期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 138, 期 4, 页码 1162-1165出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b12880
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资金
- National Science Foundation [CHE-0955864, CHE-1464898]
- Bristol-Myers Squibb
- Dreyfus Foundation
- UCLA Gold Shield Alumnae
- University of California, Los Angeles
- National Science Foundation for a GRFP [DGE-1144087]
- UCLA Graduate Division
- NSF [CHE-1048804]
- National Center for Research Resources [S10RR025631]
- Direct For Mathematical & Physical Scien [1464898] Funding Source: National Science Foundation
- Division Of Chemistry [1464898] Funding Source: National Science Foundation
The akuammiline alkaloids are a family of natural products that have been widely studied for decades. Although notable synthetic achievements have been made recently, akuammilines that possess a methanoquinolizidine core have evaded synthetic efforts. We report an asymmetric approach to these alkaloids, which has culminated in the first total syntheses of (-)-2(S)-cathafoline and the long-standing target (+)-strictamine. Moreover, the first enantioselective total synthesis of aspidophylline A is described.
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