期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 138, 期 18, 页码 5825-5828出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b03112
关键词
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资金
- NFSC [21403062, 21373080]
- HNNSF [2015JJ3039]
- Fundamental Research Funds for the Central Universities (Hunan University)
A Pd-catalyzed dehydrogenative phosphorylation of thiols is developed. A variety of thiols dehydrogenatively couple readily with all three kinds of P(O)-H compounds, i.e., H-phosphonates, H-phosphimates, and secondary phosphine oxides, providing a general access to the valuable phosphorothioates including the P-chiral compounds. A plausible mechanism is proposed.
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