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Covalent Organic Frameworks for Extracting Water from Air

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Chemistry, Multidisciplinary

Hierarchical Microtubular Covalent Organic Frameworks Achieved by COF-to-COF Transformation

Zhenjie Mu et al.

Summary: The pore environment and aggregated structure of porous materials are crucial for their properties, especially mass transfer. In this study, a COF-to-COF transformation method was used to prepare microtubular COFs. This transformation was achieved by decomposing C-3-symmetric guanidine units into C-2-symmetric hydrazine units, resulting in crystal transformation of COFs. The hierarchical structure obtained with varying reaction times led to enhanced mass transfer properties, as demonstrated by adsorption measurement and chemical catalytic reactions. This self-template strategy was also successfully applied to four other COFs with different building units.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Chemistry, Multidisciplinary

2D Covalent Organic Framework for Water Harvesting with Fast Kinetics and Low Regeneration Temperature

Chao Sun et al.

Summary: This study demonstrates that 2D covalent organic frameworks (COFs) with hydrophobic skeletons, proper hydrophilic site density, and 1D open channels can significantly lower the water diffusion and desorption energy barrier, thereby improving the efficiency of atmospheric water harvesting.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Review Chemistry, Multidisciplinary

Covalent Organic Framework Based Functional Materials: Important Catalysts for Efficient CO2 Utilization

Meng Lu et al.

Summary: The photo-/electrocatalytic reduction of CO2 and utilization of CO2 as a supporter for energy storage have shown great potential, but face obstacles such as inefficient uptake/activation of CO2 and mass transport in catalysts. Covalent organic frameworks (COFs) have been explored as catalysts for CO2 conversion due to their unique features.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Engineering, Chemical

Assemblable Carbon Fiber/Metal-Organic Framework Monoliths for Energy-Efficient Atmospheric Water Harvesting

Qiangqiang Li et al.

Summary: Atmospheric water harvesting using metal-organic frameworks (MOFs) is an attractive method for alleviating water shortage stress in arid regions. Researchers have developed a cylindrical structure by embedding commercial carbon fibers into MOF monoliths, resulting in improved heating efficiency for efficient water sorption and release.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2022)

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Review Chemistry, Multidisciplinary

Sorbents for Atmospheric Water Harvesting: From Design Principles to Applications

Wen Shi et al.

Summary: This article reviews recent progress in AWH sorbent design and study, covering innovative chemistries, integration of sophisticated architectures and functional components, and clarifies the structure-property-performance relationship. Summaries of different sorbents' features and limitations, discussions on applications, and future developments are provided.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Landscaping Covalent Organic Framework Nanomorphologies

Himadri Sekhar Sasmal et al.

Summary: This article reviews the synthetic strategies for controlling the nanomorphologies of covalent organic frameworks (COFs) and examines the impact of dimensionalities on their physicochemical properties and applications. The aim is to improve the performance of COFs in various fields by optimizing their morphological dimensions.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Multidisciplinary

Hydrazine-Hydrazide-Linked Covalent Organic Frameworks for Water Harvesting

Ha L. Nguyen et al.

Summary: We report a postsynthetic strategy and its implementation to make covalent organic frameworks with irreversible hydrazide linkages. The synthesis of three 2D and 3D hydrazine-linked frameworks and their partial oxidation were performed. The water uptake profiles of these frameworks were studied, leading to the discovery of one hydrazine-hydrazide linked COF suitable for water harvesting from air in arid conditions.

ACS CENTRAL SCIENCE (2022)

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Editorial Material Chemistry, Multidisciplinary

Postfunctionalized Covalent Organic Frameworks for Water Harvesting

Patrick W. Fritz et al.

ACS CENTRAL SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Crystalline Porous Organic Salt for Ultrarapid Adsorption/Desorption-Based Atmospheric Water Harvesting by Dual Hydrogen Bond System

Shuai Zhang et al.

Summary: In this study, a new crystalline porous organic salt material (CPOS-6) possessing a dual hydrogen bond system was synthesized and its applicability in atmospheric water harvesting (AWH) was verified for the first time. Unlike other reported CPOSs, CPOS-6 exhibits an S-shaped water sorption isotherm due to the presence of the dual hydrogen bond system. Under simulated drought conditions in Xinjiang Uygur Autonomous Region, CPOS-6 demonstrates long-term water adsorption-desorption cycling stability, low water desorption temperature, and ultrarapid adsorption-desorption kinetics. The results confirm that CPOS-6 is an effective sorbent material for AWH.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

A Highly Stable Ortho-Ketoenamine Covalent Organic Framework with Balanced Hydrophilic and Hydrophobic Sites for Atmospheric Water Harvesting

Liang-Hui Chen et al.

Summary: Atmospheric moisture can solve the shortage of fresh water in arid areas as a sustainable clean water source. A COF-ok material was reported as a promising porous sorbent for solar-driven atmospheric water harvesting, showing high water uptake, stability, and regeneration performance under low humidity conditions in a lab-scale system.

CHEMSUSCHEM (2022)

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Article Multidisciplinary Sciences

Covalent organic framework-based porous ionomers for high-performance fuel cells

Qingnuan Zhang et al.

Summary: By optimizing the three-phase microenvironment of the ion exchange proton membrane and incorporating ionic covalent organic framework, the platinum loading in fuel cells can be reduced without sacrificing mass activity and peak power density.

SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Materials and devices for atmospheric water harvesting

Yongtao Meng et al.

Summary: This article discusses the potential of atmospheric water harvesting (AWH) as a promising approach to address global water scarcity. It focuses on the suitability of sorption materials and related devices for arid regions and examines the current developments in porous adsorbents, such as silica, zeolites, metal-organic frameworks (MOFs), aerogel, and manganese oxides. It also discusses the field testing performance of AWH devices utilizing MOFs to trap and release water under solar irradiation in arid climates. The article concludes with an outlook for improving the efficiency of adsorbents and devices and explores new opportunities in the field.

CELL REPORTS PHYSICAL SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Sustainable water generation: grand challenges in continuous atmospheric water harvesting

Primoz Poredos et al.

Summary: Sorption and radiative sky cooling technologies have the potential to provide decentralized fresh water, but continuous operational devices are needed. Current energy materials and system designs have limitations that hinder continuous AWH. By addressing these challenges, 24-hour continuous fresh water generation can be achieved.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Article Chemistry, Physical

Dual-Stage Atmospheric Water Harvesting Device for Scalable Solar-Driven Water Production

Alina LaPotin et al.

Summary: Recent research has shown that a dual-stage AWH device with optimized design can achieve higher daily water productivity by recovering the latent heat of condensation and maintaining the required temperature difference between stages, without the need for additional heating units. Outdoor experiments demonstrated the effectiveness of the dual-stage water harvesting device.

JOULE (2021)

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Review Engineering, Environmental

A Roadmap to Sorption-Based Atmospheric Water Harvesting: From Molecular Sorption Mechanism to Sorbent Design and System Optimization

Kaijie Yang et al.

Summary: This review summarizes the latest progress in sorption-based atmospheric water harvesting (SAWH) technology, focusing on sorbent material design and system optimization. The article introduces water sorption mechanisms on different sorbent materials, discusses the properties and performances of various sorbents, and analyzes the influences of mass and heat transport on system performance.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Construction of Interlayer Conjugated Links in 2D Covalent Organic Frameworks via Topological Polymerization

Yuhao Zhu et al.

Summary: A new interlayer topological polymerization strategy was proposed to transform diacetylene columnar arrays in 2D COFs into conjugated enyne chains upon heating in the solid state, leading to enhanced conductivity and improved photothermal, photoacoustic, and oxygen reduction catalytic performance of the resulting COFs.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Review Chemistry, Physical

Adsorption-based atmospheric water harvesting

M. Ejeian et al.

Summary: Atmospheric water harvesting (AWH) and adsorption-based atmospheric water harvesting (ABAWH) are promising solutions to the world's water shortage, with ABAWH showing higher water supply ability in arid areas. Many modern adsorbents have been introduced for this application, but there are still challenges to address for widespread and practical use of this technology.

JOULE (2021)

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Article Chemistry, Physical

Marriage of 2D Covalent-Organic Framework and 3D Network as Stable Solar-Thermal Still for Efficient Solar Steam Generation

Zhongming Huang et al.

Summary: In this study, a diketopyrrolopyrrole-based 2D COF with broadband optical absorption and a 3D hierarchical COFHS structure were developed to achieve high solar-thermal conversion efficiency. These structures enable a high solar-to-vapor energy conversion efficiency of 93.2% and a stable water evaporation rate of 2.5 kg m(-2) h(-1), showing promise for solar-thermal water production.

SMALL METHODS (2021)

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Article Chemistry, Physical

Hydrophilicity gradient in covalent organic frameworks for membrane distillation

Shuang Zhao et al.

Summary: The study proposes a strategy to modify covalent organic framework membranes by engineering defects to create vertically aligned channels with a hydrophilicity gradient, allowing for high flux membrane distillation membranes. This method offers advantages in increasing membrane permeance and anti-fouling and anti-wetting properties.

NATURE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Embedding metal foam into metal-organic framework monoliths for triggering a highly efficient release of adsorbed atmospheric water by localized eddy current heating

Yingle Tao et al.

Summary: Utilizing metal foam (MF) embedded MOF monoliths (MF@MOFs) can overcome the thermal insulating nature of MOF monoliths and realize rapid and uniform heating through the use of localized eddy current heating (LECH), leading to significantly improved desorption kinetics for water harvesting from the atmosphere.

MATERIALS HORIZONS (2021)

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Article Chemistry, Multidisciplinary

A Porous Covalent Organic Framework with Voided Square Grid Topology for Atmospheric Water Harvesting

Ha L. Nguyen et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Multidisciplinary Sciences

Laminated self-standing covalent organic framework membrane with uniformly distributed subnanopores for ionic and molecular sieving

Yang Li et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Multidisciplinary

Water and Metal-Organic Frameworks: From Interaction toward Utilization

Xinlei Liu et al.

CHEMICAL REVIEWS (2020)

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Review Energy & Fuels

A review of metal-organic frameworks (MOFs) as energy-efficient desiccants for adsorption driven heat-transformation applications

Avishek Karmakar et al.

APPLIED ENERGY (2020)

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Review Chemistry, Multidisciplinary

Crystallinity and stability of covalent organic frameworks

Xin Huang et al.

SCIENCE CHINA-CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Confined growth of ordered organic frameworks at an interface

Yinghua Jin et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Review Materials Science, Multidisciplinary

Atmospheric Water Harvesting: A Review of Material and Structural Designs

Xingyi Zhou et al.

ACS MATERIALS LETTERS (2020)

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Review Chemistry, Multidisciplinary

Design and applications of three dimensional covalent organic frameworks

Xinyu Guan et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Bulk COFs and COF nanosheets for electrochemical energy storage and conversion

Jie Li et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Designed Synthesis of a 2D Porphyrin-Based sp2 Carbon-Conjugated Covalent Organic Framework for Heterogeneous Photocatalysis

Rufan Chen et al.

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Advances in Porous Organic Polymers for Efficient Water Capture

Yearin Byun et al.

CHEMISTRY-A EUROPEAN JOURNAL (2019)

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Rapid Cycling and Exceptional Yield in a Metal-Organic Framework Water Harvester

Nikita Hanikel et al.

ACS CENTRAL SCIENCE (2019)

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Covalent Organic Frameworks: Chemistry beyond the Structure

Sharath Kandambeth et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Nanoscience & Nanotechnology

Fabrication of Hydrazone-Linked Covalent Organic Frameworks Using Alkyl Amine as Building Block for High Adsorption Capacity of Metal Ions

Ya Li et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Chemistry, Multidisciplinary

Improved synthesis of β-ketoenamine-linked covalent organic frameworks via monomer exchange reactions

Michael C. Daugherty et al.

CHEMICAL COMMUNICATIONS (2019)

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A Moisture-Penetrating Humidity Pump Directly Powered by One-Sun Illumination

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Ultrastable Imine-Based Covalent Organic Frameworks for Sulfuric Acid Recovery: An Effect of Interlayer Hydrogen Bonding

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Chiral 3D Covalent Organic Frameworks for High Performance Liquid Chromatographic Enantioseparation

Xing Hang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Single-crystal x-ray diffraction structures of covalent organic frameworks

Tianqiong Ma et al.

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Assemblies of covalent organic framework microcrystals: multiple-dimensional manipulation for enhanced applications

Fuyu Yuan et al.

SCIENCE CHINA-CHEMISTRY (2018)

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Adsorption-based atmospheric water harvesting device for arid climates

Hyunho Kim et al.

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Reticular Chemistry in Action: A Hydrolytically Stable MOF Capturing Twice Its Weight in Adsorbed Water

Sk Md Towsif Abtab et al.

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Practical water production from desert air

Farhad Fathieh et al.

SCIENCE ADVANCES (2018)

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Crystalline Dioxin-Linked Covalent Organic Frameworks from Irreversible Reactions

Bing Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Understanding Water Adsorption and the Impact on CO2 Capture in Chemically Stable Covalent Organic Frameworks

Yuxin Ge et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2018)

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Progress and Expectation of Atmospheric Water Harvesting

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Hydrolytic Stability of Boronate Ester-Linked Covalent Organic Frameworks

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Stable Covalent Organic Frameworks for Exceptional Mercury Removal from Aqueous Solutions

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Solution Synthesis of Semiconducting Two-Dimensional Polymer via Trimerization of Carbonitrile

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Record Atmospheric Fresh Water Capture and Heat Transfer with a Material Operating at the Water Uptake Reversibility Limit

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Three-Dimensional Anionic Cyclodextrin-Based Covalent Organic Frameworks

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Covalent Triazine Frameworks via a Low-Temperature Polycondensation Approach

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Applications of covalent organic frameworks (COFs): From gas storage and separation to drug delivery

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Chemical Conversion of Linkages in Covalent Organic Frameworks

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Tunable Water and CO2 Sorption Properties in Isostructural Azine-Based Covalent Organic Frameworks through Polarity Engineering

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Nitrogen-Rich Covalent Triazine Frameworks as High-Performance Platforms for Selective Carbon Capture and Storage

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Pore surface engineering in porous, chemically stable covalent organic frameworks for water adsorption

Bishnu P. Biswal et al.

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Water Stability and Adsorption in Metal-Organic Frameworks

Nicholas C. Burtch et al.

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Designed synthesis of large-pore crystalline polyimide covalent organic frameworks

Qianrong Fang et al.

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Arjen Y. Hoekstra

NATURE CLIMATE CHANGE (2014)

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Enhancement of Chemical Stability and Crystallinity in Porphyrin-Containing Covalent Organic Frameworks by Intramolecular Hydrogen Bonds

Sharath Kandambeth et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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Covalent organic frameworks (COFs): from design to applications

San-Yuan Ding et al.

CHEMICAL SOCIETY REVIEWS (2013)

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An Azine-Linked Covalent Organic Framework

Sasanka Dalapati et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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The Chemistry and Applications of Metal-Organic Frameworks

Hiroyasu Furukawa et al.

SCIENCE (2013)

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A Crystalline Imine-Linked 3-D Porous Covalent Organic Framework

Fernando J. Uribe-Romo et al.

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Covalent organic frameworks as exceptional hydrogen storage materials

Sang Soo Han et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2008)

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Optimizing the reversibility of hydrazone formation for dynamic combinatorial chemistry

R Nguyen et al.

CHEMICAL COMMUNICATIONS (2003)

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