4.7 Article

Observation of Dirac Charge-Density Waves in Bi2Te2Se

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NANOMATERIALS
卷 13, 期 3, 页码 -

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MDPI
DOI: 10.3390/nano13030476

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topological insulator; charge-density wave; electron-phonon coupling; spin-orbit coupling; atom-surface scattering

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Experimental evidence for the existence of a charge-density wave (CDW) at the surface of a topological insulator is presented. The CDW is found to have the same period as a spin-density wave, indicating the presence of a strong electron-phonon interaction.
While parallel segments in the Fermi level contours, often found at the surfaces of topological insulators (TIs), would imply strong nesting conditions, the existence of charge-density waves (CDWs)-periodic modulations of the electron density-has not been verified up to now. Here, we report the observation of a CDW at the surface of the TI Bi2Te2Se(111), below approximate to 350 K, by helium-atom scattering and, thus, experimental evidence for a CDW involving Dirac topological electrons. Deviations of the order parameter observed below 180 K, and a low-temperature break of time reversal symmetry, suggest the onset of a spin-density wave with the same period as the CDW in the presence of a prominent electron-phonon interaction, originating from Rashba spin-orbit coupling.

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