Site-Specific Chemistry on Gold Nanorods: Curvature-Guided Surface Dewetting and Supracolloidal Polymerization

Review Chemistry, Multidisciplinary

Chemical and Physical Properties of Photonic Noble-Metal Nanomaterials

Yi-Yu Cai et al.

Summary: Colloidal noble metal nanoparticles can be assembled into different forms of artificial metamolecules and materials with tunable optical properties, allowing manipulation of light transmission and reflection.

ADVANCED MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Ion Beam Milling as a Symmetry-Breaking Control in the Synthesis of Periodic Arrays of Identically Aligned Bimetallic Janus Nanocrystals

Walker J. Tuff et al.

Summary: Bimetallic Janus nanostructures are highly functional nanomaterials that maintain partially exposed surfaces due to the union of two chemically distinct metal segments. This study demonstrates the use of a collimated ion beam as a control to selectively remove a passivating oxide shell from one side of a metal nanostructure, resulting in a substrate-bound Au-Ag Janus nanostructure. The developed procedures enable the realization of complex Janus architectures arranged in periodic arrays, advancing the field of nanometal syntheses directed by oxides.

ACS NANO (2023)

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Article Chemistry, Multidisciplinary

Self-Assembly of Atomically Aligned Nanoparticle Superlattices from Pt-Fe3O4 Heterodimer Nanoparticles

Shengsong Yang et al.

Summary: This study demonstrates the self-assembly of heterodimers consisting of two conjoined nanoparticles into multicomponent superlattices with long-range atomic alignment between the different nanoparticles. The self-assembly process exhibits a two-stage mechanism, indicating the selective epitaxial growth of the smaller domain and specific size ratios of the heterodimer domains are required for atomic alignment.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2023)

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Review Chemistry, Multidisciplinary

Molecular Engineering of Colloidal Atoms

Yan Cui et al.

Summary: Creating architectures with precise hierarchies drives the development of revolutionary functions and applications in various fields. By utilizing diverse interparticle driving motifs, such as confining templates, interactive surface ligands, and flexible shape/surface anisotropy, it is possible to organize atom-like micro- and nanoparticles into colloidal analogs of molecules. In addition, the self-regulated/adaptive co-assembly of simple unvarnished building blocks is discussed to inspire new designs of colloidal assembly strategies.

SMALL (2023)

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Article Chemistry, Multidisciplinary

Halogen Bonding-Driven Reversible Self- Assembly of Plasmonic Colloidal Molecules

Wenhao Dong et al.

Summary: This study describes the reversible self-assembly of plasmonic nanoparticles capped with complementary copolymer ligands into colloidal molecules via halogen bonding interactions. The coordination number of the colloidal molecules is determined by the number ratio of complementary halogen groups on the interacting nanoparticles. The reversibility of the halogen bonds allows for controlling the formation and disassociation of the colloidal molecules and their optical properties. The engineered reversible nanostructures may have applications in sensing, catalysis, and optoelectronic devices.

ACS NANO (2023)

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Article Multidisciplinary Sciences

A theory of entropic bonding

Thi Vo et al.

Summary: Entropy can self-assemble hard nanoparticles into colloidal crystals with structures similar to atomic and molecular crystals. A first-principles theory is proposed to describe the directional entropic forces between hard shapes by calculating and minimizing the excluded volume. The theory successfully predicts the thermodynamically preferred structures for different families of hard polyhedra.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2022)

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Review Chemistry, Multidisciplinary

Polymer-Tethered Nanoparticles: From Surface Engineering to Directional Self-Assembly Published as part of the Accounts of Chemical Research special issue Self-Assembled Nanomaterials

Ning-Ning Zhang et al.

Summary: Current interest in nanoparticle ensembles is driven by their unique collective properties that surpass those of individual nanoparticles and bulk materials. Self-assembly provides a cost-effective way to create well-defined and predictable ensembles of nanoparticles. Polymer-functionalized nanoparticles are ideal building blocks for self-assembled nanostructures due to their similar dimensions and the ability to synthesize various types of polymers. Furthermore, polymer ligands can add additional functionalities to nanoparticle assemblies, expanding their range of applications.

ACCOUNTS OF CHEMICAL RESEARCH (2022)

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Article Chemistry, Multidisciplinary

Local Chain Feature Mandated Self-Assembly of Block Copolymers

Zhanhui Gan et al.

Summary: This work demonstrates an effective approach to regulating phase behaviors of block copolymers by programming local features into linear chains. Through designing sequence-defined isomeric block copolymers, different phase behaviors can be achieved without changing the chemical structure or composition. The research highlights the significant impact of rearranging methylene units among the side chains on self-assembly processes and resulting nanostructures.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Multidisciplinary Sciences

Symmetry-breaking in patch formation on triangular gold nanoparticles by asymmetric polymer grafting

Ahyoung Kim et al.

Summary: This study demonstrates quantitative control over asymmetric polymer grafting on triangular Au nanoprisms based on polymer scaling theory. The authors show that polymers can selectively adsorb onto nanoparticle surfaces already partially coated by other chains, resulting in the formation of patchy nanoparticles with broken symmetry. These asymmetric nanoparticles exhibit intriguing plasmonic properties and their formation can be accurately predicted by a developed theory.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Multidisciplinary

Dual Atomic Coherence in the Self-Assembly of Patchy Heterostructural Nanocrystals

Hua Zhu et al.

Summary: Advances in synthesis and self-assembly techniques of nanocrystals have allowed researchers to create various nanoparticle superlattices. However, achieving rotational order of nanoparticle building blocks within the lattice has proven to be more challenging. In this study, a combination of experiments and molecular dynamics simulations was used to investigate the self-assembly of heterostructural nanocrystals (HNCs). The self-assembled HNCs formed face-centered-cubic superlattices with well-defined orientational relationships between the atomic lattices of the quantum dot hosts and gold patches. The study provides a strategy for designing and fabricating nanocrystal superlattices with complex structures and delicate orientational order.

ACS NANO (2022)

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Article Chemistry, Multidisciplinary

Patchy metal nanoparticles with polymers: controllable growth and two-way self-assembly

Hanyi Duan et al.

Summary: This study presents a novel design of polymer-patched gold nanoparticles with controllable interparticle interactions, achieving highly controllable growth and assembly of nanoparticles for hierarchical nanomaterials with interesting optical properties. The self-assembly pathway plays a crucial role in determining the interparticle distance and plasmon coupling, opening up new possibilities for the directional self-assembly of anisotropic building blocks.

NANOSCALE (2022)

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Article Chemistry, Multidisciplinary

Plasmon Energy Transfer in Hybrid Nanoantennas

Sean S. E. Collins et al.

Summary: The study synthesized hybrid nanoantennas through photo-electrochemistry, consisting of plasmonic nanoparticles with photo-conductive polymer coatings. It was found that polymerization is enhanced by photoexcitation, achieving up to 50% efficiency of nonradiative energy transfer.

ACS NANO (2021)

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Review Chemistry, Multidisciplinary

Gold Nanorods: The Most Versatile Plasmonic Nanoparticles

Jiapeng Zheng et al.

Summary: Gold nanorods are a versatile material with anisotropic shape and adjustable plasmonic properties, which have been widely used in various fields. Continuous improvement in synthetic methods enables diverse applications of Au NRs and exploration of cutting-edge technologies. The future research directions and challenges will focus on further improving synthetic methods to expand the application scope of Au NRs.

CHEMICAL REVIEWS (2021)

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Article Chemistry, Physical

Symmetry-Reduced Metal Nanostructures Offer New Opportunities in Plasmonics and Catalysis

Zachary J. Woessner et al.

Summary: Metallic nanoparticles exhibit interesting optical and catalytic properties based on their composition, size, shape, and architecture, often defined by their symmetry. Recent research has shown that symmetric reduction of NPs can be achieved in a controlled manner during seed-mediated syntheses, leading to unique and tunable optoelectronic and catalytic properties.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Article Multidisciplinary Sciences

Enhanced optical asymmetry in supramolecular chiroplasmonic assemblies with long-range order

Jun Lu et al.

Summary: The study demonstrates that the limitations of optical asymmetry in chiral assemblies of plasmonic nanoparticles can be overcome by long-range organization of nanoparticles, similar to liquid crystals. This long-range order in helical assemblies enhances optical asymmetry by reducing scattering and activating energy states with antiparallel orientation of dipoles.

SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Block-Random Copolymer-Micellization-Mediated Formation of Polymeric Patches on Gold Nanoparticles

Yiqun Yang et al.

Summary: This article presents a strategy for the scalable synthesis of high-quality patchy nanoparticles, which are produced by thermal treatment of a mixture of gold nanoparticles and thiol-terminated block-random copolymers to generate nanoparticles with controlled morphology and number of polymeric patches. Experiments and simulations show that the formation of polymeric patches is governed by the dynamic detachment/attachment of copolymers and the exchange of copolymers between the nanoparticle surface and free micelles in the solution.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Multidisciplinary Sciences

Macroscopic materials assembled from nanoparticle superlattices

Peter J. Santos et al.

Summary: Nanoparticle assembly is proposed as an ideal means to program the hierarchical organization of materials, allowing for control of nano- and microstructures while preserving nanoscale ordering. This method enables the manipulation of structural organization across molecular to macroscopic length scales.

NATURE (2021)

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Article Chemistry, Multidisciplinary

Synthesis, Assembly, Optical Properties, and Sensing Applications of Plasmonic Gap Nanostructures

Jae-Myoung Kim et al.

Summary: Plasmonic gap nanostructures have attracted extensive research due to their strongly enhanced optical responses, but the reproducible and controlled preparation of highly uniform nanogaps and the prediction, understanding, and control of their optical properties remain challenging.

ADVANCED MATERIALS (2021)

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Review Chemistry, Multidisciplinary

Controlled Assembly of Plasmonic Nanoparticles: From Static to Dynamic Nanostructures

Sunghee Lee et al.

Summary: The spatial arrangement of plasmonic nanoparticles can significantly affect their interaction with electromagnetic waves and control their optical properties. Recent advances in bottom-up chemical strategies have enabled precise control over the assembly structure of metal nanoparticles, leading to the construction of smart dynamic nanostructures capable of reversible structural changes.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Stereoselective Growth of Small Molecule Patches on Nanoparticles

Jiajing Zhou et al.

Summary: This study demonstrates a method for forming three-dimensional patches in aqueous environments using small molecules in a single step, with patch characteristics modulated by self-polymerizable aromatic dithiol and comixed ligands, indicating an autonomous assembly mechanism. This approach is independent of nanoparticle material and dimension, providing a streamlined and powerful toolset for designing heterogeneous patches at the nanoscale.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Macromolecular Ligand Engineering for Programmable Nanoprism Assembly

Yang Liu et al.

Summary: This study introduces macromolecular ligand-engineering strategies to control four molecular parameters and synthesize and assemble nanocrystals. By ligand exchange, nanocrystals are functionalized on different facets and self-assemble into supercrystals of different structures.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Editorial Material Chemistry, Multidisciplinary

From Nano to Macro: Thinking Bigger in Nanoparticle Assembly

Robert J. Macfarlane

Summary: Nanoparticle assembly allows for the synthesis of complex nanoscale structures, but further research and application will necessitate the development of new processing methods to control both micro- and macroscale structures.

NANO LETTERS (2021)

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Article Chemistry, Multidisciplinary

Electrostatic co-assembly of nanoparticles with oppositely charged small molecules into static and dynamic superstructures

Tong Bian et al.

Summary: The use of small molecules with electric charges can effectively induce attractive interactions between oppositely charged nanoparticles in water, guiding their assembly into colloidal crystals. This approach offers a facile way to fabricate, manipulate, and investigate nanostructured materials in aqueous environments.

NATURE CHEMISTRY (2021)

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Article Polymer Science

Symmetry-Broken Patches on Gold Nanoparticles through Deficient Ligand Exchange

Hanyi Duan et al.

Summary: This study presents a method for preparing high-quality symmetry-broken plasmonic gold nanoparticles and achieving asymmetric surface patterning through deficient ligand exchange. The conformational entropy of polymer ligands and the interfacial energy between polymer-grafted nanoparticles and the solvent play key roles in the formation of asymmetric surface patches.

ACS MACRO LETTERS (2021)

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Article Chemistry, Multidisciplinary

Symmetry in Seeded Metal Nanocrystal Growth

Sara E. Skrabalak

Summary: Symmetry plays a crucial role in nanomaterials, with seeded methods enabling the synthesis of complex multimetallic crystals for applications in plasmonics and catalysis. The underlying symmetry of seeds can be predictably transferred to final crystals during overgrowth, but can also be reduced in a controlled manner.Some key factors affecting symmetry preservation or reduction during seeded crystal growth include the concentrations of metal precursors and capping agents.

ACCOUNTS OF MATERIALS RESEARCH (2021)

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Review Chemistry, Multidisciplinary

Surface Capping Agents and Their Roles in Shape-Controlled Synthesis of Colloidal Metal Nanocrystals

Tung-Han Yang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Multidisciplinary Sciences

Self-limiting directional nanoparticle bonding governed by reaction stoichiometry

Chenglin Yi et al.

SCIENCE (2020)

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Article Chemistry, Multidisciplinary

What is next in polymer-grafted plasmonic nanoparticles?

Hanyi Duan et al.

GIANT (2020)

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Review Chemistry, Multidisciplinary

Polymer-guided assembly of inorganic nanoparticles

Chenglin Yi et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Self-Assembled Responsive Bilayered Vesicles with Adjustable Oxidative Stress for Enhanced Cancer Imaging and Therapy

Jibin Song et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Alternating Copolymerization of Inorganic Nanoparticles

Chenglin Yi et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Tip-Patched Nanoprisms from Formation of Ligand Islands

Ahyoung Kim et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

General Approach to the Synthesis of Heterodimers of Metal Nanoparticles through Site-Selected Protection and Growth

Jichuan Qiu et al.

NANO LETTERS (2019)

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Regioselective surface encoding of nanoparticles for programmable self-assembly

Gang Chen et al.

NATURE MATERIALS (2019)

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DNA-Encoded Protein Janus Nanoparticles

Oliver G. Hayes et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Article Chemistry, Multidisciplinary

Assembly and Dynamic Plasmonic Tuning of Ag Nanoparticles Enabled by Limited Ligand Protection

Luntao Liu et al.

NANO LETTERS (2018)

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Article Multidisciplinary Sciences

Superstructures generated from truncated tetrahedral quantum dots

Yasutaka Nagaoka et al.

NATURE (2018)

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Single-component quasicrystalline nanocrystal superlattices through flexible polygon tiling rule

Yasutaka Nagaoka et al.

SCIENCE (2018)

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Article Chemistry, Multidisciplinary

Oxidation State of Capping Agent Affects Spatial Reactivity on Gold Nanorods

Joshua G. Hinman et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

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Article Chemistry, Multidisciplinary

Surface Engineering of Spherical Metal Nanoparticles with Polymers toward Selective Asymmetric Synthesis of Nanobowls and Janus-Type Dimers

Ben Liu et al.

SMALL (2017)

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Article Chemistry, Multidisciplinary

Harnessing Colloidal Crack Formation by Flow-Enabled Self-Assembly

Bo Li et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Review Chemistry, Multidisciplinary

Bimetallic Nanocrystals: Syntheses, Properties, and Applications

Kyle D. Gilroy et al.

CHEMICAL REVIEWS (2016)

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Synthesis of Platinum Nanotubes and Nanorings via Simultaneous Metal Alloying and Etching

Zhiqi Huang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2016)

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Self-Assembling Nanocomposite Tectons

Jianyuan Zhang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2016)

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Surface patterning of nanoparticles with polymer patches

Rachelle M. Choueiri et al.

NATURE (2016)

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Diamond family of nanoparticle superlattices

Wenyan Liu et al.

SCIENCE (2016)

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1D nanocrystals with precisely controlled dimensions, compositions, and architectures

Xinchang Pang et al.

SCIENCE (2016)

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Selective assemblies of giant tetrahedra via precisely controlled positional interactions

Mingjun Huang et al.

SCIENCE (2015)

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Unconventional seed-mediated growth of ultrathin Au nanowires in aqueous solution

Bo Li et al.

CHEMICAL SCIENCE (2015)

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A general route to nanocrystal kebabs periodically assembled on stretched flexible polymer shish

Hui Xu et al.

SCIENCE ADVANCES (2015)

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Crafting Threads of Diblock Copolymer Micelles via Flow-Enabled Self-Assembly

Bo Li et al.

ACS NANO (2014)

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Copolymerization of Metal Nanoparticles: A Route to Colloidal Plasmonic Copolymers

Kun Liu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2014)

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Single-Particle Spectroscopy Reveals Heterogeneity in Electrochemical Tuning of the Localized Surface Plasmon

Chad P. Byers et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2014)

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Successive, Seed-Mediated Growth for the Synthesis of Single-Crystal Gold Nanospheres with Uniform Diameters Controlled in the Range of 5-150 nm

Yiqun Zheng et al.

PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION (2014)

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Anisotropic Overgrowth of Metal Heterostructures Induced by a Site-Selective Silica Coating

Feng Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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Self-Assembly of Amphiphilic Plasmonic Micelle-Like Nanoparticles in Selective Solvents

Jie He et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Seeded Growth of Monodisperse Gold Nanorods Using Bromide-Free Surfactant Mixtures

Xingchen Ye et al.

NANO LETTERS (2013)

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Hydrophobic Interactions Modulate Self-Assembly of Nanoparticles

Ana Sanchez-Iglesias et al.

ACS NANO (2012)

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Review Chemistry, Multidisciplinary

Functional Gold Nanorods: Synthesis, Self-Assembly, and Sensing Applications

Leonid Vigderman et al.

ADVANCED MATERIALS (2012)

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Thermoresponsive Assembly of Charged Gold Nanoparticles and Their Reversible Tuning of Plasmon Coupling

Yiding Liu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2012)

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Self-Assembly of Inorganic Nanoparticle Vesicles and Tubules Driven by Tethered Linear Block Copolymers

Jie He et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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Toward Plasmonic Polymers

Liane S. Slaughter et al.

NANO LETTERS (2012)

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Steric Hindrance Induces crosslike Self-Assembly of Gold Nanodumbbells

Marek Grzelczak et al.

NANO LETTERS (2012)

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Self-orienting nanocubes for the assembly of plasmonic nanojunctions

Bo Gao et al.

NATURE NANOTECHNOLOGY (2012)

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Shape-anisotropic colloids: Building blocks for complex assemblies

Stefano Sacanna et al.

CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2011)

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Plasmonic Vesicles of Amphiphilic Gold Nanocrystals: Self-Assembly and External-Stimuli-Triggered Destruction

Jibin Song et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2011)

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Effects of Symmetry Breaking and Conductive Contact on the Plasmon Coupling in Gold Nanorod Dimers

Liane S. Slaughter et al.

ACS NANO (2010)

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Article Chemistry, Physical

Thermal stability of gold nanorods in an aqueous solution

Renxian Zou et al.

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2010)

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Solvent-Mediated End-to-End Assembly of Gold Nanorods

Yiliang Wang et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2010)

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DNA-nanoparticle superlattices formed from anisotropic building blocks

Matthew R. Jones et al.

NATURE MATERIALS (2010)

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Step-Growth Polymerization of Inorganic Nanoparticles

Kun Liu et al.

SCIENCE (2010)

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Dumbbell-like Pt-Fe3O4 Nanoparticles and Their Enhanced Catalysis for Oxygen Reduction Reaction

Chao Wang et al.

NANO LETTERS (2009)

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Review Chemistry, Multidisciplinary

Shape control in gold nanoparticle synthesis

Marek Grzelczak et al.

CHEMICAL SOCIETY REVIEWS (2008)

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Controlled assembly of eccentrically encapsulated gold nanoparticles

Tao Chen et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2008)

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Supramolecular assembly of gold nanorods end-terminated with polymer Pom-Poms: Effect of pom-pom structure on the association modes

Zhihong Nie et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2008)

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Self-assembly of metal-polymer analogues of amphiphilic triblock copolymers

Zhihong Nie et al.

NATURE MATERIALS (2007)

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Anisotropy of building blocks and their assembly into complex structures

Sharon C. Glotzer et al.

NATURE MATERIALS (2007)

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Divalent metal nanoparticles

Gretchen A. DeVries et al.

SCIENCE (2007)

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Self-assembly of polymer-tethered nanorods

MA Horsch et al.

PHYSICAL REVIEW LETTERS (2005)

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Review Chemistry, Physical

Anisotropic metal nanoparticles: Synthesis, assembly, and optical applications

CJ Murphy et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2005)

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Preferential end-to-end assembly of gold nanorods by biotin-streptavidin connectors

KK Caswell et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2003)

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A hybridization model for the plasmon response of complex nanostructures

E Prodan et al.

SCIENCE (2003)

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Dependence of the gold nanorod aspect ratio on the nature of the directing surfactant in aqueous solution

JX Gao et al.

LANGMUIR (2003)

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Seeding growth for size control of 5-40 nm diameter gold nanoparticles

NR Jana et al.

LANGMUIR (2001)

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Site-Specific Chemistry on Gold Nanorods: Curvature-Guided Surface Dewetting and Supracolloidal Polymerization

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