Flexible and Stretchable Organic Electrochemical Transistors for Physiological Sensing Devices

Article Multidisciplinary Sciences

Vertical organic electrochemical transistors for complementary circuits

Wei Huang et al.

NATURE (2023)

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Article Multidisciplinary Sciences

High-performance and low-power source-gated transistors enabled by a solution-processed metal oxide homojunction

Xinming Zhuang et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2023)

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Article Chemistry, Multidisciplinary

Fully Transparent, Ultrathin Flexible Organic Electrochemical Transistors with Additive Integration for Bioelectronic Applications

Ashuya Takemoto et al.

Summary: Fully transparent, ultrathin, and flexible organic electrochemical transistors (OECTs) were successfully developed using the additive integration processes of selective-wetting deposition and thermally bonded lamination. These OECTs demonstrate high visible transmittance and high transconductance, with low-voltage operations. EEG acquisition and nitrate ion sensing can be performed while wearing the transparent OECTs, and simultaneous assessments of optical blood flowmetry are also compatible.

ADVANCED SCIENCE (2023)

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Article Materials Science, Multidisciplinary

Ultra-Lightweight, Highly Permeable, and Waterproof Fibrous Organic Electrochemical Transistors for On-Skin Bioelectronics

Shuai Chen et al.

Summary: This article reports a highly stable and comfortable fibrous electrolyte with potential applications in on-skin electronics.

ADVANCED MATERIALS TECHNOLOGIES (2023)

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Article Chemistry, Multidisciplinary

Perovskite Solar Cell-Gated Organic Electrochemical Transistors for Flexible Photodetectors with Ultrahigh Sensitivity and Fast Response

Jiajun Song et al.

Summary: In this study, a high-performance flexible photodetector is realized by gating an organic electrochemical transistor with a perovskite solar cell. The device exhibits high gain, fast response time, and ultrahigh detectivity under a low working voltage, allowing it to track photoplethysmogram signals and peripheral oxygen saturation. This work offers a novel strategy for high-performance flexible photodetectors in low-power, user-friendly, and wearable optoelectronics.

ADVANCED MATERIALS (2023)

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Article Engineering, Electrical & Electronic

Fully 3D-printed organic electrochemical transistors

Matteo Massetti et al.

Summary: A direct-write additive process was developed to fabricate fully 3D-printed organic electrochemical transistors (OECTs) using 3D printable inks. These OECTs can be fabricated on flexible substrates, providing high mechanical and environmental stability. They exhibit good dopamine biosensing capabilities and long-term synapse response, making them suitable for various applications such as sensors and neuromorphic hardware.

NPJ FLEXIBLE ELECTRONICS (2023)

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Article Chemistry, Multidisciplinary

Influence of Molecular Weight on the Organic Electrochemical Transistor Performance of Ladder-Type Conjugated Polymers

Han-Yan Wu et al.

Summary: Fine-tuning the molecular weight of rigid, ladder-type polymers can significantly enhance the performance of n-type OECTs, achieving record-high geometry-normalized transconductance, electron mobility, and volumetric capacitance. This improvement is attributed to more efficient intermolecular charge transport in high-molecular-weight polymers. Additionally, complementary inverters based on OECTs have demonstrated remarkable voltage gains and ultralow power consumption, making them among the best sub-1 V inverters reported to date.

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

Flexible organic electrochemical transistors for chemical and biological sensing

Li Wang et al.

Summary: Flexible organic electrochemical transistors (OECTs) have great potential in chemical and biological sensing due to their high sensitivity, biocompatibility, low cost, and light weight. This review summarizes recent progress in the fabrication and applications of flexible OECTs in sensing. Material selection, structural engineering, gate modification, and array-based sensors are discussed, highlighting the versatility and promising applications of OECT sensors.

NANO RESEARCH (2022)

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Article Biotechnology & Applied Microbiology

Genetically encoded photo-switchable molecular sensors for optoacoustic and super-resolution imaging

Kanuj Mishra et al.

Summary: Reversibly photo-switchable proteins have been utilized for super-resolution and optoacoustic imaging methods, and in this study, a prototype of a photo-switchable Ca2+ sensor was constructed based on GCaMP5G. The molecular mechanisms of the sensor were described at the structural level, demonstrating the ability to image calcium and other analytes at super-resolution and in vivo.

NATURE BIOTECHNOLOGY (2022)

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Article Biotechnology & Applied Microbiology

Sensitive identification of neoantigens and cognate TCRs in human solid tumors

Marion Arnaud et al.

Summary: NeoScreen is a method that enables sensitive identification of rare tumor antigens and corresponding T cell receptors, which can be used for personalized cancer vaccines and T cell therapies. T cells transduced with tumor antigen-specific TCRs identified by NeoScreen can regress established tumors in patient-derived xenograft mice.

NATURE BIOTECHNOLOGY (2022)

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Article Nanoscience & Nanotechnology

Three-dimensional transistor arrays for intra- and inter-cellular recording

Yue Gu et al.

Summary: The research introduces a scalable platform featuring a three-dimensional field-effect transistor array produced via compressive buckling, enabling accurate recording of transmembrane potentials and intracellular recordings in cells and cellular networks. The platform utilizes high-performance field-effect transistors for cellular interfacing, providing faithful recordings and valuable experimental data for probing the electrical behaviors of single cells and cellular networks. Leveraging the high spatial and temporal resolutions of the transistors, the study reveals new insights into signal conduction velocities and pathways within cells and cellular constructs.

NATURE NANOTECHNOLOGY (2022)

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Article Materials Science, Multidisciplinary

Tuning the antiaromatic character and charge transport of pentalene-based antiaromatic compounds by substitution

Jianglin Wu et al.

Summary: This study presents the design, synthesis, and characterization of three new antiaromatic molecules based on the pentalene core, demonstrating how electron-donating and electron-accepting substituents affect their properties. The introduction of strong electron-withdrawing or electron-donating substituents onto the antiaromatic core effectively activates charge transport capacity, as confirmed by organic field-effect transistors fabricated using these materials.

JOURNAL OF MATERIALS CHEMISTRY C (2022)

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Article Nanoscience & Nanotechnology

Printed Organic Electrochemical Transistors for Detecting Nutrients in Whole Plant Sap

Elliot J. Strand et al.

Summary: Low-cost biosensors capable of rapidly monitoring plant nutritional levels have been developed in this study, with a focus on detecting potassium concentrations in plant sap. These biosensors demonstrate a log-linear response within the expected physiological range of cations in plants, showing high sensitivity and low detection limits. These printed devices can be used for high-throughput plant health monitoring in agricultural and ecological applications.

ADVANCED ELECTRONIC MATERIALS (2022)

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Article Nanoscience & Nanotechnology

All-Inkjet-Printed Graphene-Gated Organic Electrochemical Transistors on Polymeric Foil as Highly Sensitive Enzymatic Biosensors

Silvia Demuru et al.

Summary: In this study, fully inkjet-printed graphene-gated organic electrochemical transistors (OECTs) on polymeric foil were demonstrated for the enzymatic-based biosensing of glucose and lactate. The graphene-gated transistors showed improved performance compared to printed silver-gated devices and other types of printed devices previously reported. The optimized sensing method and device configuration enabled the detection of multiple metabolites.

ACS APPLIED NANO MATERIALS (2022)

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Article Nanoscience & Nanotechnology

Photopatternable Poly(dimethylsiloxane) (PDMS) for an Intrinsically Stretchable Organic Electrochemical Transistor

Joohyuk Kang et al.

Summary: In this study, a photopatternable elastomer called TC-PDMS was developed. TC-PDMS showed high-resolution patternability and had similar stretchability and Young's modulus as conventional PDMS. The application of TC-PDMS in stretchable bioelectric devices demonstrated its ability to record electrocardiographic signals.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Chemistry, Multidisciplinary

Heteroalkyl-Substitution in Molecular Organic Semiconductors: Chalcogen Effect on Crystallography, Conformational Lock, and Charge Transport

Shakil N. Afraj et al.

Summary: The effect of heteroalkyl substitution on molecular semiconductors is studied. The devices based on tetradecylated DDTT-SeBT exhibit the highest electron mobility when fabricated by the solution-shearing method.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Stretchable Redox-Active Semiconducting Polymers for High-Performance Organic Electrochemical Transistors

Yahao Dai et al.

Summary: Organic electrochemical transistors (OECTs) have high amplification and sensitivity to biological signals, making them a promising platform for next-generation bioelectronics. However, achieving seamless tissue-electronics interfaces with softness and stretchability has been a challenge due to the lack of stretchable redox-active semiconducting polymers. This study reports a stretchable semiconductor for OECT devices, which exhibits exceptional stretchability and high OECT performance. The polymer's design features, including a nonlinear backbone architecture, moderate side-chain density, and high molecular weight, enable the combination of stretchability and OECT performance. The highly stretchable polymer semiconductor allows for fabricating intrinsically stretchable OECTs with high transconductance and biaxial stretchability, and demonstrates on-skin electrocardiogram recording with built-in amplification and unprecedented skin conformability.

ADVANCED MATERIALS (2022)

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Article Materials Science, Multidisciplinary

Woven fiber organic electrochemical transistors based on multiwalled carbon nanotube functionalized PEDOT nanowires for nondestructive detection of potassium ions

Yao Wang et al.

Summary: Fiber-based organic electrochemical transistors (FECTs) functionalized with poly(3,4-ethylenedioxythiophene)/multiwalled carbon nanotube channel have been developed to detect ultralow concentration of potassium ions in the human body. The sensors show fast response, good reproducibility, and excellent anti-interference ability, and can be easily integrated into fabric for wearable healthcare monitoring.

MATERIALS SCIENCE AND ENGINEERING B-ADVANCED FUNCTIONAL SOLID-STATE MATERIALS (2022)

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Article Chemistry, Physical

Highly stretchable organic electrochemical transistors with strain-resistant performance

Jianhua Chen et al.

Summary: This study presents a novel design strategy for stretchable organic electrochemical transistors, utilizing a honeycomb semiconducting polymer morphology for high stretchability and stable charge transport, making it suitable for various stretchable bioelectronic applications.

NATURE MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Biocompatible Ionic Liquids in High-Performing Organic Electrochemical Transistors for Ion Detection and Electrophysiological Monitoring

Ting Li et al.

Summary: This study investigates the use of a biocompatible ionic liquid [MTEOA][MeOSO3] as an additive to enhance the performance of PEDOT:PSS-based OECTs for biosensing applications. The PEDOT:PSS/[MTEOA][MeOSO3]-based OECTs show high transconductance, fast response time, and excellent switching cyclical stability. The integration of ion-selective membranes enables selective ion detection, while flexible OECTs are designed for electrocardiography (ECG) signal acquisition, showing robust performance against physical deformation and high-quality signal recording.

ACS NANO (2022)

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Article Chemistry, Multidisciplinary

Gas-Permeable Organic Electrochemical Transistor Embedded with a Porous Solid-State Polymer Electrolyte as an on-Skin Active Electrode for Electrophysiological Signal Acquisition

Jiabin Wang et al.

Summary: This study developed fibrous nanomesh organic electrochemical transistors embedded with porous solid-state polymer electrolytes for use as on-skin active electrodes, enabling the acquisition of high-quality electrocardiogram signals.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Inkjet-Printed Xerogel Scaffolds Enabled Room-Temperature Fabrication of High-Quality Metal Electrodes for Flexible Electronics

Shuaichen Wang et al.

Summary: This study presents a new method to address the issues faced in inkjet-printed metal electrodes. By inkjet printing a stable xerogel scaffold and growing high-quality copper electrodes through electroless deposition, metal electrodes with desirable electrical properties are achieved at room temperature. These metal electrodes demonstrate excellent uniformity, surface smoothness, and high interfacial energy with plastic substrates, making them suitable for fabricating various electronic devices.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Multidisciplinary Sciences

A flexible and highly sensitive organic electrochemical transistor-based biosensor for continuous and wireless nitric oxide detection

Yuping Deng et al.

Summary: A flexible and highly sensitive biosensor based on organic electrochemical transistors (OECTs) has been developed for continuous and wireless detection of nitric oxide (NO) in biological systems. The sensor shows a low response limit, wide linear range, high sensitivity, and excellent selectivity, and can continuously detect NO in the nanomolar range for hours without significant signal drift.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2022)

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Article Materials Science, Multidisciplinary

Wafer-scale microfabrication of flexible organic electrochemical transistors

Quentin Thiburce et al.

Summary: We present a photolithographic process for fabricating organic microdevices on flexible substrates. The process utilizes standard cleanroom wafer processing equipment and involves the use of a conductive polymer as the active material for organic electrochemical transistors. The transistors can be operated with both solid-state ion gel electrolytes and aqueous electrolytes, making them suitable for flexible integrated circuits and biosensors. Additionally, the process demonstrates the ability to define small features, as shown by the miniaturized transistors with 2 μm-long channels. The proposed process offers a high resolution alternative to printing techniques by leveraging established semiconductor device manufacturing techniques and facilities.

FLEXIBLE AND PRINTED ELECTRONICS (2022)

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Article Chemistry, Multidisciplinary

Readily Accessible Metallic Micro-Island Arrays for High-Performance Metal Oxide Thin-Film Transistors

Jaehyun Kim et al.

Summary: A new strategy was reported to achieve high-performance solution-processed metal oxide thin-film transistors by introducing metallic micro-island array on top of the metal oxide back channel. Al-MIA IGZO TFTs exhibited superior performance compared to controls, with high electron mobility and broad applicability.

ADVANCED MATERIALS (2022)

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Article Biophysics

Sensitive organic electrochemical transistor biosensors: Comparing single and dual gate functionalization and different COOH-functionalized bioreceptor layers

Yunjia Song et al.

Summary: The new measurement configurations based on organic electrochemical transistors (OECTs) have shown improved sensitivity and precision in detecting antibody-antigen interactions. By utilizing specific bioreceptor layers and dual gate functionalization, drift effects are minimized, leading to more accurate results.

BIOSENSORS & BIOELECTRONICS (2022)

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Article Electrochemistry

Layer-by-layer assembly of composite conductive fiber-based organic electrochemical transistor for highly sensitive detection of sialic acid

Rufeng Zhu et al.

Summary: A novel conductive fiber composite based on layer-by-layer assembly technology has been successfully prepared. The composite fiber exhibits flexibility, conductivity, and washability. The fiber-based organic electrochemical transistors (FECTs) assembled from the composite fiber show excellent electrical properties and stability. A sialic acid biosensor based on the modified gate electrode of FECTs has been developed, which can detect the sialic acid content in saliva. The sensor can be seamlessly integrated into fabrics, providing an efficient detection platform for wearable healthcare applications.

ELECTROCHIMICA ACTA (2022)

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Article Chemistry, Multidisciplinary

Antibody-Coated Wearable Organic Electrochemical Transistors for Cortisol Detection in Human Sweat

Silvia Demuru et al.

Summary: The dysregulation of cortisol is associated with various pathological states, and monitoring cortisol levels can help prevent severe stress, fatigue, and mental illnesses. Existing methods for cortisol detection face challenges due to its low concentration and the high ionic strength of biofluids. However, a label-free and fast sensor based on antibody-coated organic electrochemical transistors has been developed, offering high sensitivity for cortisol detection. This wearable device enables point-of-care cortisol detection in a short amount of time, allowing personalized well-being monitoring.

ACS SENSORS (2022)

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Article Multidisciplinary Sciences

Wearable microneedle-based electrochemical aptamer biosensing for precision dosing of drugs with narrow therapeutic windows

Shuyu Lin et al.

Summary: The study introduces a microneedle-based electrochemical aptamer biosensing patch for minimally invasive monitoring of interstitial fluid and real-time measurement of drug pharmacokinetics. By transforming a clinical-grade needle into a high-quality gold nanoparticle-based substrate through a cost-effective fabrication scheme, reliable in vivo detection of ISF analytes, including those without natural recognition elements, is achieved.

SCIENCE ADVANCES (2022)

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Article Engineering, Electrical & Electronic

Flexible organic integrated electronics for self-powered multiplexed ocular monitoring

Baojun Lin et al.

Summary: Smart contact lens has attracted extensive research interest for its noninvasive real-time detection of the human body and provision of biomedical information. In this study, we successfully demonstrated a self-powered multiplexed sensor based on organic solar cells, which can detect biomarkers in tears and transmit the signals wirelessly to a computer.

NPJ FLEXIBLE ELECTRONICS (2022)

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Article Engineering, Electrical & Electronic

Systematic Analysis of Self-Assembled Nanodielectric Architecture and Organization Effects on Organic Transistor Switching

Katie Stallings et al.

Summary: The unconventional self-assembled nanodielectric (SAND) architecture, composed of alternating inorganic and pi-organic layers, shows superior thin-film transistor performance and is compatible with various semiconductors. The interactions within the organic layers play a significant role in the structural organization and dielectric response of SAND.

ACS APPLIED ELECTRONIC MATERIALS (2022)

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Review Materials Science, Multidisciplinary

The 2021 flexible and printed electronics roadmap

Yvan Bonnassieux et al.

Summary: This roadmap presents perspectives and visions from leading researchers in the fields of flexible and printable electronics, covering device technologies, fabrication techniques, and design and modeling approaches essential for future development of new applications leveraging flexible electronics (FE). It aims to serve as a resource on the current status and future challenges, highlighting the broad opportunities made available by FE technologies.

FLEXIBLE AND PRINTED ELECTRONICS (2021)

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Review Chemistry, Multidisciplinary

Organic Electrochemical Transistors for In Vivo Bioelectronics

Ali Nawaz et al.

Summary: Organic electrochemical transistors (OECTs) are a focus of intense research with great potential in expanding the horizons of the bioelectronics industry. Their unique characteristics, such as electrolyte-gating and aqueous stability, make them particularly suitable for in vivo applications. OECTs form a soft mechanical contact with the biological milieu, ensuring a high signal-to-noise ratio and amplification capability, making them desirable for a wide range of in vivo applications.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

A Transparent, Highly Stretchable, Solvent-Resistant, Recyclable Multifunctional Ionogel with Underwater Self-Healing and Adhesion for Reliable Strain Sensors

Liguo Xu et al.

Summary: This study introduces multifunctional ionogels with desirable properties prepared via one-step photoinitiated polymerization, showing excellent mechanical strength, resilience, and underwater adhesion. The ionogels, rich in noncovalent interactions, exhibit high tolerance against water and various organic solvents, making them promising for wearable sensors in detecting large body motions and subtle muscle movements.

ADVANCED MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Influence of Side Chains on the n-Type Organic Electrochemical Transistor Performance

David Ohayon et al.

Summary: n-Type polymers with electron transporting properties are crucial in transducing biological events involving electron generation. Researchers have developed a new family of donor-acceptor-type polymers based on the NDI-T2 backbone, studying how side chain variations affect polymer film performance in bioelectronic devices like OECTs.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Fabrication of Aptamer-Modified Paper Electrochemical Devices for On-Site Biosensing

Haixiang Yu et al.

Summary: Electrochemical aptamer-based sensors are powerful tools for analyte detection, and paper-based sensors offer a portable, low-cost, and rapid detection method for a broad range of targets. By using ambient vacuum filtration, we have developed a simple, economic, and environmentally friendly strategy for fabricating aptamer-modified paper electrochemical devices (PEDs) with customizable three-electrode systems, enabling sensitive and specific detection of small molecules in minimally processed biosamples. The sensitivity and stability of these aptamer-modified PEDs are comparable to commercial gold electrode-based E-AB sensors, suggesting the potential for high performance on-site detection of various analytes.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

High-Gain Chemically Gated Organic Electrochemical Transistor

Siew Ting Melissa Tan et al.

Summary: Organic electrochemical transistors (OECTs) have shown promising performance as transducers and amplifiers of low potentials due to their exceptional transconductance enabled by the volumetric charging of organic mixed ionic/electronic conductors (OMIECs). However, current approaches that directly conduct chemical reactions within the OECT electrolyte do not fully leverage the OECT's large transconductance, resulting in sub-unity transduction of gate to drain current. This study presents an alternative device architecture that separates chemical transduction and amplification processes to achieve high-gain chemical OECT transducers.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Multidisciplinary Sciences

Transition metal-catalysed molecular n-doping of organic semiconductors

Han Guo et al.

Summary: The study presents a method for achieving higher n-doping efficiency in a shorter time using precursor molecular dopants, as well as discussing the technological implications for improved semiconductor devices and new opportunities in n-doping research and applications.

NATURE (2021)

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Article Multidisciplinary Sciences

Flexible complementary circuits operating at sub-0.5 V via hybrid organic inorganic electrolyte-gated transistors

Yao Yao et al.

Summary: High-performance EGT complementary circuits with balanced electrical output for both p-type and n-type components have been achieved, enabling ultrahigh voltage gains and low driving voltages. NAND and NOR logic circuits with excellent logic response and impressive mechanical flexibility have been realized. The HCIN also enables amplification and monitoring of EOG signals, critical for wearable medical sensors and human-computer interaction interfaces.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

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Article Chemistry, Analytical

Microfluidics integrated n-type organic electrochemical transistor for metabolite sensing

Anil Koklu et al.

Summary: The study demonstrates the integration of a microfluidic system with an n-type accumulation mode OECT for real-time enzymatic metabolite detection. The integrated design provides new insights into the mechanisms leading to high sensor sensitivities, crucial for the development of portable and autonomous lab-on-a-chip technologies.

SENSORS AND ACTUATORS B-CHEMICAL (2021)

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Article Nanoscience & Nanotechnology

Self-Assembled Nanodielectrics for Solution-Processed Top-Gate Amorphous IGZO Thin-Film Transistors

Katie Stallings et al.

Summary: Metal oxide semiconductors, such as a-IGZO, have shown impressive progress as alternatives to amorphous silicon in electronics applications, but require compatible unconventional gate dielectric materials. Solution-processable self-assembled nanodielectrics (SANDs) composed of alternating organic and inorganic oxide layers offer high capacitances and low processing temperatures, yet have not been implemented in the top-gate TFT architecture.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Microfluidic Integrated Organic Electrochemical Transistor with a Nanoporous Membrane for Amyloid-β Detection

Anil Koklu et al.

Summary: Alzheimer's disease is a neurodegenerative disorder with no specific cure, emphasizing the importance of early diagnosis. A common pathological change in AD-affected brains is the accumulation of Aβ protein into plaques, which was detected using a micron-scale OECT in this study.

ACS NANO (2021)

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Article Nanoscience & Nanotechnology

Ionic Network Based on Dynamic Ionic Liquids for Electronic Tattoo Application

Zhiwu Chen et al.

Summary: Electronic tattoos are gaining popularity in wearable electronics for their lightweight and noninvasive features, but face challenges in terms of flexibility, skin compatibility, adhesion, repairability, and erasability. By using a dynamic ionic liquid, a flexible electronic tattoo with healing and erasable abilities has been developed, allowing for intelligent monitoring of physiological indicators and simultaneous detection of multiple signals, showing great potential in the field of intelligent wearable electronics.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Doping Indium Oxide Films with Amino-Polymers of Varying Nitrogen Content Markedly Affects Charge Transport and Mechanical Flexibility

Zhi Wang et al.

Summary: This study investigates the correlation between polymer structure and charge transport in solution-processed indium oxide: polymer blend flexible thin film transistors. By introducing amino-polymers, it is possible to enhance electron doping capacity and carrier mobility, thereby improving the performance of TFTs.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Organic Electrochemical Transistor Common-Source Amplifier for Electrophysiological Measurements

James E. Tyrrell et al.

Summary: This study explores the potential and advantages of OECT amplifiers in bioelectronics by implementing high-performance interdigitated electrode OECTs. By determining the stability of performance parameters through variations in OECT geometries and conducting simulations and physical measurements, the study demonstrates the superior performance of OECT amplifiers in transducing and amplifying physiological signals.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Ultrahigh-Gain Organic Electrochemical Transistor Chemosensors Based on Self-Curled Nanomembranes

Leticia M. M. Ferro et al.

Summary: This study presents microtubular electrochemical devices based on strain engineering, utilizing the unique shape features of self-curled nanomembranes to achieve high-performance OECTs. These novel OECTs exhibit lower operating voltage, improved ion doping, and higher signal amplification gain, and can be used to detect biomarkers related to neurological diseases.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Pushing the Limits of Flexibility and Stretchability of Solar Cells: A Review

Emilie Dauzon et al.

Summary: Emerging forms of soft, flexible, and stretchable electronics have the potential to revolutionize the future electronics industry, with stretchable photovoltaics as self-powering systems showing great promise for various applications. Current research is focused on achieving wearability and stretchability in electronic systems, utilizing both extrinsic and intrinsic approaches for inducing stretchability.

ADVANCED MATERIALS (2021)

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Article Multidisciplinary Sciences

An organic transistor matrix for multipoint intracellular action potential recording

Yasutoshi Jimbo et al.

Summary: An organic electrochemical transistor (OECT) matrix is shown for intracellular action potential recording, where the driving voltage simultaneously causes electroporation. The recorded peak amplitudes were larger than extracellular field potential recording, and could be further enhanced by tuning the driving voltage and OECT geometry. Miniaturization and multiplexed recording capabilities were demonstrated through a 4 x 4 action potential mapping using a matrix of 5- x 5-mu m(2) OECTs, realized with a mild fabrication process and simple circuit without limiting potential applications of organic electronics.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

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Review Engineering, Biomedical

Sensing Inflammation Biomarkers with Electrolyte-Gated Organic Electronic Transistors

Bernhard Burtscher et al.

Summary: The overview of cytokine biosensing on organic electronic platforms highlights the importance of monitoring inflammation biomarkers in real time. The technologies provided by OECTs and EGOFETs offer low-cost point-of-care solutions that can significantly benefit the healthcare system and professionals.

ADVANCED HEALTHCARE MATERIALS (2021)

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Review Engineering, Biomedical

Current-Driven Organic Electrochemical Transistors for Monitoring Cell Layer Integrity with Enhanced Sensitivity

Katharina Lieberth et al.

Summary: This report provides an overview of using organic electrochemical transistors (OECT) as biosensors for impedance sensing of cell layers, with a focus on the enhanced ion-sensitivity achieved through current-driven OECT. The potential applications of this technology in drug delivery and toxicology studies are also discussed.

ADVANCED HEALTHCARE MATERIALS (2021)

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Article Nanoscience & Nanotechnology

Integrated Ionic-Additive Assisted Wet-Spinning of Highly Conductive and Stretchable PEDOT:PSS Fiber for Fibrous Organic Electrochemical Transistors

Yanping Chen et al.

Summary: In this study, an integrated ionic-additive assisted wet-spinning strategy was used to improve the conductivity and stretchability of PEDOT:PSS fiber, resulting in a fiber with extremely high conductivity and 30% stretchability. Additionally, an all-solid-state fibrous organic electrochemical transistor (OECT) device with a transconductance of 2.44 mS was fabricated based on this fiber.

ADVANCED ELECTRONIC MATERIALS (2021)

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Article Multidisciplinary Sciences

Ultrafast, sensitive, and portable detection of COVID-19 IgG using flexible organic electrochemical transistors

Hong Liu et al.

Summary: A rapid, low-cost, and portable SARS-CoV-2 IgG detection platform based on OECTs was reported, with remote control via mobile phone. By optimizing ion concentrations and pH values, specific detection of the virus was achieved in minutes, showing promise in the diagnosis and prognosis of COVID-19.

SCIENCE ADVANCES (2021)

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Article Chemistry, Multidisciplinary

A sensitive platform for DNA detection based on organic electrochemical transistor and nucleic acid self-assembly signal amplification

Chaohui Chen et al.

Summary: This study demonstrated a highly sensitive DNA detection method by combining OECT and HCR, showing great potential in improving detection efficiency and selectivity.

RSC ADVANCES (2021)

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Article Multidisciplinary Sciences

Electrolyte-gated transistors for enhanced performance bioelectronics

Fabrizio Torricelli et al.

Summary: This primer discusses the various architectures and mechanisms of electrolyte-gated transistors (EGTs), as well as their applications in bioelectronics. It covers the materials and fabrication methods used in EGT structures, as well as the integration of functional bio-layers and biosystems. The primer also explores the advantages, limitations, possible optimizations, and future directions of EGTs in the field of bioelectronics.

NATURE REVIEWS METHODS PRIMERS (2021)

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Review Materials Science, Multidisciplinary

Dielectric materials for electrolyte gated transistor applications

Wei Huang et al.

Summary: This review summarizes recent progress in developing dielectric materials for electrolyte gated transistors (EGTs), emphasizing the importance of electrolyte dielectrics and their impact on EGT performance and integration. The discussion covers various types of electrolyte dielectric materials, driven by different applications, and highlights the structure and operation of emerging electrolyte-based transistors. Overall, the understanding and development of electrolyte dielectrics have opened up new possibilities for EGTs and related devices.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Review Materials Science, Multidisciplinary

n-Type organic semiconducting polymers: stability limitations, design considerations and applications

Sophie Griggs et al.

Summary: This review outlines the design strategies and challenges for developing high performing n-type materials in OTFT, OECT, and OTE fields. It discusses the limitations of n-type materials, specifically their ambient stability issues, and suggests synthetic methods to overcome them. Recent advancements in high performing n-type materials are detailed, along with their design principles.

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