期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 138, 期 3, 页码 810-813出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b13104
关键词
-
资金
- National Natural Science Foundation of China [21222207, 21572231]
A highly enantioselective hydrosilylation of 1,2-dicarbonyl compounds was successfully realized for the first time utilizing the combination of tricyclohexylphosphine and chiral alkenylborane derived in situ from diyne as a frustrated Lewis pair catalyst. A variety of optically active a-hydroxy ketones and esters were obtained in 52-98% yields with 86-99% ees.
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