期刊
JOURNAL OF SEPARATION SCIENCE
卷 40, 期 1, 页码 314-335出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/jssc.201600849
关键词
Biomacromolecules; Membranes; Molecularly imprinted polymers; Surface imprinting; Thin films
资金
- Australian component of the European Framework Programme 7 (FP7)
- Commonwealth of Australia (Department of Innovation Industry, Research and Science) under the International Science Linkages (ISL) program
This review describes recent advances associated with the development of surface imprinting methods for the synthesis of polymeric membranes and thin films, which possess the capability to selectively and specifically recognize biomacromolecules, such as proteins and single-and double-stranded DNA, employing epitope or whole molecule approaches. Synthetic procedures to create different molecularly imprinted polymer membranes or thin films are discussed, including grafting/in situ polymerization, drop-, dip-, or spin-coating procedures, electropolymerization as well asmicro-contact or stamp lithography imprinting methods. Highly sensitive techniques for surface characterization and analyte detection are described, encompassing luminescence and fluorescence spectroscopy, X-ray photoelectron spectroscopy, FTIR spectroscopy, surface-enhanced Raman spectroscopy, atomic force microscopy, quartz crystal microbalance analysis, cyclic voltammetry, and surface plasmon resonance. These developments are providing new avenues to produce bioelectronic sensors and new ways to explore through advanced separation science procedures complex phenomena associated with the origins of biorecognition in nature.
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