☆ 4.6 Review

Development and prospects of garnet ceramic scintillators: A review

JOURNAL OF ADVANCED CERAMICS (2022)

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Summary: LuAG:Ce ceramic scintillators have great potential in high-energy physics due to their low cost, bright light, and fast decay time. This study investigates the optical and scintillation performance of LuAG:Ce ceramic samples co-doped with Mg2+ and Ca2+, as well as their radiation damage induced by neutrons and protons. The results show that LuAG:Ce ceramic samples have excellent radiation hardness and lower radiation damage compared to LYSO:Ce crystals.

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Article Optics

Influence of matrix composition and its fluctuations on excitation relaxation and emission spectrum of Ce ions in (Gdx Y1-x)3Al2Ga3O12: Ce scintillators

S. Nargelas et al.

Summary: Cerium-doped mixed garnet-type single crystals with varying yttrium content were studied to optimize scintillation properties by adjusting the matrix composition. Analysis of optical absorption and photoluminescence spectroscopy revealed a composite origin of Ce3+ emission band, with Ce3+ ions located in different positions due to compositional fluctuations in the mixed crystal lattice.

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Article Chemistry, Applied

Fabrication and long persistent luminescence of Ce3+-Cr3+co-doped yttrium aluminum gallium garnet transparent ceramics

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Summary: In this study, Ce3+-doped transparent ceramics were successfully prepared and the effects of Ce3+ concentration and annealing atmospheres on their performance were investigated.

JOURNAL OF RARE EARTHS (2022)

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Towards effective indirect radioisotope energy converters with bright and radiation hard scintillators of (Gd,Y)3Al2Ga3O12 family

M. Korzhik et al.

Summary: Ceramics of quaternary garnets doped with Ce, Tb have been fabricated and evaluated as prospective materials for indirect energy converters. The samples showed good temperature stability and tolerance to irradiation, and the role of X-rays in increasing the conversion efficiency has been clarified.

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Ce3+-Doped Yttrium Aluminum Garnet Transparent Ceramics for High-Resolution X-Ray Imaging

Tao Ji et al.

Summary: This paper introduces a new type of TC scintillator material (YAG:Ce3+ TCs), which has high transmittance and steady-state light yield, and can achieve excellent X-ray imaging performance. Due to its structural stability, it can work stably under long-term X-ray irradiation, providing new opportunities for the development of high-quality X-ray imaging.

ADVANCED OPTICAL MATERIALS (2022)

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Seed-Crystal-Induced Cold Sintering Toward Metal Halide Transparent Ceramic Scintillators

Kai Han et al.

Summary: This study presents a novel cold sintering technique to fabricate transparent TPP2MnBr4 ceramic wafers with high optical transparency and exceptional scintillation performance, enabling high spatial resolution X-ray medical imaging.

ADVANCED MATERIALS (2022)

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Mixed precipitants derived nanocrystalline powders and RE doped LuAG transparent ceramics

Ding Zhou et al.

Summary: LuAG nanocrystalline powders were synthesized using ammonium hydroxide and ammonium hydrogen carbonate as mixed precipitant. The obtained LuAG powders showed good sinterability and high optical quality when sintered at low temperature in H-2 atmosphere by PLSH technology. Transparent ceramics doped with various rare earth ions could be prepared without sintering aids and HIP post-treatment.

CERAMICS INTERNATIONAL (2022)

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Ultrafast GGAG:Ce X-ray scintillation ceramics with Ca2+and Mg2+co-dopants

Xin Huang et al.

Summary: In this study, Gd3Ga3Al2O12:Ce scintillation ceramics codoped with Me2+ (Me = Mg, Ca) were fabricated. The co-doping with Ca2+ and Mg2+ showed a synergistic effect on accelerating the scintillation process and decreasing the light yield. Among the co-doped samples, GGAG:Ce co-doped with 0.1 at% Ca2+ and 0.1 at% Mg2+ exhibited the fastest decay time and a relatively high light yield.

CERAMICS INTERNATIONAL (2022)

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High-entropy transparent ceramics: Review of potential candidates and recently studied cases

Guangran Zhang et al.

Summary: High-entropy ceramics have been a recent focus of extensive research, with potential applications in various fields. Current studies mainly concentrate on the properties and fabrication methods of high-entropy ceramics.

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J. T. Jarrell et al.

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2022)

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(Gd,Ce)2O3-Al2O3-SiO2 scintillation glass

A. Amelina et al.

Summary: A heavy scintillation glass composed of Gd2O3-Al2O3-SiO2 doped with Ce, which combines high light yield and fast scintillation kinetics, has been developed. This material shows potential for use in large volume detectors, medical imaging, and other high energy physics applications due to its low-cost production capability.

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Fabrication and properties of non-stoichiometric Tb2(Hf1-xTbx)2O7-x magneto-optical ceramics

Lixuan Zhang et al.

Summary: Non-stoichiometric Tb-2(Hf1-xTbx)(2)O7-x ceramics were successfully fabricated and investigated for their phase composition, densification process, microstructure, optical transmittance, and Verdet constant. The results showed that the transmittance and Verdet constant of the ceramics increased with the increase of Tb content, and the Verdet constant was higher compared to the commercial Tb3Ga5O12 crystal, suggesting the great potential of non-stoichiometric Tb-2(Hf1-xTbx)(2)O7-x ceramics for Faraday isolator applications.

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Ce3+ doped Lu3Al5O12 ceramics prepared by spark plasma sintering technology using micrometre powders: Microstructure, luminescence, and scintillation properties

Yun Shi et al.

Summary: Ce3+ doped Lu3Al5O12 ceramics were successfully fabricated by SPS, and their properties such as grain size and photoluminescence were investigated. The results showed that the SPS ceramics had smaller grain size, excellent thermal stability, and higher radioluminescence intensity.

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Influence of calcium doping concentration on the performance of Ce,Ca: LuAG scintillation ceramics

Danyang Zhu et al.

Summary: Ce,Ca:LuAG scintillation ceramics with different Ca2+ co-doping concentrations were prepared, and the influence of Ca2+ concentration on optical quality was systematically studied. The results showed that good optical transmittance and high fast scintillation component can be obtained within a certain range of Ca2+ concentrations.

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY (2022)

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Scintillation properties of YAlO3:Ce perovskite co-doped by Mg2+ions

M. Kucera et al.

Summary: The effect of Mg2+ co-doping on the scintillation, luminescence, and optical properties of YAlO3:Ce perovskite was studied. Increasing Mg content accelerated the scintillation decays while reducing the light yield.

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Optical, luminescence and scintillation properties of Mg2+-codoped (Lu, Y)3Al2Ga3O12:Pr garnet crystals: The effect of Y admixture

Krittiya Sreebunpeng et al.

Summary: In this study, Mg-codoped Lu3-xYxAl2Ga3O12:Pr (x = 0, 1, 2, and 3) garnet crystals were grown by the micro-pulling down method, and their scintillation characteristics and temperature dependence of radioluminescence (RL) spectra were investigated. The LuY2Al2Ga3O12:Pr,Mg sample exhibited a high light yield and short scintillation decay time.

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Role of the Dilution of the Gd Sublattice in Forming the Scintillation Properties of Quaternary (Gd,Lu)3Al2Ga3O12: Ce Ceramics

Mikhail Korzhik et al.

Summary: By doping with super-stoichiometric gadolinium additive or co-doping with a low concentration of magnesium, phosphorescence in quaternary garnet can be effectively suppressed, confirming that it is not an intrinsic property of the material. Monte-Carlo simulation of electronic excitation transfer shows that hopping migration along the gadolinium sublattice plays a crucial role in forming the scintillation kinetic parameters. Substituting the integrity of the gadolinium sublattice with heavier lutetium ions increases the role of self-trapped states in the excitation of Ce3+ ions, ensuring an increase in the fraction of short (about 20 ns) and very long (about 600 ns) components in the scintillation kinetics.

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On fast LuAG:Ce scintillation ceramics with Ca2+ co-dopants

Wanqiu Ma et al.

Summary: The effects of Ca2+ co-doping on the scintillation properties of LuAG:Ce were investigated, showing significant improvement in scintillation performance. Especially the 0.2 at.% Ca2+ co-doped sample exhibited high light yield, fast scintillation decay time, and minimal slow component contamination. The role of Ca2+ in the scintillation mechanism of LuAG:Ce ceramics was also discussed in the study.

JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2021)

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Sintering parameter optimization of Tb3Al5O12 magneto-optical ceramics by vacuum sintering and HIP post-treatment

Xiaoying Li et al.

Summary: Transparent terbium aluminum garnet (TAG) ceramics were successfully prepared through vacuum sintering and HIP post-treating, showing that increasing sintering temperature can enhance optical quality. Additionally, the addition of sintering aid TEOS improves optical quality and inhibits valence state changes during annealing. The Verdet constant of the TAG ceramics at room temperature is significantly higher than that of commercial TGG crystals.

JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2021)

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Fabrication and properties of transparentmagneto-optical ceramics

Lixuan Zhang et al.

Summary: Transparent Tb2Ti2O7 magneto-optical ceramics were successfully fabricated using co-precipitated nano-powders and HIP post-treatment, showing excellent magneto-optical properties and promising applications in Faraday rotators.

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY (2021)

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Luminescence and scintillation properties of Mo co-doped Y0.8Gd2.2(Al5-xGax)O12: Ce multicomponent garnet crystals

Ongsa Sakthong et al.

Summary: Mo co-doped Y0.8Gd2.2(Al5-xGax)O12:Ce multicomponent garnet crystals were grown by the micro-pulling down method and their luminescence and scintillation properties were investigated. The temperature dependences of radioluminescence yield and photoluminescence decay time were measured to study the temperature stability of these crystals, with a decrease of radioluminescence yield at low temperature observed in correlation with the appearance of large thermoluminescence peaks.

OPTICAL MATERIALS (2021)

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Research progress of gadolinium aluminum garnet based optical materials

Guiyuan Liu et al.

Summary: Gadolinium aluminum garnet (GdAG) is a compound with cubic structure used as a matrix material in optics. This paper reviews recent findings in the directions of phosphors, scintillators, and solid-state lasers using GdAG and its derivatives. Challenges in synthesis and application of GdAG-based optical materials are discussed, along with proposed future development directions.

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Luminescence and scintillation properties of Gd3Sc2(Al3-xGax)O12:Ce (x=1, 2, 3) garnet crystals

Warut Chewpraditkul et al.

Summary: The luminescence and scintillation characteristics of Ce3+-doped Gd3Sc2(Al3-xGax)O-12 garnet crystals were studied, showing a blue shift in luminescence with increasing Ga content. The decrease in luminescence intensity and decay time at high temperature was observed for all samples, attributed to thermal ionization of Ce3+ and decrease of thermal activation energies with higher Ga content. Additionally, different samples exhibited comparable light yield values but with varying scintillation decay times.

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The scintillation mechanisms in Ce and Tb doped (GdxY1-x)Al2Ga3O12 quaternary garnet structure crystalline ceramics

M. Korzhik et al.

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Exciton interaction with Ce3+ and Ce4+ ions in (LuGd)3(Ga, Al)5O12 ceramics

Vasilii Khanin et al.

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JOURNAL OF LUMINESCENCE (2021)

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Xibin Wang et al.

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JOURNAL OF RARE EARTHS (2021)

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Yiheng Wu et al.

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JOURNAL OF THE EUROPEAN CERAMIC SOCIETY (2021)

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Efficient spectral regulation in Ce:Lu3(Al,Cr)5O12 and Ce:Lu3(Al,Cr)5O12/Ce:Y3Al5O12 transparent ceramics with high color rendering index for high-power white LEDs/LDs

Tianyuan Zhou et al.

Summary: Ce,Cr:LuAG TCs achieved efficient spectral regulation through Cr3+ doping, enhancing their luminescence properties in white LED/LD applications. By combining with other materials, such as 0.5 at% Ce:YAG TC, even better results were obtained in terms of CRI values for TC based white LEDs and LDs.

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Fine-grained Ce,Y:SrHfO3 Scintillation Ceramics Fabricated by Hot Isostatic Pressing

Zhu Danyang et al.

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Article Optics

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Fabrication of Ce:(Gd2Y)(Ga3Al2)O12 scintillator ceramic by oxygen-atmosphere sintering and hot isostatic pressing

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Effect of reducing Lu3+ content on the fabrication and scintillation properties of non-stoichiometric Lu3-xAl5O12:Ce ceramics

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Sintering of GGAG:Ce3+, xY3+ transparent ceramics in oxygen atmosphere

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CERAMICS INTERNATIONAL (2017)

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Luminescent and scintillation properties of Ce-doped Tb3Al5O12 crystal grown from Al-rich composition

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Large Size Czochralski Growth and Scintillation Properties of Mg2+ Co-doped Ce : Gd3Ga3Al2O12

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2016)

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Photostimulated luminescence and defects creation processes in Ce3+-doped epitaxial films of multicomponent Lu3-xGdxGayAl5-yO12 garnets

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Crystal growth and scintillation properties of multi-component oxide single crystals: Ce:GGAG and Ce:La-GPS

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Sintering and characterisation of Gd3Al3Ga2O12/Y3Al5O12 layered composite scintillation ceramic

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Optical and scintillation properties of Ce-doped (Gd2Y1)Ga2.7Al2.3O12 single crystal grown by Czochralski method

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Microstructure and optical properties of transparent Nd:GAGG ceramics prepared via solid-state reactive sintering

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Towards Bright and Fast Lu3Al5O12:Ce,Mg Optical Ceramics Scintillators

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Role of Y Admixture in (Lu1-xYx)3Al5O12: Pr Ceramic Scintillators Free of Host Luminescence

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Microstructure and optical characteristics of Ce:Gd-3(Ga,Al)(5)O-12 ceramic for scintillator application

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Flat Panel X-ray Imaging of LuAG:Ce,Mg Ceramic Scintillators

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Highly transparent ZrO2-doped (Ce,Gd)3Al3Ga2O12 ceramics prepared via oxygen sintering

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ESR and TSL study of hole and electron traps in LuAG:Ce,Mg ceramic scintillator

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OPTICAL MATERIALS (2015)

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Antisite defects in nonstoichiometric Lu3Al5O12:Ce ceramic scintillators

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Review Materials Science, Multidisciplinary

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Fabrication and Scintillation Performance of Nonstoichiometric LuAG:Ce Ceramics

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The Effects of Cation Concentration in the Salt Solution on the Cerium Doped Gadolinium Gallium Aluminum Oxide Nanopowders Prepared by a Co-precipitation Method

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Cz grown 2-in. size Ce:Gd3(Al,Ga)5O12 single crystal; relationship between Al, Ga site occupancy and scintillation properties

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High Energy Resolution Transparent Ceramic Garnet Scintillators

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Development of Transparent Ceramic Ce-Doped Gadolinium Garnet Gamma Spectrometers

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Homogeneity of Gd-based garnet transparent ceramic scintillators for gamma spectroscopy

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Effect of the Pr3+ → Gd3+ energy transfer in multicomponent garnet single crystal scintillators

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Gd3+ to Ce3+ energy transfer in multi-component GdLuAG and GdYAG garnet scintillators

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Luminescence and scintillation characteristics of Gd3Al2Ga3O12:Ce3+ scintillators

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Comparative study of ceramic and single crystal Ce:GAGG scintillator

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Review Crystallography

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Scintillation Properties of Transparent Ceramic Pr:LuAG for Different Pr Concentration

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2012)

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2 inch diameter single crystal growth and scintillation properties of Ce:Gd3Al2Ga3O12

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The Harmful Effects of Sintering Aids in Pr:LuAG Optical Ceramic Scintillator

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Transparent Garnet Ceramic Scintillators for Gamma-ray Detection

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Microstructure, optical, and scintillation characteristics of Pr3+ doped Lu3Al5O12 optical ceramics

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Scintillator-oriented combinatorial search in Ce-doped (Y,Gd)3(Ga,Al)5O12 multicomponent garnet compounds

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Comparative study of transparent ceramic and single crystal Ce doped LuAG scintillators

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2010)

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Evidence of the Inhomogeneous Ce3+ Distribution across Grain Boundaries in Transparent Polycrystalline Ce3+-Doped (Gd,Y)(3)Al5O12 Garnet Optical Ceramics

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Effects of Gd3+Substitution on the Fabrication of Transparent (Y1-xGdx)3Al5O12 Ceramics

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2009)

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Basic Properties of Ceramic Pr:LuAG Scintillators

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2009)

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Scintillation Properties of Praseodymium Doped LuAG Scintillator Compared to Cerium Doped LuAG, LSO and LaBr3

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2009)

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2009)

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Pr3+-doped complex oxide single crystal scintillators

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Synthesis and luminescent properties of Pr-doped Lu3Al5O12 translucent ceramic

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JOURNAL OF RARE EARTHS (2009)

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Optical and Scintillation Properties of Inorganic Scintillators in High Energy Physics

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2008)

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Article Engineering, Electrical & Electronic

Crystal growth and scintillation properties of 2-inch-diameter Pr:Lu3Al5O12 (Pr:LuAG) single crystal

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2008)

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Cerium-doped lutetium aluminum garnet phosphors and optically transparent ceramics prepared from powder precursors by a urea homogeneous precipitation method

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THIN SOLID FILMS (2008)

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Multiple synthesis routes to transparent ceramic lutetium aluminum garnet

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Luminescence and scintillation properties of YAG:Ce single crystal and optical ceramics

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Improvement of ceramic YAG(Ce) scintillators to (YGd)3Al5O12(Ce) for gamma-ray detectors

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NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (2007)

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Growth and luminescence properties of Pr-doped LU3(Ga,Al)5O12 single crystals

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JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS (2007)

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Scintillation characteristics of Lu3Al5O12:Ce optical ceramics

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Luminescence of undoped and Ce3+-doped Lu(Sc,Y)AG crystals

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JOURNAL OF LUMINESCENCE (2007)

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The temperature dependence of gamma-ray responses of YAG:Ce ceramic scintillators

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IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2006)

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Scintillation characteristics of pr-doped Lu3Al5O12 single crystals

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Development of novel scintillator crystals

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JOURNAL OF CRYSTAL GROWTH (2006)

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Article Physics, Applied

Antisite defect-free Lu3(GaxAl1-x)5O12:Pr scintillator

M Nikl et al.

APPLIED PHYSICS LETTERS (2006)

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Article Crystallography

Growth and scintillation properties of Pr-doped Lu3Al5O12 crystals

H Ogino et al.

JOURNAL OF CRYSTAL GROWTH (2006)

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Article Materials Science, Ceramics

Fabrication of transparent cerium-doped lutetium aluminum garnet (LuAG:Ce) ceramics by a solid-state reaction method

HL Li et al.

JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2005)

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Article Engineering, Electrical & Electronic

Evaluation of properties of YAG (Ce) ceramic scintillators

T Yanagida et al.

IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2005)

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Article Crystallography

Thermoluminescence and scintillation of praseodymium-activated Y3Al5O12 and LuAlO3 crystals

Winicjusz Drozdowski et al.

JOURNAL OF CRYSTAL GROWTH (2005)

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Article Nuclear Science & Technology

Scintillation response of Ce-doped or intrinsic scintillating crystals in the range up to 1 MeV

JA Mares et al.

RADIATION MEASUREMENTS (2004)

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Article Optics

Single mode tm and Tm,Ho:LuAG lasers for LIDAR applications

K Scholle et al.

LASER PHYSICS LETTERS (2004)

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Article Instruments & Instrumentation

Properties of Yb-doped scintillators: YAG, YAP, LuAG

S Belogurov et al.

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (2004)

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Article Engineering, Electrical & Electronic

Properties of LYSO and recent LSO scintillators for phoswich PET detectors

CM Pepin et al.

IEEE TRANSACTIONS ON NUCLEAR SCIENCE (2004)

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Article Materials Science, Multidisciplinary

Growth and optical properties of Yb doped new scintillator crystals

A Yoshikawa et al.

OPTICAL MATERIALS (2003)

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Article Optics

Inorganic scintillators: today and tomorrow

MJ Weber

JOURNAL OF LUMINESCENCE (2002)

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Article Chemistry, Multidisciplinary

Refractive index and dispersion of fluorides and oxides

RD Shannon et al.

JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA (2002)

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Article Instruments & Instrumentation

Scintillation properties of Lu3Al5O12:Ce single-crystalline films

Y Zorenko et al.

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT (2002)

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Article Engineering, Chemical

Controlled synthesis of nanostructured particles by flame spray pyrolysis

L Mädler et al.

JOURNAL OF AEROSOL SCIENCE (2002)

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Article Nuclear Science & Technology

Defect states in Lu3Al5O12 : Ce crystals

A Vedda et al.

RADIATION EFFECTS AND DEFECTS IN SOLIDS (2002)

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Article Physics, Applied

High-energy-resolution scintillator:: Ce3+ activated LaBr3

EVD van Loef et al.

APPLIED PHYSICS LETTERS (2001)

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Article Physics, Applied

High-energy-resolution scintillator:: Ce3+ activated LaCl3

EVD van Loef et al.

APPLIED PHYSICS LETTERS (2000)

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