☆ 4.8 Review

Circularly Polarized Light Responsive Materials: Design Strategies and Applications

ADVANCED MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Multispectral and Circular Polarization-Sensitive Carbon Dot-Polydiacetylene Capacitive Photodetector

Nitzan Shauloff et al.

Summary: Multispectral photodetectors (MSPs) and circularly polarized light (CPL) sensors play important roles in opto-electronics, photonics, and imaging. A capacitive photodetector composed of an interdigitated electrode coated with carbon dot/anthraquinone-polydiacetylene provides wavelength selectivity based on the absorbance of carbon dots. Polymerized-anthraquinone photodetector films incorporating carbon dots of different excitation wavelengths produce optical capacitive fingerprints within a broad spectral range. Circular light polarization selectivity is achieved through chiral polymerization of the polydiacetylene framework. This platform exhibits rapid photo-response, high fidelity, and recyclability, while being cost-effective and environmentally friendly.

SMALL (2023)

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Review Materials Science, Multidisciplinary

Advances in circularly polarized luminescence materials based on helical polymers

Shi-Yi Li et al.

Summary: Helical polymers are widely used in various fields due to their unique structure and optical activity. In recent years, they have become a new favorite in the field of circularly polarized luminescence (CPL) materials. This review introduces CPL materials and discusses the advantages and classification of CPL materials based on helical polymers. The research progress of CPL materials of helical polymers is summarized, aiming to stimulate interest and promote further development.

JOURNAL OF MATERIALS CHEMISTRY C (2023)

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Review Chemistry, Multidisciplinary

The Interaction of 2D Materials With Circularly Polarized Light

Rong Rong et al.

Summary: Due to spin-valley locking degree of freedom, 2D materials exhibit strongly bound exciton and chiral optical selection rules, making them promising for optoelectronic and spin/valleytronic devices. The interaction of circularly polarized light with 2D materials has led to fascinating phenomena and is reviewed in this paper, covering various materials such as graphene, black phosphorous, transition metal dichalcogenides, and van der Waals heterostructures. The challenges and opportunities for theoretical and experimental advancements are also discussed.

ADVANCED SCIENCE (2023)

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Article Chemistry, Multidisciplinary

Visible Helicity Induction and Memory in Polyallene toward Circularly Polarized Luminescence, Helicity Discrimination, and Enantiomer Separation

Lei Xu et al.

Summary: Inspired by natural helices like DNA, the researchers successfully induced one-handed helical structures in achiral polymers using chiral amines and alcohols, and the induced helices were able to maintain their structure even after the chiral inducer was removed. These induced helices formed stable gels and showed helicity discrimination ability. They also demonstrated efficient enantioselective crystallization and separation of enantiomers. This research has significant implications for developing novel chiral materials.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Review Chemistry, Multidisciplinary

Recent Advances in Ultrathin Chiral Metasurfaces by Twisted Stacking

Zexiang Han et al.

Summary: Artificial chiral nanostructures have been extensively studied for their unique chiroptical activities. Controlled twisted stacking of nanomaterials has emerged as a general strategy to introduce optical chirality into achiral solid-state systems. Recent progress in planar chiral metasurfaces is summarized, discussing the building blocks, fabrication methods, as well as circular dichroism and its modulation in twisted stacked nanostructures. The review highlights the growing applications of these chiral metasurfaces, including polarization conversion, information encryption, chiral sensing, and as an engineering platform for hybrid metadevices. Future prospects are also provided.

ADVANCED MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Twisting of Porphyrin by Assembly in a Metal-Organic Framework yielding Chiral Photoconducting Films for Circularly-Polarized-Light Detection

Chun Li et al.

Summary: Researchers have successfully prepared a crystalline film based on porphyrin with chiral properties and demonstrated excellent optoelectronic performance. By assembling in a metal-organic framework film, the porphyrin core becomes twisted and chiral. The close packing and crystalline order of the porphyrin cores in the film result in outstanding optoelectronic properties. Through exciting the Soret band of porphyrin, efficient photoconduction with a high On-Off ratio is achieved. Moreover, handedness-dependent circularly-polarized-light photoconduction is obtained. The combination of assembly-induced chirality with the rich porphyrin chemistry opens up possibilities for organic materials with exceptional chiral and optoelectronic properties.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Chemistry, Multidisciplinary

Absolute asymmetric synthesis driven by circularly polarized Light

Chenlu He et al.

Summary: This article reviews the historical research on circularly polarized light (CPL)-induced absolute asymmetric synthesis, including chiral organic molecules, helical polymers, supramolecular assemblies, and noble metal nanostructures. However, based on these results, it is concluded that the chiral photon-matter interaction is very weak, resulting in a very small enantiomeric excess for the product. Therefore, the recently emerged superchiral field technology, which can enhance the dissymmetry of the optical field and near-field, is highlighted.

CHINESE CHEMICAL LETTERS (2023)

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Article Chemistry, Multidisciplinary

Charge-Transfer Complex Doped Photothermal Hydrogels for Discriminating Circularly Polarized Near-Infrared Light

Zhuoer Wang et al.

Summary: This study reports a general method to build hydrogels from pi-conjugated amino acids with charge-transfer complexes, allowing for tunable response to circularly polarized light. The hybrid hydrogels showed adjustable photothermal performance and tunable Cotton effects from visible light to NIR-I region.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2023)

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Article Nanoscience & Nanotechnology

Selectively Regulating the Chiral Morphology of Amino Acid-Assisted Chiral Gold Nanoparticles with Circularly Polarized Light

Hongdan Wang et al.

Summary: This study proposes a method for site-selective chirality regulation through circularly polarized light, which can control the morphology evolution of cysteine-assisted chiral gold nanoparticles and result in increased or decreased circular dichroism signal intensity. It provides a promising alternative strategy for producing high-chirality nanomaterials that can be applied in biomedicine and enantiomer photocatalytic reactions.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Photo-Imprinting of the Helical Organization in Liquid-Crystal Networks Using Achiral Monomers and Circularly Polarized Light

Hirotoshi Sakaino et al.

Summary: Control over molecular motion is achieved by fabricating cholesteric liquid-crystal networks using circularly polarized light, without the need for chiral dopant or plasticizer. The resulting materials exhibit excellent thermal stability, reversible light-induced memory features, and the ability to fabricate photo-patterned films of liquid-crystal networks with opposite helical senses.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Physical

Self-Assembled Helical Structures of Pyrene-Conjugated Amino Acids for Near-Infrared Chiroptical Materials and Chiral Photothermal Agents

Zhuoer Wang et al.

Summary: The researchers successfully realized chiroptical properties in the near-infrared (NIR) region using a charge-transfer strategy and applied it to photothermal agents. They self-assembled pyrene-conjugated amino acid derivatives into helical structures with supramolecular tilt chirality. By manipulating the amino acid domains, they achieved chiroptical activity evolution in the NIR region and controlled the photothermal performance using circularly polarized NIR light.

CHEMISTRY OF MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Circularly Polarized Light Can Override and Amplify Asymmetry in Supramolecular Helices

Jun Su Kang et al.

Summary: The study shows that circularly polarized light can induce chirality at the supramolecular level, and the chirality information can be nonlinearly amplified in the system. Opposite chirality can override molecular information when the enantiomeric excess is low.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Materials Science, Multidisciplinary

Lead-Free Chiral 2D Double Perovskite Microwire Arrays for Circularly Polarized Light Detection

Yingjie Zhao et al.

Summary: This study fabricated lead-free chiral 2D double perovskite single-crystalline microwire arrays with excellent environmental stability, realizing outstanding circularly polarized light photodetectors with high responsivity and detectivity.

ADVANCED OPTICAL MATERIALS (2022)

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Article Materials Science, Multidisciplinary

Flexible, Programmable, Chiroptical Polymer Films of Twisted Stacking Layers for Circular Polarization-Based Multiplex Color Display

Yifan Xie et al.

Summary: Flexible films with strong and tunable chiroptical responses are in high demand for various applications. This research presents a simple and cost-effective method to fabricate flexible chiroptical polymeric films with giant optical activity, by aligning two anisotropic polydiacetylene layers in a twisted fashion. The films demonstrate a full color, high brightness, fast responsive, multiplex laser display based on circular polarization, and show potential for applications in circular polarized luminescence and optical encryption.

ADVANCED OPTICAL MATERIALS (2022)

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Review Materials Science, Multidisciplinary

Emerging materials for circularly polarized light detection

Xiaobo Shang et al.

Summary: Detecting circularly polarized light (CPL) signals is crucial in advanced sensing technologies, with CPL detectors of different wavelengths having distinct applications. This review introduces the working principle and material design strategies of state-of-the-art CPL photodetectors, as well as recent developments in chiral materials for CPL detection and strategies for improving detection capabilities.

JOURNAL OF MATERIALS CHEMISTRY C (2022)

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Article Chemistry, Multidisciplinary

Ultrasensitive Near-Infrared Circularly Polarized Light Detection Using 3D Perovskite Embedded with Chiral Plasmonic Nanoparticles

Hongki Kim et al.

Summary: Chiral organic ligand-incorporated low-dimensional metal-halide perovskites with chiral plasmonic gold nanoparticles demonstrate remarkable chirality in the near-infrared region and high sensitivity for self-powered NIR detection.

ADVANCED SCIENCE (2022)

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Review Chemistry, Multidisciplinary

Self-assembled inorganic chiral superstructures

Jiawei Lv et al.

Summary: Controlled assembly of inorganic nanoparticles into higher-order structures with collective functionalities, particularly chiral superstructures, has attracted significant attention due to their unique chiroptical properties and potential applications. Various strategies have been developed to prepare self-assembled inorganic chiral superstructures based on the preference of building blocks and external factors. Compared to organic counterparts, these inorganic chiral superstructures exhibit superior optical activity.

NATURE REVIEWS CHEMISTRY (2022)

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Article Nanoscience & Nanotechnology

Cellulose Nanocrystal/TiO2 Nanotube Composites for Circularly Polarized Light Detection

Yingying Yu et al.

Summary: Circularly polarized light (CPL) detection is important in advanced optoelectronics, and traditional methods using optical elements have limitations due to integration challenges. This study explores a composite structure of chiral cellulose nanocrystals (CNCs) and TiO2 nanotube arrays (TNAs) for CPL detection, achieving effective distinguishability with a high anisotropy factor (g(ph)) of 0.33. The CNC-TNA photoelectrodes show fast response time, good cycling stability, and the ability to track the phase difference of elliptically polarized light, offering a potential approach for CPL detection.

ACS APPLIED NANO MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Controlled Synthesis of Cyclic-Helical Polymers with Circularly Polarized Luminescence

Lei Xu et al.

Summary: Cyclic polymers prepared via ring-expansion polymerization with chiral Pd-II catalysts exhibit predictable molecular weight and low dispersity, and can be used for the synthesis of cyclic bottlebrush polymers with a chiral helical backbone, showing interesting optical properties.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Nanoscience & Nanotechnology

Polarization-sensitive optoionic membranes from chiral plasmonic nanoparticles

Jiarong Cai et al.

Summary: In this study, chiral gold nanoparticles were assembled into nanoporous membranes to achieve high sensitivity to circular polarization through light-induced polarization-dependent ion accumulation. By using suitable modification, a photocurrent as high as 2.41 times higher can be obtained under right-handed circularly polarized light. This technology holds great potential for applications in chiral photonics.

NATURE NANOTECHNOLOGY (2022)

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Article Nanoscience & Nanotechnology

Direct Detection of Near-Infrared Circularly Polarized Light via Precisely Designed Chiral Perovskite Heterostructures

Xinyuan Zhang et al.

Summary: In this study, a novel chiral metal halide perovskite (CMHP) heterostructure was designed, which achieved self-powered direct near-infrared circularly polarized light detection by synthesizing crystalline 3D MAPbI(3) on a 2D chiral (R-BPEA)(2)PbI4 crystal. Compared with individual chiral (R-BPEA)2PbI4, the heterostructure not only retained spin selectivity but also had a broader absorbance range. By utilizing the built-in electric potential in the heterojunction, devices operating without external energy supply were realized.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Optically Programmable Circularly Polarized Photodetector

Can Zhang et al.

Summary: A fundamentally novel approach in designing a programmable circularly polarized light photodetector utilizing the chiral properties of achiral polymers and high-quality film was demonstrated, achieving switchable detection of left- and right-handed CPL signals. This device also exhibited excellent discrimination between different CPL signals, making it a promising tool in various scientific fields and imaging applications.

ACS NANO (2022)

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Article Chemistry, Multidisciplinary

Robust Spin-Dependent Anisotropy of Circularly Polarized Light Detection from Achiral Layered Hybrid Perovskite Ferroelectric Crystals

Xiaoqi Li et al.

Summary: For the first time, this study demonstrates the robust angular anisotropy of circularly polarized light (CPL) detection in a new layered hybrid perovskite ferroelectric crystal. This crystal, which crystallizes in an optically active achiral polar point group, exhibits remarkable bulk photovoltaic effect (BPVE) and highly sensitive self-powered CPL detection performance.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Multidisciplinary

Chiral Non-Fullerene Acceptor Enriched Bulk Heterojunctions Enable High-Performance Near-Infrared Circularly Polarized Light Detection

Lixuan Liu et al.

Summary: This study presents the successful development of high-performing direct near-infrared circularly polarized light photodetectors with high dissymmetry factor, responsivity, detectivity, and response speed. Introducing supramolecular chirality achieved an optimal balance between optoelectronic performance and chiroptical properties, enabling the photodetector to exhibit excellent performance in the NIR region.

SMALL (2022)

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Article Multidisciplinary Sciences

Organic donor-acceptor heterojunctions for high performance circularly polarized light detection

Danlei Zhu et al.

Summary: In this paper, the authors propose a strategy to fabricate multi-wavelength circularly polarized light photodetectors using bilayer donor-acceptor heterojunctions with chiral active layers. The resulting photodetectors exhibit excellent stability and high responsivity, making them promising for large-scale circularly polarized light integrated photonic applications.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Multidisciplinary

Chiral Rashba Ferroelectrics for Circularly Polarized Light Detection

Chang-Chun Fan et al.

Summary: A pair of 2D chiral perovskite ferroelectrics with enhanced CPL detection performance have been reported in this study, achieved through the chirality-transfer-induced chiral&polar ferroelectric phase.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Spin-Selective Charge Transport in Lead-Free Chiral Perovskites: The Key towards High-Anisotropy in Circularly-Polarized Light Detection

Abhishek Maiti et al.

Summary: A pair of zero-dimensional lead-free chiral perovskites is introduced for the detection of circularly polarized light (CPL). Due to the intrinsic chirality, these perovskites exhibit chirality-induced spin-selectivity, making them suitable for CPL detection. Although the self-powered CPL detector shows a limited anisotropy factor, the factor increases under bias.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Multidisciplinary Sciences

Circularly polarized light-sensitive, hot electron transistor with chiral plasmonic nanoparticles

Seok Daniel Namgung et al.

Summary: This study demonstrates a highly efficient CPL-detecting transistor using chiral plasmonic nanoparticles and a conducting oxide. The transistor successfully distinguishes circular polarization state and exhibits high photoresponsivity. This research contributes to the rational design and fabrication of high-performance CPL detectors and opto-neuromorphic operations.

NATURE COMMUNICATIONS (2022)

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Article Materials Science, Multidisciplinary

Controlling the Helicity Direction of Nanoribbons by Circularly Polarized Light

Hongdan Wang et al.

Summary: Using a new supramolecular organogel, helical nanoribbons with high helicity degree can be generated by irradiating with right- or left-circularly polarized light. The helical direction of the nanoribbons can be controlled by the direction of the circularly polarized light. This concept has potential applications in biology, pharmacology, and chiral optics.

ACS MATERIALS LETTERS (2022)

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Article Engineering, Biomedical

Stimulation of neural stem cell differentiation by circularly polarized light transduced by chiral nanoassemblies

Aihua Qu et al.

Summary: Chiral photons can accelerate neural stem cells differentiation into neurons by engaging with DNA-bridged chiral assemblies of gold nanoparticles, resulting in improved conversion efficiency. The light-induced mechanical deformation of actin nanofibres at a frequency of 50 Hz plays a key role in stimulating the differentiation process. Additionally, circularly polarized light following a polarity-optimized protocol has shown promising results in reducing amyloid plaque formation in a mouse model of Alzheimer's disease.

NATURE BIOMEDICAL ENGINEERING (2021)

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Article Chemistry, Multidisciplinary

Spin-Dependent Photovoltaic and Photogalvanic Responses of Optoelectronic Devices Based on Chiral Two-Dimensional Hybrid Organic-Inorganic Perovskites

Jingying Wang et al.

Summary: Research has shown that integrating chiral organic ligands into two-dimensional hybrid organic-inorganic perovskites can introduce spintronics applications, leading to spin-dependent photovoltaic and photogalvanic responses. This discovery may have potential applications in optoelectronic devices sensitive to light helicity.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Consequences of Chirality in Directing the Pathway of Cholesteric Helix Inversion of π-Conjugated Polymers by Light

Chidambar Kulkarni et al.

Summary: Controlling main-chain motion of chiral pi-conjugated polymers through light manipulation can lead to unexpected new functionalities, with the configuration of chiral centers determining the handedness of polymer organization, and different light irradiation methods affecting polymer alignment and helicity.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Multi-Modal Chiral Superstructures in Self-Assembled Anthracene-Terminal Amino Acids with Predictable and Adjustable Chiroptical Activities and Color Evolution

Zhuoer Wang et al.

Summary: The study uncovers the universal existence of supramolecular tilt helical superstructures in self-assembled pi-conjugated amino acid derivatives, providing insights into the chiroptical phenomena and facilitating the rational design and fabrication of emerging chiroptical materials.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Chiral Lead-Free Hybrid Perovskites for Self-Powered Circularly Polarized Light Detection

Dong Li et al.

Summary: Metal-halide perovskites have emerged as promising alternatives for CPL detection due to their CPL-sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. This study successfully developed lead-free halide double perovskites, demonstrating significant chirality and self-powered CPL detection capabilities. The research suggests that hybrid double perovskites can be promising photoelectronic candidates for exploring new green circularly polarized light-sensitive materials with high performance.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Biochemical Research Methods

Angular optimization for cancer identification with circularly polarized light

Nozomi Nishizawa et al.

Summary: This study experimentally verified the potential for cancer identification using circularly polarized light scattering and observed significant differences in circular polarizations between cancerous and healthy tissues. Line-scanning experiments showed step-like behaviors in circular polarization corresponding to tissue states, whether cancerous or normal. Different resolutions for identifying cancerous tissues were induced by oblique and perpendicular incidence, indicating the importance of selecting optical arrangements based on resolution priorities.

JOURNAL OF BIOPHOTONICS (2021)

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Article Multidisciplinary Sciences

π-Extended perylene diimide double-heterohelicenes as ambipolar organic semiconductors for broadband circularly polarized light detection

Li Zhang et al.

Summary: In this study, a novel approach of skeleton merging was introduced to address the dilemma between strong coupling with circular polarized light and high charge-carrier mobility in high-performance chiral organic semiconducting molecules. The resulting pi-extended double helicene structure exhibits high dissymmetry factor, extended pi-planar system for charge transport properties, near-infrared light absorption, and ambipolar charge transport abilities, enabling high photoresponsivity and external quantum efficiency in both p- and n-type modes under NIR light irradiation. These characteristics allow for high-performance broadband CPL detections up to the NIR spectral region.

NATURE COMMUNICATIONS (2021)

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Article Materials Science, Multidisciplinary

Combining Soft with Hard Condensed Matter for Circular Polarized Light Sensing and Logic Operations

Paul Grey et al.

Summary: The study demonstrates a light sensor capable of discriminating right- from left-handed circular polarized light (CPL) by incorporating chiral nematic photonic cellulose nanocrystal (CNC) films with silicon-based thin-film photodiodes. By subjecting the films to specific wavelengths, photocurrents that are over 50% distinct between the two CP states are generated, providing a basis for binary output depending on the handedness of the light. Adding monovalent salt to the CNC suspension induces a blueshift to the photonic band gap, enabling a larger wavelength gamut and application possibilities, with measured results used to optimize device response through electromagnetic simulations.

ADVANCED OPTICAL MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Polarization-Sensitive Halide Perovskites for Polarized Luminescence and Detection: Recent Advances and Perspectives

Xiaobo Wang et al.

Summary: This paper comprehensively summarizes the research status and development direction in the field of polarization-sensitive HPs, introducing principles, methods, and strategies.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Local Growth Mediated by Plasmonic Hot Carriers: Chirality from Achiral Nanocrystals Using Circularly Polarized Light

Lucas Besteiro et al.

Summary: This study explores the possibility of growing chiral plasmonic nanocrystals from nonchiral seeds using circularly polarized light, and introduces a novel theoretical methodology to simulate realistic photogrowth processes. The results demonstrate strongly anisotropic and chiral growth of nanocrystals, even for those with subwavelength sizes.

NANO LETTERS (2021)

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Article Chemistry, Multidisciplinary

Circularly Polarized Light Detection by Chiral Photonic Cellulose Nanocrystal with ZnO Photoconductive Layer in Ultraviolet Region

Boyu Zhang et al.

Summary: This study proposes a novel design strategy for direct CPL detection using a combination of chiral photonic cellulose nanocrystals and ultraviolet-sensitive ZnO photoconductive materials. The design achieved the detection of CPL polarization state with competitive performance, providing a new approach for CPL detection.

NANOMATERIALS (2021)

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Article Chemistry, Multidisciplinary

Chirality Remote Control in Nanoporous Materials by Circularly Polarized Light

Anemar Bruno Kanj et al.

Summary: The study introduces a nanoporous solid material that induces chirality and enantioselective enrichment through circularly polarized light. Based on a crystalline metal-organic framework, the material utilizes photoswitchable fluorinated azobenzenes to induce chirality through trans-to-cis photoisomerization. Experimental results demonstrate that CPL causes chiral photoresolution, resulting in an optically active material.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Chiral 2D-Perovskite Nanowires for Stokes Photodetectors

Yingjie Zhao et al.

Summary: High-performance Stokes-parameter photodetectors are realized based on solution-processed chiral-perovskite nanowire arrays, which exhibit responsive circularly polarized light and large polarized ratio to linearly polarized light due to chiral ammonium cations and strictly aligned nanowires. The detectors demonstrate promising applications towards polarization imaging with their small footprint and high performance.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Realization of vis-NIR Dual-Modal Circularly Polarized Light Detection in Chiral Perovskite Bulk Crystals

Yu Peng et al.

Summary: This study presents the visible-near-infrared dual-modal CPL-sensitive direct detection in bulk single crystals of two-dimensional chiral perovskite for the first time. By designing new chiral semiconductors with strong light-matter interaction, high detection performance is achieved.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Heterogeneous Integration of Chiral Lead-Chloride Perovskite Crystals with Si Wafer for Boosted Circularly Polarized Light Detection in Solar-Blind Ultraviolet Region

Xinyuan Zhang et al.

Summary: By growing chiral HOIP single crystals onto silicon wafers, a strong built-in electric field at the heterojunction is generated, providing a driving force for separating/transporting carriers under CPL excitation. The transfer of chirality and significant amplification of circular polarization sensitivity in the transport process lead to an anisotropy factor of up to 0.4 at zero bias, making it the highest among reported CPL-UV photodetectors. This integration of chiral HOIP crystals with silicon technology opens up possibilities for high-performance CPL detectors in the solar-blind UV region and other advanced optoelectronic devices.

SMALL (2021)

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Article Optics

Multifunctional metasurfaces enabled by simultaneous and independent control of phase and amplitude for orthogonal polarization states

Mingze Liu et al.

Summary: Monochromatic light has three fundamental properties: amplitude, phase, and polarization. A versatile transmission-mode all-dielectric metasurface platform is proposed in this work, capable of independently manipulating the phase and amplitude for two orthogonal states of polarization in the visible frequency range, enabling various light-field manipulation capabilities. This technology opens new possibilities in polarization optics, information encoding, and optical data storage.

LIGHT-SCIENCE & APPLICATIONS (2021)

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Article Chemistry, Multidisciplinary

Great Amplification of Circular Polarization Sensitivity via Heterostructure Engineering of a Chiral Two-Dimensional Hybrid Perovskite Crystal with a Three-Dimensional MAPbI3 Crystal

Xinyuan Zhang et al.

Summary: The construction of a heterostructure crystal, integrating a chiral two-dimensional perovskite with its three-dimensional counterpart, significantly enhances circular polarization sensitivity for CPL detectors. This strategy allows for the creation of a CPL detector with a greatly amplified anisotropy factor, providing a novel approach to modulate circular polarization sensitivity in chiral hybrid perovskites for advanced chiroptical devices.

ACS CENTRAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Circularly Polarized Photodetectors Based on Chiral Materials: A Review

Can Zhang et al.

Summary: Chiral materials can directly detect CPL without the need for additional polarizers and quarter-wave plates. CPL photodetectors play a significant role in photonics techniques, including optical communication and spin information. Current challenges and future opportunities in the development of CPL photodetectors need further exploration.

FRONTIERS IN CHEMISTRY (2021)

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Article Materials Science, Multidisciplinary

Chiral hybrid organic-inorganic metal halides: A route toward direct detection and emission of polarized light

Herman Duim et al.

Summary: This article discusses the potential of chiral hybrid organic-inorganic metal halides (HMHs) in the field of optics, examining the impact of chiral transfer on electronic structure and optical properties. It further explores efforts to improve and tune the chiroptical response, while also proposing future research directions for enhancing chiral HMHs.

MATTER (2021)

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Article Chemistry, Multidisciplinary

Optically active covalent organic frameworks and hyperbranched polymers with chirality induced by circularly polarized light

Yuting Wang et al.

Summary: Axial chirality was induced in covalent organic frameworks and hyperbranched polymers using circularly polarized light, composed of benzene-1,3,5-triyl core units and oligo(benzene-1,4-diyl) linker units. The variation in induction efficiency was rationalized through internal rotation dynamics studied via CPMAS C-13 NMR experiments, including CODEX measurements.

CHEMICAL COMMUNICATIONS (2021)

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Article Polymer Science

Improved enantioselectivity in thiol-ene photopolymerization of sulphur-containing polymers with circularly polarized luminescence†

Chen-Lu He et al.

Summary: Circularly polarized light-triggered enantioselective thiol-ene reactions allow for the synthesis of optically active poly(thioether) directly from racemic monomers, but low enantioselectivity has been a challenge. The addition of achiral hydrogen atom donors can greatly enhance enantioselectivity and lead to the synthesis of poly(thioether) with distinct circularly polarized luminescence. The enantioselectivity of these reactions can be experimentally controlled by varying reaction kinetics, resulting in polymers with a significant excess of enantiomeric units.

POLYMER CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Metasurface-Empowered Optical Multiplexing and Multifunction

Shuqi Chen et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Chiral Reduced-Dimension Perovskite for an Efficient Flexible Circularly Polarized Light Photodetector

Lin Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Biochemistry & Molecular Biology

Homochiral Supramolecular Thin Film from Self-Assembly of Achiral Triarylamine Molecules by Circularly Polarized Light

Changjun Park et al.

MOLECULES (2020)

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Article Chemistry, Multidisciplinary

Guanosine Assembly Enabled Gold Nanorods with Dual Thermo- and Photoswitchable Plasmonic Chiroptical Activity

Song Wang et al.

ACS NANO (2020)

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Article Chemistry, Multidisciplinary

Aggregation-Induced Circularly Polarized Luminescence: Chiral Organic Materials for Emerging Optical Technologies

Andrea Nitti et al.

ADVANCED MATERIALS (2020)

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Enantioselective synthesis of near enantiopure compound by asymmetric autocatalysis triggered by asymmetric photolysis with circularly polarized light

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Asymmetric synthesis utilizing circularly polarized light mediated by the photoequilibrium of chiral olefins in conjunction with asymmetric autocatalysis

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Absolute asymmetric photoreactions of aliphatic amino acids by circularly polarized synchrotron radiation: Critically pH-dependent photobehavior

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Synthetic helical polymers: Conformation and function

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Synchronous enantiomeric enrichment of both reactant and product by absolute asymmetric synthesis using circularly polarized light. Part 1. Theoretical and experimental verification of the asymmetric photoisomerization of methyl norbornadiene-2-carboxylate to methyl quadricyclane-1-carboxylate

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Control of chirality of an azobenzene liquid crystalline polymer with circularly polarized light

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Switching a helical polymer between mirror images using circularly polarized light

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