4.8 Article

An anomalous Hall effect in altermagnetic ruthenium dioxide

期刊

NATURE ELECTRONICS
卷 5, 期 11, 页码 735-+

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NATURE PORTFOLIO
DOI: 10.1038/s41928-022-00866-z

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资金

  1. National Natural Science Foundation of China (NSFC) [52271235, 52121001]
  2. NSFC on the Science Foundation Ireland (SFI)-NSFC Partnership Programme (NSFC) [51861135104]
  3. Ministry of Education of the Czech Republic [LM2018110]
  4. Grant Agency of the Czech Republic [19-28375X]
  5. EU FET Open RIA grant [766566]
  6. LNSM-LNSpin
  7. National Grid Infrastructure MetaCentrum [CESNET LM2015042]
  8. Alexander von Humboldt Foundation
  9. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [TRR 173-268565370]

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This study reports an anomalous Hall effect in collinear altermagnetic ruthenium dioxide, with an anomalous Hall conductivity exceeding 1,000 omega(-1) cm(-1). The phenomenon arises from an alternative magnetic phase in RuO2, characterized by alternating spin polarization in both real-space crystal structure and momentum-space band structure. The results could potentially lead to the exploration of topological Berry phases and dissipationless quantum transport in crystals of abundant elements and with a compensated antiparallel magnetic order.
The anomalous Hall effect is a time-reversal symmetry-breaking magneto-electronic phenomenon originally discovered in ferromagnets. Recently, ruthenium dioxide (RuO2) with a compensated antiparallel magnetic order has been predicted to generate an anomalous Hall effect of comparable strength to ferromagnets. The phenomenon arises from an altermagnetic phase of RuO2 with a characteristic alternating spin polarization in both real-space crystal structure and momentum-space band structure. Here we report an anomalous Hall effect in RuO2 with an anomalous Hall conductivity exceeding 1,000 omega(-1) cm(-1). We combine the vector magnetometry and magneto-transport measurements of epitaxial RuO2 films of different crystallographic orientations. We show that the anomalous Hall effect dominates over an ordinary Hall contribution, and a contribution due to a weak field-induced magnetization. Our results could lead to the exploration of topological Berry phases and dissipationless quantum transport in crystals of abundant elements and with a compensated antiparallel magnetic order. By combining vector magnetometry and magneto-transport measurements of epitaxial films with different crystallographic orientations, an anomalous Hall effect can be measured in collinear altermagnetic ruthenium dioxide with an anomalous Hall conductivity exceeding 1,000 omega(-1) cm(-1).

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