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Noncrystalline Carbon Anodes for Advanced Sodium-Ion Storage

SMALL METHODS (2023)

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Summary: In this study, oxygen-doped vertically aligned carbon aerogels (VCAs) with hierarchically tailored channels were synthesized as anodes in sodium-ion batteries (SIBs) and potassium-ion batteries (PIBs) using a controllable unidirectional ice-templating technique. The VCAs exhibited excellent cycling performance and storage capacity, making them promising candidates for energy storage applications.

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Summary: By studying the microstructure of hard carbon materials, it is found that sodium storage capacities in the low potential plateau region involve contributions from both interlayer intercalation and micropores filling, with the ratio depending on the microstructure. The dominance of interlayer intercalation and micropores filling processes in the low potential plateau region can be distinguished by the potential inflection point at the end of the discharge curve. A microstructure-dependent mechanism is proposed to explain the sodium storage behaviors in different hard carbon materials.

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Combining Experimental and Theoretical Techniques to Gain an Atomic Level Understanding of the Defect Binding Mechanism in Hard Carbon Anodes for Sodium Ion Batteries

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Effect of Different Nitrogen Configurations on Sodium Storage Properties of Carbon Anodes for Sodium Ion Batteries

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Influence of Pore Architecture and Chemical Structure on the Sodium Storage in Nitrogen-Doped Hard Carbons

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Summary: Hard carbon as an anode material for sodium-ion batteries has a different sodium-storage mechanism compared to graphite, where it operates through the intercalation of Na+ into the graphitic layers to form sodium-graphite intercalation compounds. This insight may help in designing better HC materials for high-energy density SIBs.

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