期刊
SURFACES AND INTERFACES
卷 37, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.surfin.2023.102710
关键词
CNC-g-PAA; MnO2; Nanorods; Catalytic activity; Antimicrobial activity; Molecular docking analysis
Cellulose nanocrystal grafted poly acrylic acid (CNC-g-PAA) doped MnO2 nanorods with different concentrations were synthesized. The influence of CNC-g-PAA on the catalysis and antibacterial behavior of MnO2 was analyzed. Various characterization approaches were used to investigate the optical, structural, morphological features, and chemical composition of the synthesized materials. The catalytic activity of CNC-g-PAA doped MnO2 increased gradually with a higher doping ratio, and 9 mL CNC-g-PAA doped MnO2 showed significant antibacterial effects against Escherichia coli.
Various concentrations of cellulose nanocrystal grafted poly acrylic acid (CNC-g-PAA) doped MnO2 nanorods (NRs) were synthesized through a hydrothermal process. This work aimed to analyze the influence of CNC-g-PAA (3, 6, and 9 mL) on MnO2 for catalysis and antibacterial behavior. Various characterization approaches were utilized to investigate the optical, structural, morphological features, and chemical composition of synthesized materials. FTIR results were used to assess the vibrational and rotational modes of the presence of functional groups (O-H, C-O and Mn-O) in synthesized samples. Electronic spectra revealed a bathochromic shift upon doping that led to decrease in band gap energy. The catalytic activity of CNC-g-PAA doped MnO2 increased gradually with a higher doping ratio owing to a reduction in electron-hole (e(-) -h(+)) pair recombination. As a result, 9 mL CNC-g-PAA doped MnO2 is suggested as a valuable and superior catalyst for cleaning the envi-ronment and wastewater. In addition, 9 mL CNC-g-PAA doped MnO2 revealed a significant inhibition area for Escherichia coli in comparison to Staphylococcus aureus at high and low doses correspondingly. Further, molecular docking studies of these NRs were performed to get insight into the mystery behind these bactericidal activities.
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