期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 138, 期 33, 页码 10378-10381出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.6b03972
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A new series of bifunctional Ru complexes with pendent Lewis acidic boranes were prepared by late stage modification of an active hydrogen-transfer catalyst. The appended boranes modulate the reactivity of a metal hydride as well as catalytic hydrogenations. After installing acidic auxiliary groups, the complexes become multifunctional and catalyze the cis-selective hydrogenation of alkynes with higher rates, conversions, and selectivities compared with the unmodified catalyst.
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