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Research Progress on the Preparation and Action Mechanism of Natural Deep Eutectic Solvents and Their Application in Food

FOODS (2022)

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Article Chemistry, Applied

Analysis of the influencing mechanism of the freeze-thawing cycles on in vitro chicken meat digestion based on protein structural changes

Xue Bai et al.

Summary: This study investigated the impact of freeze-thaw cycles on the digestive and protein structural properties of chicken breasts during in vitro digestion. The results showed that with an increase in freeze-thaw cycles, the hardness, chewiness, and shear force of chicken breasts increased, while digestibility decreased and particle size increased. The study also confirmed that freeze-thaw cycles led to the disruption of protein structure and induced protein aggregation.

FOOD CHEMISTRY (2023)

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Article Food Science & Technology

Mechanisms of Change in Emulsifying Capacity Induced by Protein Denaturation and Aggregation in Quick-Frozen Pork Patties with Different Fat Levels and Freeze-Thaw Cycles

Nan Pan et al.

Summary: In this study, it was found that protein denaturation and aggregation caused by multiple freeze-thaw cycles and fat levels altered the distribution of surface chemical groups and particle sizes of protein, thereby affecting the emulsifying properties.

FOODS (2022)

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Article Chemistry, Applied

Development of natural deep eutectic solvents (NADESs) as anti-freezing agents for the frozen food industry: Water-tailoring effects, anti-freezing mechanisms and applications

You Tian et al.

Summary: The study investigated the properties of nature-inspired natural deep eutectic solvents (NADESs) as anti-freezing agents, finding them to possess excellent anti-freezing capacity, with Pro:Sor (1:1) showing the greatest temperature sensitivity and best anti-frosting capacity. Applications in frozen chicken breast further demonstrated the potentials of NADESs as antifreezing agents for the industry.

FOOD CHEMISTRY (2022)

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Article Food Science & Technology

Greener extraction of anthocyanins and antioxidant activity from blackberry (Rubus spp) using natural deep eutectic solvents

Oscar Zannou et al.

Summary: This study investigates an efficient and greener strategy for extracting blackberry anthocyanins using natural deep eutectic solvents (NaDESs). Sixteen different NaDESs were synthesized and compared with conventional solvents. The results showed that NaDESs exhibited superior extraction properties for antioxidants and anthocyanins in blackberry. This research provides a promising approach for future investigations on phytochemicals in plants.

LWT-FOOD SCIENCE AND TECHNOLOGY (2022)

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Review Food Science & Technology

Research progress on quality deterioration mechanism and control technology of frozen muscle foods

Xin Du et al.

Summary: This review examines the deterioration characteristics and mechanisms of frozen muscle foods, as well as novel freezing technologies and bioactive antifreeze substances. It also reviews thawing technologies to address the loss of water and nutrients. The review concludes that physical damage caused by ice crystals is the primary reason for eating quality deterioration, and these novel techniques and substances can enhance the eating quality of frozen muscle foods.

COMPREHENSIVE REVIEWS IN FOOD SCIENCE AND FOOD SAFETY (2022)

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Article Biotechnology & Applied Microbiology

Microwave-assisted deep eutectic solvent extraction of phenolic compounds from brewer's spent grain

Juan C. Lopez-Linares et al.

Summary: The study demonstrates the effectiveness of using deep eutectic solvents and microwave assistance for the extraction of phenolic compounds from brewer's spent grain. It shows that the process can recover phenolic compounds and produce residual extracted solids with undisturbed structural carbohydrates, suitable for use in biorefinery applications.

JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY (2021)

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Article Agricultural Engineering

Comprehensive analysis of important parameters of choline chloride-based deep eutectic solvent pretreatment of lignocellulosic biomass

Huanfei Xu et al.

Summary: Choline chloride based deep eutectic solvents have great potential in lignocellulosic biomass pretreatment. Multivariate analysis methods were used to reveal the pretreatment mechanism and found that properties of hydrogen bond donnors and severity of DES had significant influence on the pretreatment effect. Molecular simulation and four-dimensional color graphs were utilized for further optimization of pretreatment conditions to improve economic benefits and energy consumption indicators.

BIORESOURCE TECHNOLOGY (2021)

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Review Chemistry, Multidisciplinary

Deep Eutectic Solvents: A Review of Fundamentals and Applications

Benworth B. Hansen et al.

Summary: Deep eutectic solvents (DESs) exhibit significant depressions in melting points and tunable physicochemical properties, but there is still a lack of predictive understanding of their microscopic mechanisms and structure-property relationships. Research on complex hydrogen bonding is crucial for a deeper understanding and development of fundamental frameworks for DESs.

CHEMICAL REVIEWS (2021)

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Article Agriculture, Multidisciplinary

Green and efficient removal of heavy metals from Porphyra haitanensis using natural deep eutectic solvents

Xi Yang et al.

Summary: This study investigated the use of 28 kinds of NADESs as eluents for heavy metal removal from Porphyra haitanensis, achieving removal rates ranging from 17.4% to 100%. The optimal condition included 10% water content and a solid-liquid ratio of 1:20, with the addition of 20% natural surfactant arabic gum further enhancing heavy metal removal rates. Adsorption mechanism experiments revealed that the pseudo second-order model and Freundlich adsorption model can better explain the adsorption mechanism of NADESs on heavy metals removal.

JOURNAL OF THE SCIENCE OF FOOD AND AGRICULTURE (2021)

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Article Chemistry, Applied

Tracking aggregation behaviour and gel properties induced by structural alterations in myofibrillar protein in mirror carp (Cyprinus carpio) under the synergistic effects of pH and heating

Xin Du et al.

Summary: The synergistic effect of pH and heating on myofibrillar protein in mirror carp was found to impact the protein's structure, aggregation behavior, and gel properties. Adjusting pH and temperature could modulate the three-dimensional network structure and gel properties of the protein.

FOOD CHEMISTRY (2021)

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Article Chemistry, Applied

Sonication-synergistic natural deep eutectic solvent as a green and efficient approach for extraction of phenolic compounds from peels of Carya cathayensis Sarg

Xizhe Fu et al.

Summary: Combining natural deep eutectic solvent with pulse-ultrasonication technique demonstrated significant synergistic effect and high efficiency in extracting phenolic compounds from Carya cathayensis Sarg. peels. The development and validation of a second-order kinetic model further confirmed the synergistic effect and influence during extraction.

FOOD CHEMISTRY (2021)

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Article Food Science & Technology

Effect of freeze-thaw cycles on the quality of quick-frozen pork patty with different fat content by consumer assessment and instrument-based detection

Nan Pan et al.

Summary: The study evaluated the quality changes of quick-frozen patties with different fat contents and freeze-thaw cycles, showing that repeated freeze-thaw cycles accelerated the deterioration of patty quality and rendered them unacceptable after 3 cycles.

MEAT SCIENCE (2021)

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Article Biochemistry & Molecular Biology

Ultrasound-Assisted Extraction of Anthocyanins Using Natural Deep Eutectic Solvents and Their Incorporation in Edible Films

Patricia Velasquez et al.

Summary: The study focused on developing active edible films with antioxidant and antibacterial capabilities by extracting anthocyanins from Chilean Luma chequen berries using specially designed natural deep eutectic solvents (NADES), and incorporating them into the film matrix. The research demonstrated that ultrasound-assisted extraction is effective in extracting anthocyanins with high antioxidant and antibacterial activities in the extracts.

MOLECULES (2021)

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Article Biology

Natural deep eutectic systems, an emerging class of cryoprotectant agents

Ana Rita Jesus et al.

Summary: The study demonstrated the high potential of using NADES as cryoprotectant agents, showing low cytotoxicity and good post-thaw recovery without the need for removing NADES from the freezing media.

CRYOBIOLOGY (2021)

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Article Chemistry, Physical

Aliphatic amino acids as possible hydrogen bond donors for preparing eutectic solvents

Farouq S. Mjalli et al.

Summary: Deep eutectic solvents have been competing with ionic liquids due to their lower production cost, simple synthesis, and favorable biodegradability. In this study, a group of four aliphatic-type amino acids were successfully coupled with tetrabutylammonium chloride to form new eutectic solvents at different molar compositions, which were characterized in terms of their phase-change behavior and physicochemical properties within a specific temperature range. The relationship between various properties and temperature was investigated, showing different trends for density, surface tension, refractive index, pH, viscosity, and conductivity.

JOURNAL OF MOLECULAR LIQUIDS (2021)

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Review Plant Sciences

Natural Deep Eutectic Solvents (NADES): Phytochemical Extraction Performance Enhancer for Pharmaceutical and Nutraceutical Product Development

Ni Putu Ermi Hikmawanti et al.

Summary: The selection of extracting solvent is crucial for the extraction of natural products from plants. The pharmacological properties of plant extracts are related to their solubility, stability, and bioavailability. Deep eutectic solvents have the potential to improve the extraction performance of plant metabolites and can be used in pharmaceutical formulations development.

PLANTS-BASEL (2021)

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Article Acoustics

Recovery of β-carotene from pumpkin using switchable natural deep eutectic solvents

Alena Stupar et al.

Summary: The study developed a green and sustainable extraction procedure for beta-carotene recovery from pumpkin using NADES solvents and ultrasound assisted extraction, resulting in high extraction efficiency and stability. The extracted carotenoids showed high stability over a 180-day storing period.

ULTRASONICS SONOCHEMISTRY (2021)

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Article Food Science & Technology

Physical Properties of Chitosan Films Containing Pomegranate Peel Extracts Obtained by Deep Eutectic Solvents

Aikaterini Kyriakidou et al.

Summary: This study investigated the incorporation of pomegranate peel extract in chitosan films using green deep eutectic solvents as extraction solvents. The optimized extraction process yielded high amounts of total polyphenols and flavonoids, and the addition of the extract affected the properties of the chitosan films.

FOODS (2021)

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Article Chemistry, Analytical

Vortex-assisted natural deep eutectic solvent dispersive liquid-liquid microextraction based on the solidification of a floating organic drop for the determination of benzoic acid and sorbic acid in condiments

Xiaoming Zhu et al.

Summary: A simple, inexpensive, reliable and environmentally friendly method based on vortex-assisted dispersive liquid-liquid microextraction combined with solidification of a floating organic drop (VA-DLLME-SFO) followed by high performance liquid chromatography with a diode array detector (HPLC-DAD) was developed to determine benzoic acid (BA) and sorbic acid (SA) in ketchup and powder bags of instant noodles. The method showed good linearity, low detection limits and accurate recoveries, making it a reliable approach for the analysis of chemical compounds in food samples.

ANALYTICAL METHODS (2021)

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Article Chemistry, Multidisciplinary

Effect of deep eutectic solvent's characteristics on extraction and bioactivity of polyphenols fromSapodillapulp

Suman Kumar Saha et al.

Summary: In this study, a sustainable and efficient deep eutectic solvent-based ultrasound-assisted extraction method for Sapodilla pulp polyphenols was developed. Low pH and high polarity in acid-based DESs significantly enhanced the recovery of polyphenols. Oxalic acid DES showed the highest yield due to the presence of three OH groups, which retarded the interaction between DES and target compounds.

CHEMICAL PAPERS (2021)

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Review Food Science & Technology

The perspectives of natural deep eutectic solvents in agri-food sector

Aleksandra Mrsan et al.

CRITICAL REVIEWS IN FOOD SCIENCE AND NUTRITION (2020)

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Review Food Science & Technology

Naturally sourced biosubstances for regulating freezing points in food researches: Fundamentals, current applications and future trends

You Tian et al.

TRENDS IN FOOD SCIENCE & TECHNOLOGY (2020)

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Article Agriculture, Multidisciplinary

Quantitative Determination of Thiamine-Derived Taste Enhancers in Aqueous Model Systems, Natural Deep Eutectic Solvents, and Thermally Processed Foods

Laura Brehm et al.

JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY (2020)

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Article Chemistry, Physical

NADES as potential solvents for anthocyanin and pectin extraction from Myrciaria cauliflora fruit by-product: In silico and experimental approaches for solvent selection

Lais Benvenutti et al.

JOURNAL OF MOLECULAR LIQUIDS (2020)

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Article Food Science & Technology

Formulation of choline chloride/ascorbic acid natural deep eutectic solvent: Characterization, solubilization capacity and antioxidant property

Jordy Kim Ung Ling et al.

LWT-FOOD SCIENCE AND TECHNOLOGY (2020)

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Review Food Science & Technology

Developments of mathematical models for simulating vacuum cooling processes for food products - a review

Zhiwei Zhu et al.

CRITICAL REVIEWS IN FOOD SCIENCE AND NUTRITION (2019)

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Article Biotechnology & Applied Microbiology

Physicochemical Properties, Cytotoxicity, and Antioxidative Activity of Natural Deep Eutectic Solvents Containing Organic Acid

A. Mitar et al.

CHEMICAL AND BIOCHEMICAL ENGINEERING QUARTERLY (2019)

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Article Thermodynamics

Influence of temperature, water content and type of organic acid on the formation, stability and properties of functional natural deep eutectic solvents

Lizandra Kamradt Savi et al.

FLUID PHASE EQUILIBRIA (2019)

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Article Chemistry, Physical

Sustainable synthesis of natural deep eutectic solvents (NADES) by different methods

Ana Pr Santana et al.

JOURNAL OF MOLECULAR LIQUIDS (2019)

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Article Food Science & Technology

Microwave-assisted extraction of soluble sugars from banana puree with natural deep eutectic solvents (NADES)

Analia Veronica Gomez et al.

LWT-FOOD SCIENCE AND TECHNOLOGY (2019)

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Article Chemistry, Multidisciplinary

Natural Deep Eutectic Solvents as Agents for Improving Solubility, Stability and Delivery of Curcumin

Tomasz Jelinski et al.

PHARMACEUTICAL RESEARCH (2019)

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Article Agricultural Engineering

Enhanced extraction of natural pigments from Curcuma longa L. using natural deep eutectic solvents

Yanhong Liu et al.

INDUSTRIAL CROPS AND PRODUCTS (2019)

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Article Agriculture, Multidisciplinary

Multiple Hydrogen-Bonding Interactions Enhance the Solubility of Starch in Natural Deep Eutectic Solvents: Molecule and Macroscopic Scale Insights

Chen Cao et al.

JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY (2019)

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Article Chemistry, Applied

Enabling technologies for the extraction of grape-pomace anthocyanins using natural deep eutectic solvents in up-to-half-litre batches extraction of grape-pomace anthocyanins using NADES

Manuela Panic et al.

FOOD CHEMISTRY (2019)

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Article Biotechnology & Applied Microbiology

Effects of natural deep eutectic solvents on lactic acid bacteria viability during cryopreservation

Ying Qiao et al.

APPLIED MICROBIOLOGY AND BIOTECHNOLOGY (2018)

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Article Biology

Natural deep eutectic systems as alternative nontoxic cryoprotective agents

Vania I. B. Castro et al.

CRYOBIOLOGY (2018)

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Article Chemistry, Applied

Green and efficient removal of cadmium from rice flour using natural deep eutectic solvents

Yao Huang et al.

FOOD CHEMISTRY (2018)

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Article Chemistry, Applied

Novel approaches mediated by tailor-made green solvents for the extraction of phenolic compounds from agro-food industrial by-products

Maria de los Angeles Fernandez et al.

FOOD CHEMISTRY (2018)

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Article Chemistry, Applied

Natural deep eutectic solvents as green plasticizers for chitosan thermoplastic production with controlled/desired mechanical and barrier properties

Andrea C. Galvis-Sanchez et al.

FOOD HYDROCOLLOIDS (2018)

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Article Chemistry, Physical

Gas solubility and rheological behavior study of betaine and alanine based natural deep eutectic solvents (NADES)

Tausif Altamash et al.

JOURNAL OF MOLECULAR LIQUIDS (2018)

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Review Plant Sciences

Natural Deep Eutectic Solvents: Properties, Applications, and Perspectives

Yang Liu et al.

JOURNAL OF NATURAL PRODUCTS (2018)

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Article Biochemistry & Molecular Biology

Food-Grade Synthesis of Maillard-Type Taste Enhancers Using Natural Deep Eutectic Solvents (NADES)

Maximilian Kranz et al.

MOLECULES (2018)

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Article Engineering, Chemical

Extraction of polyphenolic antioxidants from orange peel waste using deep eutectic solvents

Baranse Ozturk et al.

SEPARATION AND PURIFICATION TECHNOLOGY (2018)

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Article Chemistry, Multidisciplinary

A Greener Approach to Prepare Natural Deep Eutectic Solvents

Federico J. V. Gomez et al.

CHEMISTRYSELECT (2018)

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Article Chemistry, Applied

A functional natural deep eutectic solvent based on trehalose: Structural and physicochemical properties

Ruipu Xin et al.

FOOD CHEMISTRY (2017)

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Article Chemistry, Physical

Natural deep eutectic solvents from choline chloride and betaine - Physicochemical properties

Ivo M. Aroso et al.

JOURNAL OF MOLECULAR LIQUIDS (2017)

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Article Biochemistry & Molecular Biology

Deep Eutectic Solvents as Novel and Effective Extraction Media for Quantitative Determination of Ochratoxin A in Wheat and Derived Products

Luca Piemontese et al.

MOLECULES (2017)

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Article Chemistry, Analytical

Deep eutectic solvent-based dispersive liquid-liquid microextraction

Mir Ali Farajzadeh et al.

ANALYTICAL METHODS (2016)

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Article Engineering, Environmental

Ammonium-based deep eutectic solvents as novel soil washing agent for lead removal

Soumyadeep Mukhopadhyay et al.

CHEMICAL ENGINEERING JOURNAL (2016)

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Article Chemistry, Physical

Properties and thermal behavior of natural deep eutectic solvents

R. Craveiro et al.

JOURNAL OF MOLECULAR LIQUIDS (2016)

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Article Chemistry, Physical

Deep eutectic solvent based ultrasonic assisted liquid phase microextraction for the FAAS determination of cobalt

Muhammad Balal Arain et al.

JOURNAL OF MOLECULAR LIQUIDS (2016)

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Review Chemistry, Analytical

Natural designer solvents for greening analytical chemistry

Magdalena Espino et al.

TRAC-TRENDS IN ANALYTICAL CHEMISTRY (2016)

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Article Environmental Sciences

Assessing the toxicity and biodegradability of deep eutectic solvents

Qing Wen et al.

CHEMOSPHERE (2015)

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Article Environmental Sciences

Evaluation of toxicity and biodegradability of choline chloride based deep eutectic solvents

Kristina Radosevic et al.

ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY (2015)

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Article Chemistry, Applied

Tailoring properties of natural deep eutectic solvents with water to facilitate their applications

Yuntao Dai et al.

FOOD CHEMISTRY (2015)

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Article Chemistry, Analytical

Deep eutectic liquid organic salt as a new solvent for liquid-phase microextraction and its application in ligandless extraction and pre-concentraion of lead and cadmium in edible oils

Mehdi Karimi et al.

TALANTA (2015)

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Article Chemistry, Multidisciplinary

Biocompatible Deep Eutectic Solvents Based on Choline Chloride: Characterization and Application to the Extraction of Rutin from Sophora japonica

Bing-Yi Zhao et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2015)

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Article Chemistry, Applied

Natural deep eutectic solvents providing enhanced stability of natural colorants from safflower (Carthamus tinctorius)

Yuntao Dai et al.

FOOD CHEMISTRY (2014)

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Review Chemistry, Multidisciplinary

Natural Deep Eutectic Solvents - Solvents for the 21st Century

Alexandre Paiva et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2014)

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Article Chemistry, Multidisciplinary

Insights into the Synthesis and Properties of Deep Eutectic Solvents Based on Cholinium Chloride and Carboxylic Acids

C. Florindo et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2014)

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Article Chemistry, Analytical

Natural deep eutectic solvents as new potential media for green technology

Yuntao Dai et al.

ANALYTICA CHIMICA ACTA (2013)

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Article Plant Sciences

Are Natural Deep Eutectic Solvents the Missing Link in Understanding Cellular Metabolism and Physiology?

Young Hae Choi et al.

PLANT PHYSIOLOGY (2011)

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Article Chemistry, Multidisciplinary

Freeze-Drying of Aqueous Solutions of Deep Eutectic Solvents: A Suitable Approach to Deep Eutectic Suspensions of Self-Assembled Structures

Maria C. Gutierrez et al.

LANGMUIR (2009)

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