期刊
JOURNAL OF POWER SOURCES
卷 305, 期 -, 页码 115-121出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2015.11.060
关键词
Layered titanate; Nano; Anode; Lithium-ion battery; Pseudocapacitance; Continuous hydrothermal flow synthesis
资金
- Engineering and Physical Sciences Research Council [EP/L015862/1]
- A Star (Singapore)
- EPSRC [EP/M009394/1]
- EPSRC [EP/M009394/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/M009394/1, 1570039] Funding Source: researchfish
Ultra-thin layered sodium titanate nano-sheets were synthesised using a continuous hydrothermal flow process and the as-prepared materials were investigated as an anode material for lithium-ion batteries. In comparison to previous studies on similar materials, the layered titanates herein showed high electrochemical activity at lower potentials. Cyclic voltammetry measurements in the potential range of 0.05 -2.1 V vs. Li/Li+, revealed that charge storage occurred from both lithium-ion intercalation as well as pseudocapacitive surface chemical processes. During electrochemical cycling tests, a high specific current of 0.5 A g(-1) was applied and the cells achieved a stable specific capacity of ca. 120 mAh g(-1) for over 1200 cycles. Even at an applied current of 10 A g(-1), the electrode material delivered a stable specific capacity of 38 mAh g(-1), which suggests that this material may be suitable for high power applications. (C) 2015 Elsevier B.V. All rights reserved.
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