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Inspired by Wood: Thick Electrodes for Supercapacitors

ACS NANO (2023)

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Bing Yan et al.

Summary: Structural and compositional optimization of carbon-based electrodes can significantly improve capacitive properties. In this study, a facile and efficient approach was proposed to anchor N/O-codoped carbon nanotubes on carbonized wood matrix, resulting in unique three-dimensional hierarchically porous structures and interconnected conductive networks. The electrodes exhibited ultrahigh mass loading and impressive capacitive properties.

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Summary: This study presents a method to fabricate a lightweight carbonized wood (CW) electrode with high loading of active materials and conductivity, resulting in an integrated electrode with remarkable energy density and rate performance in supercapacitors.

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Zhen Zhang et al.

Summary: Constructing a thick electrode with excellent electrochemical performance using carbon materials is a challenge due to poor ion transport and conductivity. In this study, a low-tortuous, hierarchically porous, and aligned channels thick electrode was developed without complex structural design. This approach demonstrates potential for lightweight carbon-based thick electrodes for energy storage applications.

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Hygroscopic Chemistry Enables Fire-Tolerant Supercapacitors with a Self-Healable Solute-in-Air Electrolyte

Huarong Xia et al.

Summary: This study demonstrates a fire-tolerant supercapacitor that can recover after burning with a self-healable solute-in-air electrolyte. By using fire-tolerant electrodes and separator, along with a hygroscopic electrolyte that absorbs water from the air for self-recovery at low temperatures, the supercapacitor exhibits high safety and reliability.

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A. Dias et al.

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Assessment of the effectiveness of liquid hot water and steam explosion pretreatments of fast-growing poplar (Populus trichocarpa) wood

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Summary: The study compared the effects of liquid hot water and steam explosion pretreatment methods on fast-growing Populus trichocarpa wood, finding that pretreatment significantly improved enzymatic digestibility and chemical composition of the wood, particularly affecting the content of hemicelluloses.

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Summary: In this study, conductive carbon aerogels with ultralow density and superhydrophilicity were developed based on synergistic hydrogen bonding, electrostatic interaction, and pi-pi interaction within regularly arranged layered porous structures. These aerogels exhibit high compressibility, fatigue resistance, excellent capacitive performance, and can be used as strain sensors.

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Removal of flue gas mercury by porous carbons derived from one-pot carbonization and activation of wood sawdust in a molten salt medium

Jianping Yang et al.

Summary: Porous carbons derived from one-pot carbonization and activation of wood sawdust in a molten salt medium showed superior performance in Hg-0 removal compared to carbons derived from N-2 pyrolysis method. The best molar ratio of LiCl-KCl was found to be 59:41, with an optimal molten salt temperature of 700 degrees C and a mass ratio of wood sawdust to molten salt of 1:10. The carbonization method displayed good applicability at temperatures ranging from 50 to 125 degrees C, with a high saturation Hg-0 adsorption capacity.

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Wood-Derived High-Mass-Loading MnO2 Composite Carbon Electrode Enabling High Energy Density and High-Rate Supercapacitor

Lian Chen et al.

Summary: This study reports the high-mass-loading of manganese oxide (MnO2) electrode with wood-derived carbon (WC) as the current collector for high-energy-density devices. The WC@MnO2-20 electrode showed remarkable high-rate performance and high capacitance retention. The obtained symmetric supercapacitor exhibited high areal/specific capacitance and high energy densities, with good cyclic stability. This research provides a feasible strategy for the design of high-energy-density supercapacitors.

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Summary: In order to make electric vehicles more viable for the general population, rechargeable batteries need to support rapid charging and increase energy density. This study introduces graphite oxide frameworks with enlarged interlayer spacing through a solvothermal reaction, resulting in ultrafast charging properties.

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Summary: In this study, novel layered MnO2 nanodots were synthesized and utilized as the cathode material for aqueous zinc-ion batteries/hybrid capacitors (ZIBs/ZICs) for the first time. The delta-MnO2 NDs displayed high specific capacity, impressive rate capacity, large specific energy, and superior durability. The H+/Zn2+ co-insertion energy storage mechanism of the cathode was also verified. The quantization design strategy provides a new approach for the design and development of advanced cathodes for aqueous ZIBs and ZICs.

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Wood Biochar Monolith-Based Approach to Increasing the Volumetric Energy Density of Supercapacitor

Lin Yang et al.

Summary: This study presents a novel approach for fabricating high-performance thick electrodes using wood biochar monoliths (WBMs). The thick electrode made with intensified WBMs exhibited record-high capacitances and could be easily augmented with pseudocapacitive materials. This research provides a practical method for increasing the volumetric energy density and demonstrates the potential of WBMs as a low-cost, high-performance alternative to advanced nanoporous carbon materials.

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Feng Wang et al.

Summary: This study explores the development of thick carbon electrodes derived from basswood and their application in high energy density supercapacitors. The anisotropic structural carbon electrodes derived from wood exhibit different transfer kinetics of the electrolyte, which significantly impacts the electrochemical performance, especially at high current density. The results show that the cross-sectional wood-derived carbon with high specific surface area contributes to excellent electrochemical performance, attributed to its hierarchical porous structure that allows easy access for the electrolytes even at high current density. This work provides insights into the dynamic behaviors of electrolyte in different wood sections and can be extended to other wood species and wood-like structures for energy storage applications.

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Summary: This article reviews the application of nanocellulose materials in sustainable energy storage, particularly in the field of supercapacitors. Nanocellulose-derived composite materials exhibit good electrical conductivity and tunable microstructures, showing great potential. The article introduces the fabrication strategies of nanocellulose-derived hybrid materials and discusses the use of nanocellulose in constructing composite electrode materials for supercapacitors.

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Summary: This study successfully prepared transparent wood with improved mechanical properties, thermal stability, and hydrophobicity through the treatment and coating of wood. The transparent wood underwent sodium chlorite treatment, epoxy impregnation, and perfluorodecyltriethoxysilane coating, resulting in enhanced transparency and functionality.

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Chenting Zhang et al.

Summary: The study on the pyrolysis of cellulose revealed that high temperature affects the transformation of organics and the evolution of bio-char structure. With increasing temperature, the bio-oil production first increases and then decreases, while the structure of bio-char undergoes reconstruction, forming different functional groups and graphite structures.

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3D Porous Oxidation-Resistant MXene/Graphene Architectures Induced by In Situ Zinc Template toward High-Performance Supercapacitors

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Summary: In this study, a wood-derived carbon thick electrode with a thickness of 1.532 mm demonstrated the best supercapacitance performance, with high active material loading, specific capacitance, and power densities. It also exhibited excellent cycling stability.

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Ruwei Chen et al.

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