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Article
Chemistry, Physical
Yangzheng Hou et al.
Summary: This study presents a new structure for zinc-iodine batteries (ZIBs) that addresses the issues of low electron conductivity, shuttle effect, and highly soluble iodine species. By employing a double fixation strategy and specific materials, the ZIBs demonstrate excellent electrochemical performance.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2023)
Article
Chemistry, Physical
Leiqian Zhang et al.
Summary: By constructing a sulfonate-rich ion-exchange layer (SC-PSS) to modulate the transport and reaction of polyiodide and Zn2+, the corrosion and dendritic growth issues on the anode of zinc-iodine batteries can be addressed. The resulting batteries exhibit proper performance over 6000 cycles with high-capacity retention (90.2%) and reversibility (99.89%). The SC-PSS layer blocks polyiodide permeation through electrostatic repulsion and restricts undesirable 2D diffusion of Zn2+ by facilitating desolvation and chemisorption.
ADVANCED ENERGY MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Wei Zhang et al.
Summary: In this study, a multifunctional additive NHP was introduced to regulate zinc deposition and suppress side reactions in aqueous electrolyte. The results showed that the NHP additive enabled highly reversible Zn plating/stripping behaviors, and improved the electrochemical performances of zinc-ion batteries and zinc-based capacitors.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Multidisciplinary
Dan Xie et al.
Summary: A high-quality and ZnF2-riched inorganic/organic hybrid solid electrolyte interface (SEI) layer was constructed on the surface of Zn metal anode (ZMA) by introducing multifunctional fluoroethylene carbonate (FEC) into aqueous electrolyte. The addition of FEC effectively regulated the solvated structure of Zn2+ and hindered the formation of dendrites, thus suppressing dendrites growth and parasitic reactions. The ZMA in FEC-included ZnSO4 electrolyte exhibited a long cycle life and stable coulombic efficiency.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: To stabilize the zinc anode in zinc metal batteries, researchers have developed a controlled electrolytic method using a high dipole moment solvent dimethyl methylphosphonate (DMMP) to create a monolithic solid electrolyte interphase (SEI). This DMMP-based electrolyte generates a homogeneous and robust phosphate SEI (Zn-3(PO4)(2) and ZnP2O6). With the protection provided by this in situ monolithic SEI, the zinc electrode exhibits long-term cycling performance and high Coulombic efficiency in both zinc|zinc and zinc|copper cells. The use of a DMMP-H2O hybrid electrolyte in a full V2O5|zinc battery also results in high capacity retention following a large number of cycles.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Review
Chemistry, Multidisciplinary
Mingnan Li et al.
Summary: Lithium metal batteries (LMBs) have high energy density but face challenges with the instability of the Li metal/electrolyte interface. This review provides a systematic summary of recent progress in electrolytes for high-performance LMBs, including understanding the mechanism, addressing challenges, and analyzing various electrolyte strategies. Suggestions for optimum electrolyte properties and promising research directions are also discussed.
Review
Chemistry, Multidisciplinary
Yanqun Lv et al.
Summary: This review presents the recent development of beyond aqueous electrolytes for Zn-ion batteries, including various types of electrolytes and the critical issues and corresponding strategies for designing beyond aqueous electrolytes.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yongqiang Yang et al.
Summary: A eutectic electrolyte based on N-methylacetamide is proposed for zinc-iodine battery, which improves the performance of the battery by restricting free water and inhibiting the formation of intermediate products. The adoption of activated carbon-coated carbon fiber cloth as an adsorptive cathode enables high capacity retention and coulombic efficiency for the battery.
ENERGY & ENVIRONMENTAL SCIENCE
(2022)
Review
Chemistry, Multidisciplinary
Yanyan Wang et al.
Summary: This review provides an overview of advanced electrolyte strategies for optimizing zinc-ion batteries, including improving the compatibility between cathode materials and electrolytes, inhibiting anode corrosion and dendrite growth, extending electrochemical stability windows, enabling wearable applications, and enhancing temperature tolerance. The underlying scientific mechanisms, electrolyte design principles, and recent progress are presented to enhance understanding and inspiration for readers.
Article
Chemistry, Multidisciplinary
Shao-Jian Zhang et al.
Summary: This study proposes a structure confinement strategy using starch to suppress polyiodide shuttling in Zn-I-2 batteries, resulting in a highly reversible and long-cycling Zn-I-2 battery with high Coulombic efficiency. The starch effectively inhibits Zn corrosion triggered by polyiodide, providing a cheap yet effective strategy for high-cyclability Zn-I-2 batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Song Chen et al.
Summary: The dynamic coordination chemistry of phytic acid with zinc ions can modulate the interfacial redox process of zinc, improving the cycling stability and specific capacity of aqueous zinc batteries.
Article
Chemistry, Multidisciplinary
Xuesong Zhao et al.
Summary: This study presents an effective approach to improve the reversibility and stability of Zn anodes by regulating the pH environment and limiting H2O activity using advanced acidic electrolytes. The results demonstrate that this method can achieve high coulombic efficiency and smooth Zn deposition, as well as ultra-stable cycling of Zn-V2O5 full cell.
Article
Chemistry, Multidisciplinary
Leiqian Zhang et al.
Summary: In this study, a quaternization engineering approach was used to improve the cycling durability of aqueous rechargeable zinc-iodine batteries. By precisely controlling the polyiodide using a commercial acrylic fiber skeleton, a high-rate and ultra-stable polymer-based zinc-iodine battery was developed. The quaternization strategy significantly eliminated the polyiodide shuttle issue and allowed for unique solution-based iodine chemistry in the battery.
Review
Multidisciplinary Sciences
Sailin Liu et al.
Summary: This review examines the failure mechanism of rechargeable zinc metal batteries under temperature influence, presents current electrolyte strategies for improving battery performance in harsh temperatures, and offers perspectives on their industrial application.
Article
Chemistry, Multidisciplinary
Miaomiao Liu et al.
Summary: This study demonstrates the enhancement of physicochemical confinement effect and electrocatalytic redox conversion of iodine in zinc-iodine batteries by embedding a single iron atom in porous carbon with a metal-nitrogen-carbon bridging structure, which is crucial for fabricating high-performing batteries.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Multidisciplinary
Fuhua Yang et al.
Summary: It is demonstrated that H-2 evolution in aqueous zinc-ion batteries primarily originates from solvated water and can be suppressed by additives, leading to improved cycle stability and electrochemical performance.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Zhijie Wang et al.
Summary: There is always a trade-off between non-flammability and battery performance in traditional non-flammable electrolytes. Previous research has overlooked the contribution of solvated anions in boosting electrolyte stability. By introducing anions with similar donor numbers, the stability of electrolyte against Li can be improved.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Physical
Haiji Huang et al.
Summary: This study reports a method to control the electrolyte structure and interface in aqueous zinc-ion batteries (AZIBs) by adding trace amounts of the organic compound GBL. The addition of GBL weakens the bonding strength between zinc ions and solvated water, reducing water activity and suppressing corrosion and side products. This method improves the stability and cycling life of the zinc anode significantly, and maintains stability and high capacity under harsh testing conditions.
ADVANCED ENERGY MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Jianfeng Mao et al.
Summary: This article reviews the advances and advantages of automotive LIB recycling, as well as the evaluation of new cycling-oriented designs. The research shows that practical battery recycling can address environmental pollution and resource waste, while promoting sustainability.
ENERGY & ENVIRONMENTAL SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Junnan Hao et al.
Summary: A similar antisolvent strategy has been used to enhance Zn reversibility and suppress dendrite growth in Zn plating/stripping, with promising results shown in 50% methanol electrolyte. This low-cost strategy can be easily applied to other solvents, demonstrating practical universality and potential for enhancing performance in electrochemistry and energy storage research.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Multidisciplinary Sciences
Zedong Zhao et al.
Summary: This study developed a fluorinated covalent organic framework film as a protective layer for aqueous zinc anode battery, aiming to reduce zinc dendrite growth and electrolyte corrosion, achieve horizontally arranged zinc deposition, and improve stability and cycling performance.
NATURE COMMUNICATIONS
(2021)
Article
Nanoscience & Nanotechnology
Jianghe Liu et al.
Summary: The gel electrolyte based on the PVA/Zn/ethylene glycol system shows high ionic conductivity and excellent antifreezing performance. The antifreezing Zn-ion hybrid supercapacitor fabricated with this gel electrolyte exhibits outstanding electrochemical properties and cyclic stability, even under low temperatures, demonstrating its potential for flexible energy storage devices in subzero-temperature environments.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: By tuning the solvation structure of the electrolyte and using fire-retardant triethyl phosphate as a cosolvent, the challenges of cathode dissolution, water reactivity, and zinc dendrites in aqueous zinc-ion batteries have been successfully addressed. The optimized electrolyte structure leads to high average Coulombic efficiency in Zn/Cu cells and enables over 1000 cycles at high current density.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Peng Sun et al.
Summary: The addition of glucose in ZnSO4 electrolyte can improve the performance of Zn ion batteries by suppressing Zn dendrite growth and side reactions, enhancing stability.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Physical
Mengdie Yan et al.
Summary: This study demonstrates the improvement of zinc anodes in low-cost aqueous electrolytes by adding polymers of different polarities, resulting in over 1300 hours of operation time and high Coulombic efficiency under 2 mA/cm², 2 mAh/cm² conditions.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Xiaohui Zeng et al.
Summary: Inspired by the bio-adhesion principle, a stable SEI layer of polydopamine was successfully constructed on a Zn anode, offering multifunctional features that regulate Zn nucleation, enhance Zn-ion conductivity, and block interfacial side reactions. This approach significantly improved the performance and stability of rechargeable aqueous zinc-ion batteries.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Review
Chemistry, Multidisciplinary
Shilin Zhang et al.
Summary: The search for alternatives to traditional Li-ion batteries has led to the development of rechargeable liquid metal batteries, which operate at room or intermediate temperatures to address challenges related to high temperature operation, corrosive reactions, and hermetic sealing. These new paradigms aim to overcome drawbacks of conventional liquid metal batteries and enable both conventional and new functionalities by applying alternative electrodes, manipulating electrolyte design concepts, and engineering electrode-electrolyte interfaces.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Canbin Deng et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Chemistry, Physical
Xiaohui Zeng et al.
ADVANCED ENERGY MATERIALS
(2020)
Article
Chemistry, Inorganic & Nuclear
Mostafa Mohsen et al.
JOURNAL OF SOLID STATE CHEMISTRY
(2020)
Article
Chemistry, Multidisciplinary
Longsheng Cao et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2020)
Article
Chemistry, Multidisciplinary
Lu Zhang et al.
ADVANCED FUNCTIONAL MATERIALS
(2019)
Article
Chemistry, Multidisciplinary
Funian Mo et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2019)
Article
Chemistry, Multidisciplinary
Zhiming Zhao et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2019)
Article
Chemistry, Physical
Fei Wang et al.
Article
Chemistry, Multidisciplinary
Chong Zhang et al.
CHEMICAL COMMUNICATIONS
(2018)
Article
Multidisciplinary Sciences
Bin Li et al.
NATURE COMMUNICATIONS
(2015)
Article
Materials Science, Multidisciplinary
T. Rajkumar et al.
MATERIALS CHEMISTRY AND PHYSICS
(2008)
Article
Chemistry, Physical
MI Zaki et al.
COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS
(2001)
