期刊
JOURNAL OF POWER SOURCES
卷 311, 期 -, 页码 29-34出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2016.02.022
关键词
Cobalt phosphate; Electrocatalyst; Sodium-air battery; Aqueous electrolyte; Sodium super ionic conductor
资金
- UNIST (Ulsan National Institute of Science and Technology) [1.150034.01]
- National Research Foundation of Korea [NRF-2014R1A2A1A11052110]
Bifunctional catalysts are prominent to attain high capacity, maximum energy efficiency and long cycle life for aqueous rechargeable Na-air batteries. In this work, we report the synthesis of bi-functional noble metal free, Co-3(PO4)(2) nanostructures by facile precipitation technique and evaluated its electrocatalytic activity. Co-3(PO4)(2) nanostructure was investigated as a potential electrocatalyst for rechargeable aqueous Na-air battery for the first time. The synthesized Co-3(PO4)(2) grain-like nanostructures showed better oxygen evolution activity compared to Pt/C catalyst. The fabricated Na-air battery with the Co-3(PO4)(2) catalyst as air-cathode delivered low overpotential and its round trip energy efficiency reached up to 83%. The Na-air battery exhibited stable cycle performance up to 50 cycles. (C) 2016 Elsevier B.V. All rights reserved.
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