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Ni-based ultrathin nanostructures for overall electrochemical water splitting

MATERIALS CHEMISTRY FRONTIERS (2023)

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Article Chemistry, Multidisciplinary

In Situ Electronic Redistribution Tuning of NiCo2S4 Nanosheets for Enhanced Electrocatalysis

Hui Su et al.

Summary: Metal Ru and vacancy engineering are used to enhance the activity of NiCo2S4 electrocatalysts for both oxygen evolution and hydrogen evolution reactions. Decorated with Ru single atoms and nanoclusters, the electrocatalysts exhibit significantly improved OER and HER performance, outperforming most reported materials in overall water splitting. Bader charge analysis reveals the promotion of electron interactions, contributing to the enhanced electrochemical performance.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Physical

Iron, rhodium-codoped Ni2P nanosheets arrays supported on nickel foam as an efficient bifunctional electrocatalyst for overall water splitting

Meng-Ting Chen et al.

Summary: In order to enhance the overall water splitting efficiency, low-cost, abundant, and efficient bifunctional electrocatalysts for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) are highly attractive yet challenging. The Fe,Rh-codoped Ni2P nanosheets arrays exhibited excellent catalytic performance for both OER and HER, with a small voltage of 1.62 V to drive a current density of 10 mA cm(-2) for overall water splitting. This work provides an alternative option for fabricating advanced catalysts in electrocatalysis and energy devices.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Article Chemistry, Physical

A chainmail effect of ultrathin N-doped carbon shell on Ni2P nanorod arrays for efficient hydrogen evolution reaction catalysis

Heng Zhang et al.

Summary: The innovative chainmail design enhances the activity and stability of water splitting reactions, with Ni2P@NC/NF showing better performance under alkaline and neutral conditions compared to pure Ni2P, along with high Faradaic efficiency.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2022)

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Review Chemistry, Multidisciplinary

Emerging 2D materials for antimicrobial applications in the pre- and post-pandemic era

Cemile Gokce et al.

Summary: Infectious diseases caused by viral or bacterial pathogens pose serious threats to humanity and can lead to pandemics, as seen with COVID-19. Nanotechnology, particularly 2D materials, offer promising antimicrobial solutions for disinfection, surface coatings, air filtering, and drug delivery systems to combat future pandemics.

NANOSCALE (2022)

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Article Chemistry, Multidisciplinary

Fluorine Engineered Self-Supported Ultrathin 2D Nickel Hydroxide Nanosheets as Highly Robust and Stable Bifunctional Electrocatalysts for Oxygen Evolution and Urea Oxidation Reactions

Swati J. Patil et al.

Summary: In the field of electrocatalytic water splitting, developing efficient noble-metal-free electrocatalysts remains a challenge. A scalable one-step synthesis approach was used to prepare self-supported fluorine-modified 2D ultrathin nickel hydroxide nanosheets, which demonstrated enhanced redox activity, electrical conductivity, and a large number of exposed active sites for improved charge migration during electrocatalytic reactions.

SMALL (2022)

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Article Chemistry, Physical

Iron-nickel aerogels anchored on GO nanosheets as efficient oxygen evolution reaction catalysts under industrial conditions

Yiwen Zhang et al.

Summary: In this study, a facile method was used to prepare a nickel-iron aerogel and graphene oxide composite, which exhibited high activity and stability in electrocatalytic water splitting. The special morphology and synergistic effect of the composite allowed for high current density at a low overpotential, and it showed considerable performance even in industrial operating environments.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Chemistry, Multidisciplinary

Sulfur and oxygen dual vacancies manipulation on 2D NiS2/CeO2 hybrid heterostructure to boost overall water splitting activity

W. Y. Liao et al.

Summary: The 2-dimensional NiS2/CeO2 with unique heterostructure and abundant sulfur and oxygen vacancies (v-NiS2/CeO2 HS) prepared through solvothermal reaction and annealing shows positive effects on promoting the kinetics of oxygen evolution reaction and hydrogen evolution reaction, resulting in low overpotential and high current density. This provides a direction for the development of low-cost, earth-abundant electrocatalysts.

MATERIALS TODAY CHEMISTRY (2022)

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Article Chemistry, Physical

Robust Pt/TiO2/Ni(OH)2 nanosheet arrays enable outstanding performance for high current density alkaline water electrolysis

Aiqun Kong et al.

Summary: In this study, a novel and simple strategy to construct Pt-decorated TiO2/beta-Ni(OH)(2) nanosheet arrays was developed. It was found that the few-layered Ti3C2 played a versatile role in the unique growth mechanism of Pt/TiO2/beta-Ni(OH)(2). The interconnected array electrode exhibited remarkable hydrogen evolution reaction (HER) performance at high current densities, outperforming most reported HER electrocatalysts. The synergistic effect of Pt and TiO2/Ni(OH)(2) was demonstrated to enhance the HER performance.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Experimental investigations on morphology controlled bifunctional NiO nano-electrocatalysts for oxygen and hydrogen evolution

Vishesh Manjunath et al.

Summary: This study reports on morphology-controlled NiO electrocatalyst as a single catalyst for both oxygen and hydrogen evolution. The 0D nanoparticles exhibit better overpotential and long-term stability compared to the 2D porous NiO nanoplates due to their larger surface area and active sites.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Electrochemistry

Non-Thermal Plasma Assisted Fabrication of Ultrathin NiCoOx Nanosheets for High-Performance Supercapacitor

Birhanu Bayissa Gicha et al.

Summary: Ultrathin nanosheets fabricated from TMLDHs using Ar-plasma exfoliation strategy show improved supercapacitive performance, with high areal capacitance and excellent cyclic stability. The material also exhibits good energy density and power density, making it a promising candidate for energy conversion and storage applications.

BATTERIES & SUPERCAPS (2022)

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Article Chemistry, Multidisciplinary

Design of NiCo2O4@NiMoO4 core-shell nanoarrays on nickel foam to explore the application in both energy storage and electrocatalysis

Ya'nan Meng et al.

Summary: NiCo2O4@NiMoO4 core-shell nanowires and nanosheets with high electrochemical capabilities were successfully synthesized. These materials exhibited large specific capacity, excellent cycling stability, and high-rate capability, making them promising candidates for energy storage and electrocatalysis.

MATERIALS CHEMISTRY FRONTIERS (2022)

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Article Materials Science, Multidisciplinary

Electronic structure regulation of an ultra-thin MOF-derived NiSe2/NiS2@NC heterojunction for promoting the hydrogen evolution reaction

Kebin Lu et al.

Summary: Transition metal selenides are considered promising electrocatalysts for the hydrogen evolution reaction due to their narrow bandgap, unique morphology, and low cost. In this study, a NiSe2/NiS2@NC electrocatalyst with abundant heterogeneous interfaces was designed and synthesized using a metal-organic framework as a precursor, showing improved catalytic performance in HER due to optimized electronic structure and accelerated kinetics.

MATERIALS ADVANCES (2022)

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Article Chemistry, Physical

Tuning the morphology and electron structure of metal-organic framework-74 as bifunctional electrocatalyst for OER and HER using bimetallic collaboration strategy

Cheng Chen et al.

Summary: 2D NiFe-MOF-74 nanosheets on nickel foam exhibit increased surface area, efficient utilization of active metal sites, and enhanced electrocatalytic activity through the collaboration of Ni and Fe metals, making them promising for water-splitting applications.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Energy & Fuels

Review on Synthesis and Catalytic Coupling Mechanism of Highly Active Electrocatalysts for Water Splitting

Wenhao Liu et al.

Summary: In summary, although IrO2 and Pt/C are currently considered as state-of-the-art electrocatalysts for water splitting, their poor durability and high cost highlight the need for the development of new, low-cost, highly active, and stable electrocatalysts. The alloy effect, interface effect, various defects, and doping effects are believed to be the main reasons to improve the intrinsic catalytic activities of electrocatalysts.

ENERGY TECHNOLOGY (2021)

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Article Chemistry, Physical

Cu2Se nanowires shelled with NiFe layered double hydroxide nanosheets for overall water-splitting

Hongyun Qi et al.

Summary: A core-shell nanostructure Cu2Se@NiFe-LDHNS electrocatalyst with excellent OER and HER performance is reported, providing an efficient strategy for overall water-splitting. The catalyst shows a synergistic effect from ultrathin NiFe-LDHNS, Cu2Se nanowires, and the core-shell structure, offering large surface area and ample active sites.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Review Materials Science, Multidisciplinary

Ni-based layered double hydroxide catalysts for oxygen evolution reaction

L. Yang et al.

Summary: This review comprehensively summarizes recent developments of Ni-based layered double hydroxides (LDHs) in oxygen evolution reaction (OER), including fabrication strategies, electrocatalyst applications, and structural modifications. It identifies obstacles hindering the practical use of Ni-based LDHs and emphasizes the need for more research in structural rational design and application in real water electrolysis techniques.

MATERIALS TODAY PHYSICS (2021)

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Article Chemistry, Physical

Fe doping and oxygen vacancy modulated Fe-Ni5P4/NiFeOH nanosheets as bifunctional electrocatalysts for efficient overall water splitting

Cheng-Fei Li et al.

Summary: This study demonstrates the efficient design of bifunctional catalysts using doping and vacancy double control strategy for the significant enhancement of hydrogen and oxygen evolution reactions. The Fe-doped Ni5P4/Fe-doped Ni(OH)2 hybrid nanosheets with rich oxygen vacancies show excellent catalytic performances with low overpotentials and cell voltage for water splitting.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Electrochemistry

Selenide/sulfide heterostructured NiCo2Se4/NiCoS4 for oxygen evolution reaction, hydrogen evolution reaction, water splitting and Zn-air batteries

Keke Wang et al.

Summary: A novel NiCo2Se4/NiCoS4 catalyst with excellent performance in OER, HER, OWS, and ZABs has been developed, showing small overpotentials and superior stability compared to benchmark catalysts. The structural advantages of the nanoflowers and heterostructure interfaces are key to the catalytic synergistic effects, making the catalyst promising for electrochemical devices.

ELECTROCHIMICA ACTA (2021)

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Article Chemistry, Inorganic & Nuclear

Electrochemically Controlled Synthesis of Ultrathin Nickel Hydroxide Nanosheets for Electrocatalytic Oxygen Evolution

Li-Ming Cao et al.

Summary: By utilizing a high electrodeposition potential, a novel OER catalyst with abundant catalytically active sites and specific micro-nano structure has been successfully synthesized on the material surface, exhibiting excellent electrocatalytic performance at low overpotentials.

INORGANIC CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Recent Development of Oxygen Evolution Electrocatalysts in Acidic Environment

Li An et al.

Summary: The review focuses on understanding the oxygen evolution reaction (OER) mechanisms in acid, analyzing strategies to enhance activity and stability, and summarizing state-of-the-art catalysts for OER. Prevailing OER mechanisms are reviewed for designing efficient electrocatalysts, approaches to improve activity are discussed, and factors affecting catalyst stability are analyzed. Noble-metal-based OER catalysts and non-noble-metal-based catalysts progress are reviewed, and challenges and perspectives for developing active and robust OER catalysts in acid are discussed.

ADVANCED MATERIALS (2021)

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Article Chemistry, Physical

High-valent bimetal Ni3S2/Co3S4 induced by Cu doping for bifunctional electrocatalytic water splitting

Hui Su et al.

Summary: Novel bimetallic sulfide electrocatalysts with excellent HER and OER activity have been synthesized, outperforming most reported bifunctional metal sulfides. This is attributed to the introduction of Cu cation promoting the formation of high-valent Ni/Co sites, which enhances the intrinsic catalytic activity by modulating the d-band center of Co and reducing the adsorption energy of intermediates.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Engineering, Environmental

Regulating the electronic structure of ultrathin Ni-based chalcogenide nanosheets through iron modification towards high electrocatalytic activities

Zhiyu Shao et al.

Summary: In this study, Fe2O3/NiSe2 and Fe2O3/Ni3S2 heterostructures with abundant anion defects were successfully constructed, showing outstanding electrocatalytic activities by reducing the energy barrier of intermediates. The integration of interface engineering and anion defects significantly improved the catalytic performances of the Fe2O3-modified NiSe2 and Ni3S2 catalysts.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Ni(OH)2 Templated Synthesis of Ultrathin Ni3S2 Nanosheets as Bifunctional Electrocatalyst for Overall Water Splitting

Chunqiao Jin et al.

Summary: In this study, cobalt-doped Ni3S2 ultrathin nanosheets were successfully synthesized using a simple topochemical conversion strategy, demonstrating excellent electrocatalytic activity. A universal strategy for synthesizing ultrathin nanosheets of nonlayered materials was proposed.

SMALL (2021)

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Article Chemistry, Physical

Ultrafine Nickel Nanoparticles Encapsulated in N-Doped Carbon Promoting Hydrogen Oxidation Reaction in Alkaline Media

Jie Wang et al.

Summary: In this study, a highly efficient Ni-based catalyst for HOR in alkaline electrolyte was reported, showing excellent activity and superior stability. Theoretical calculations revealed that the d-band state of Ni encapsulated in ultrathin N-doped carbon shell is downshifted, leading to a low limiting energy pathway for HOR.

ACS CATALYSIS (2021)

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Article Chemistry, Applied

Highly active sites of NiVB nanoparticles dispersed onto graphene nanosheets towards efficient and pH-universal overall water splitting

Muhammad Arif et al.

Summary: The study developed high-performance non-noble metal electrocatalysts for pH-universal water splitting with low overpotential. The catalyst demonstrated excellent electrocatalytic performance in various pH conditions, showing promising potential for efficient water splitting.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Transition Metal-Based 2D Layered Double Hydroxide Nanosheets: Design Strategies and Applications in Oxygen Evolution Reaction

Birhanu Bayissa Gicha et al.

Summary: Layered double hydroxides (LDHs) with 2D structures show great potential in electrocatalysis due to their ease of preparation and structural flexibility, but their application is limited by stacking structures and low activity. Strategies are being developed to adjust their morphological and electronic structure to enhance their performance in catalysis.

NANOMATERIALS (2021)

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Article Chemistry, Physical

Amorphous Ni1-xFex Oxyhydroxide Nanosheets with Integrated Bulk and Surface Iron for a High and Stable Oxygen Evolution Reaction

Birhanu Bayissa Gicha et al.

Summary: Amorphous Ni1-xFex oxyhydroxide nanosheets were synthesized by facile electrodeposition, showing high activity and stability for the oxygen evolution reaction (OER). The integrated bulk and surface Fe in the nanosheets demonstrated synergistic effects, enhancing OER activity and stability, potentially enabling the generation of cheap and clean hydrogen energy.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Perspective on intermetallics towards efficient electrocatalytic water-splitting

Carsten Walter et al.

Summary: Intermetallic compounds show attractive electronic, physical, and chemical properties, making them ideal materials for electrocatalytic applications. However, their widespread use is often hindered by complex and energy-intensive processes, leading to larger particles and decreased surface areas. Alternative synthetic strategies are being explored to achieve high performance and stable electrode materials.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Heterojunction-induced nickel-based oxygen vacancies on N-enriched porous carbons for enhanced alkaline hydrogen oxidation and oxygen reduction

Jin-Tao Ren et al.

Summary: The study successfully prepared a Ni/NiO/N-doped porous carbon catalyst, which can effectively improve the activity and durability of hydrogen oxidation and oxygen reduction reactions in alkaline electrolyte, making it a promising electrode catalyst for hydroxide exchange membrane fuel cells.

MATERIALS CHEMISTRY FRONTIERS (2021)

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Article Chemistry, Physical

Alloy-strain-output induced lattice dislocation in Ni3FeN/Ni3Fe ultrathin nanosheets for highly efficient overall water splitting

Zijian Li et al.

Summary: The study develops Ni3FeN/Ni3Fe electrocatalysts through lattice defect engineering, showing excellent performance for the OER and HER in alkaline media. This approach provides a new strategy for high-performance water splitting.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Review Chemistry, Physical

A vast exploration of improvising synthetic strategies for enhancing the OER kinetics of LDH structures: a review

Arun Karmakar et al.

Summary: This article explores the advantages and challenges of layered double hydroxide (LDH) materials in the field of oxygen evolution reaction, discussing various strategies to overcome the inherent drawbacks of LDHs.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

2D MOF-derived porous NiCoSe nanosheet arrays on Ni foam for overall water splitting

Yue Zhou et al.

Summary: The study presents a general strategy for the rational design and synthesis of multifunctional 2D porous electrocatalysts, demonstrating excellent electrochemical activity and long-term stability in overall water splitting applications. The porous NiCoSe nanosheet arrays show low overpotential for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER), making them promising candidates for future renewable energy systems.

CRYSTENGCOMM (2021)

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Review Electrochemistry

Understanding the Mechanism of the Oxygen Evolution Reaction with Consideration of Spin

Xiaoning Li et al.

Summary: This article discusses the electron behavior during the oxygen evolution reaction (OER) by considering the spin attribute, highlighting the high requirements on the spin structure of electrocatalysts. Understanding the coupling between spin, charge, orbital, and lattice parameters is necessary for optimizing geometric and electronic structures in transition metal systems. It also explores the potential dependency of OER efficiency on the electrocatalyst spin configuration and the relevance of factors like crystal field, coordination, oxidation, bonding, electron number, conductivity, and magnetism with spin.

ELECTROCHEMICAL ENERGY REVIEWS (2021)

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Review Chemistry, Multidisciplinary

Advance in Using Plasma Technology for Modification or Fabrication of Carbon-Based Materials and Their Applications in Environmental, Material, and Energy Fields

Xin Sun et al.

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Boronization-Induced Ultrathin 2D Nanosheets with Abundant Crystalline-Amorphous Phase Boundary Supported on Nickel Foam toward Efficient Water Splitting

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ADVANCED ENERGY MATERIALS (2020)

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Ultrathin Ni(0)-Embedded Ni(OH)2 Heterostructured Nanosheets with Enhanced Electrochemical Overall Water Splitting

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Fe-Based Electrocatalysts for Oxygen Evolution Reaction: Progress and Perspectives

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Earth-abundant transition-metal-based bifunctional catalysts for overall electrochemical water splitting: A review

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Fe-Doped Ni-Co Phosphide Nanoplates with Planar Defects as an Efficient Bifunctional Electrocatalyst for Overall Water Splitting

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Single Ni Atoms and Clusters Embedded in N-Doped Carbon Tubes on Fibers Matrix with Bifunctional Activity for Water Splitting at High Current Densities

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Pt-Based Nanocrystal for Electrocatalytic Oxygen Reduction

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Synergistic coupling of CoFe-LDH arrays with NiFe-LDH nanosheet for highly efficient overall water splitting in alkaline media

Rong Yang et al.

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Fe-Ni Layered Double Hydroxide Arrays with Homogeneous Heterostructure as Efficient Electrocatalysts for Overall Water Splitting

Kuangfu Huang et al.

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Template-free synthesis of three-dimensional NiFe-LDH hollow microsphere with enhanced OER performance in alkaline media

Haihong Zhong et al.

JOURNAL OF ENERGY CHEMISTRY (2019)

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Fabrication of NiFe layered double hydroxide with well-defined laminar superstructure as highly efficient oxygen evolution electrocatalysts

Hao Zhang et al.

NANO RESEARCH (2019)

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Controlled Self-Assembled NiFe Layered Double Hydroxides/Reduced Graphene Oxide Nanohybrids Based on the Solid-Phase Exfoliation Strategy as an Excellent Electrocatalyst for the Oxygen Evolution Reaction

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NiFe-based nanostructures on nickel foam as highly efficiently electrocatalysts for oxygen and hydrogen evolution reactions

Wei Zhang et al.

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Recent advances in layered double hydroxide electrocatalysts for the oxygen evolution reaction

Zhengyang Cai et al.

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Ar Plasma-Exfoliated Ultrathin NiCo-Layered Double Hydroxide Nanosheets for Enhanced Oxygen Evolution

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Engineering borate modified NiFe layer double hydroxide nanoarrays as hydroxyl ions hungry electrocatalysts for enhanced oxygen evolution

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Metal-organic framework-derived hierarchical MoS2/CoS2 nanotube arrays as pH-universal electrocatalysts for efficient hydrogen evolution

Baoshan Tang et al.

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Single Ru atoms with precise coordination on a monolayer layered double hydroxide for efficient electrooxidation catalysis

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Recent progress made in the mechanism comprehension and design of electrocatalysts for alkaline water splitting

Congling Hu et al.

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Electrodeposition of Ni-Co-Fe mixed sulfide ultrathin nanosheets on Ni nanocones: a low-cost, durable and high performance catalyst for electrochemical water splitting

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Mesoporous Nanocast Electrocatalysts for Oxygen Reduction and Oxygen Evolution Reactions

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Interface engineering: few-layer MoS2 coupled to a NiCo-sulfide nanosheet heterostructure as a bifunctional electrocatalyst for overall water splitting

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Ce-Doped NiFe-Layered Double Hydroxide Ultrathin Nanosheets/Nanocarbon Hierarchical Nanocomposite as an Efficient Oxygen Evolution Catalyst

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Bifunctional Heterostructure Assembly of NiFe LDH Nanosheets on NiCoP Nanowires for Highly Efficient and Stable Overall Water Splitting

Haojie Zhang et al.

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S. Anantharaj et al.

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Facile assembly of Ni(OH)(2) nanosheets on nitrogen-doped carbon nanotubes network as high-performance electrocatalyst for oxygen evolution reaction

Jian Wu et al.

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Single-Atom Au/NiFe Layered Double Hydroxide Electrocatalyst: Probing the Origin of Activity for Oxygen Evolution Reaction

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