期刊
CELL REPORTS PHYSICAL SCIENCE
卷 4, 期 1, 页码 -出版社
CELL PRESS
DOI: 10.1016/j.xcrp.2022.101210
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This study investigates multivalent cations-modulated low-frequency noise in graphene nanopores and demonstrates that the noise originates from surface charge fluctuations induced by reversible adsorption-desorption of ions. The amplitude of the noise can be greatly controlled up to about 3 orders of magnitude by adding trace amounts of multivalent cations. Additionally, the low-frequency noise can be suppressed by 2 orders of magnitude by adding organic solvents with a high dielectric constant to inhibit interactions between surface charge and ions.
Atomically thin 2D nanopores have emerged as promising platforms from nanofluidics research to practical applications. Low-frequency flicker noise in 2D nanopores limits detection accuracy and perfor-mance of nanopore sensors. However, the physical mechanisms of low-frequency noise are still under debate and achieving its control in 2D nanopores remains challenging. Here, we report multivalent -cations-modulated low-frequency noise in graphene nanopores and demonstrate that low-frequency noise originates from surface charge fluctuations induced by reversible adsorption-desorption of ions. Unexpectedly, its amplitude can be greatly controlled up to about 3 orders of magnitude by a trace of multivalent cations (at least 0.1% of concentration in mixture solutions). Moreover, low-frequency noise can be suppressed by 2 orders of magnitude via adding organic solvents with a high dielectric constant based on suppressing interactions between surface charge and ions. Our findings will facilitate understanding of low-frequency noise in nano -fluidics and design of related applications including ultrasensitive nanofluidic devices.
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