

Article Chemistry, Multidisciplinary

Dissipative self-assembly of vesicular nanoreactors

Subhabrata Maiti et al.

NATURE CHEMISTRY (2016)

Article Materials Science, Multidisciplinary

Aqueous Light-Controlled Self-Assembly of Nanoparticles

Dipak Samanta et al.

ADVANCED OPTICAL MATERIALS (2016)

Article Multidisciplinary Sciences

Transient assembly of active materials fueled by a chemical reaction

Job Boekhoven et al.

SCIENCE (2015)

Article Chemistry, Multidisciplinary

Fuel-Controlled Reassembly of Metal-Organic Architectures

Christopher S. Wood et al.

ACS CENTRAL SCIENCE (2015)

Article Chemistry, Multidisciplinary

Generic Concept to Program the Time Domain of Self-Assemblies with a Self-Regulation Mechanism

Thomas Heuser et al.

NANO LETTERS (2015)

Review Physiology

ACTIN DYNAMICS, ARCHITECTURE, AND MECHANICS IN CELL MOTILITY

Laurent Blanchoin et al.

PHYSIOLOGICAL REVIEWS (2014)

Article Multidisciplinary Sciences

Maximum Allowed Solvent Accessibilites of Residues in Proteins

Matthew Z. Tien et al.

PLOS ONE (2013)

Article Multidisciplinary Sciences

Topotactic Interconversion of Nanoparticle Superlattices

Robert J. Macfarlane et al.

SCIENCE (2013)

Article Chemistry, Multidisciplinary

Programmable Shape-Shifting Micelles

Miao-Ping Chien et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2010)

Article Multidisciplinary Sciences

Structural diversity in binary nanoparticle superlattices

EV Shevchenko et al.

NATURE (2006)

Article Biochemistry & Molecular Biology

Unfolding pathways of human serum albumin: Evidence for sequential unfolding and folding of its three domains

MK Santra et al.

INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES (2005)