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Review
Chemistry, Physical
Xingyun Li et al.
Summary: Amorphous alloys, also known as metallic glasses, are solid metallic materials with long-range disordered atomic structures. They have metallic characters and distinct properties associated with the amorphous structure, making them highly promising materials for catalyzing electrochemical reactions. This minireview summarizes the preparation, characterization, and electrocatalytic performances of various metallic amorphous alloy materials, discusses the influences of the amorphous alloy structure on different electrochemical reactions, and provides a summary of the advantages and challenges of amorphous alloys in electrocatalysis, along with future research directions.
Article
Engineering, Environmental
Dongqing Liu et al.
Summary: In this work, metal glass (MG) was used as the current collector for Li anode in Li metal batteries. By fabricating a CuZr MG ribbon with a lithiophilic surface, Li dendrites growth was impeded, resulting in high coulombic efficiency and low overpotential. The potential of MGs for practical application in lithium batteries was demonstrated.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Multidisciplinary
Ali Saad et al.
Summary: Transition metal borides are promising electrocatalysts for water splitting due to their conductivity and durability. In this work, the authors successfully synthesized highly crystalline ternary borides Mo2NiB2, which showed low overpotentials for both the oxygen evolution reaction and hydrogen evolution reaction in alkaline media.
Review
Chemistry, Physical
Rui Jiang et al.
Summary: This article highlights the substantial progress of metallic glass (MG) structures in electrocatalytic processes and their applications in energy storage devices. It discusses the structure-activity relationship of MG and electrochemical reaction kinetics, and proposes challenges and possibilities for designing highly-efficient MG-based electrode materials. The integration of high-throughput methods, artificial intelligence technology, and advanced characterization techniques is crucial for screening materials with remarkable performance.
ADVANCED ENERGY MATERIALS
(2022)
Article
Engineering, Environmental
Dongqing Liu et al.
Summary: In this work, a mesoporous IrNiTa (INT) MG ribbon with outstanding catalytic activity for both HER and OER is prepared. By combining experimental characterizations and theoretical calculations, the excellent catalytic performance is attributed to the large surface area of the mesoporous structure, good charge transfer at the electrode/electrolyte interface, super hydrophilicity/aerophobicity of the MG ribbon, and the promotion of Ni and Ta atoms towards the intrinsic activity of Ir atoms in the INT (HER) and of surface IrO2 layer (OER). Furthermore, using INT MG ribbons as both the cathode and anode for overall water splitting requires a smaller cell voltage and achieves a higher current density compared to traditional Pt/C||IrO2 couple, demonstrating the potential use of MGs as integrated bifunctional electrodes for scalable water electrolysis.
CHEMICAL ENGINEERING JOURNAL
(2022)
Review
Chemistry, Physical
A. Avani et al.
Summary: This paper focuses on the importance of nanostructured MoO3 in energy catalysis, summarizes its crystal structure and properties, and outlines its application advancement in hydrogen evolution reaction and oxygen evolution reaction.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2022)
Article
Chemistry, Physical
Tayyaba Najam et al.
Summary: This review summarizes the recent progress in precious and non-precious carbon based single-atom catalytic active sites for metal-air/O-2 batteries, water electrolyzers, and fuel-cells commercialization. The intrinsic catalytic activity, including the role of center-metal-atoms, metal-coordinated atoms, and the surrounding environment, is systematically discussed. The review focuses on the synthesis/identification approaches of active sites, their catalytic performance, and the factors influencing the performance, with equal emphasis on experimental results and theoretical calculations.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Premnath Kumar et al.
Summary: Hydrogen production through water splitting using Ni2P/CNT as efficient electrocatalysts has shown low overpotential and enhanced stability for hydrogen and oxygen evolution reactions in acidic and alkaline media. The use of carbon support has been proven to improve activity and stability compared to unsupported electrocatalysts.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Physical
Zongzhao Li et al.
Summary: The study successfully developed a high-performance cobalt phosphide@nitrogen-doped carbon catalyst through a simple phosphating process in an alkaline environment, showing excellent hydrogen and oxygen evolution reaction performances. A symmetric two-electrode water splitting setup demonstrated low working potentials, indicating that low-temperature phosphating treatment can be a simple and effective method for producing water splitting electrocatalysts.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Physical
Yu Jin et al.
Summary: The high anode overpotential of the oxygen evolution reaction (OER) in water electrolysis has been successfully addressed through the design and preparation of a group of nanoporous (Fe-Ni-Co)-based metallic glasses (NP-FeNiCo-MGs). The composite electrodes exhibit high catalytic activity towards water oxidation in 1 M KOH solutions, showing great potential for clean energy applications.
JOURNAL OF ALLOYS AND COMPOUNDS
(2021)
Article
Chemistry, Physical
Zongshan Lin et al.
Summary: This study reports a facile method to prepare Ru-based aerogels for hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and water electrolysis. Ru aerogel shows comparable performance with Pt/C for HER, while Ru0.7Co0.3 aerogel exhibits superior OER performance. The combined Ru and Ru0.7Co0.3 aerogel catalyst outperforms the Pt/C + RuO2 couple in practical overall water splitting test.
JOURNAL OF POWER SOURCES
(2021)
Article
Chemistry, Physical
Tayyaba Najam et al.
Summary: This study discusses a novel non-precious metal-based catalyst which shows remarkable performance in oxygen/hydrogen evolution reactions within nitrogen-doped carbon nanotubes, indicating potential for efficient water-splitting operations.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Physical
Yuan Wang et al.
Summary: The study systematically analyzed the structural parameters of bimetallic NiFe-MOFs influencing the performance and stability of the oxygen evolution reaction, leading to efficient MOF-nanocomposite electrocatalysts with low overpotential and excellent stability. Optimization of properties and addition of a conductive support substrate played a crucial role in achieving these results.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Physical
Z. Li et al.
Summary: This review discusses the application of cobalt phosphide nanocatalysts in electrocatalytic water splitting, including reaction mechanisms, synthesis methods, catalytic active sites, as well as strategies for improving performance and challenges for practical applications.
MATERIALS TODAY ENERGY
(2021)
Article
Materials Science, Multidisciplinary
Jin-Won Bae et al.
Summary: This study investigates the wet etching behavior of amorphous Cu50Zr50 thin films in a hydrogen peroxide-based copper wet etchant using electrochemical and surface analysis techniques. A new dissolution mechanism in the presence of fluoride ions in the hydrogen peroxide solution is proposed, indicating a strong dependence of the wet etching rate of amorphous CuZr on the existence of fluoride ions in the wet etchant.
ECS JOURNAL OF SOLID STATE SCIENCE AND TECHNOLOGY
(2021)
Article
Chemistry, Physical
Dinh Chuong Nguyen et al.
Summary: The Co and Nb dual-doping strategy modifies the electronic structure of MoS2, enhancing the efficiency of the Co,Nb-MoS2/TiO2 HSs catalyst for hydrogen evolution, oxygen evolution reaction, and oxygen reduction reaction. The unique hollow spherical structure and synergistic effects between TiO2 core and MoS2 shell provide effective channels for electron transfer and facilitate ion diffusion.
Article
Chemistry, Multidisciplinary
Zhe Jia et al.
Summary: A scalable strategy of alloying five equiatomic elements into a high-entropy metallic glass (HEMG) for HER in both alkaline and acidic conditions is proposed, with surface dealloying creating a nanosponge-like architecture offering abundant active sites. Experimental results demonstrate superior performance of this catalyst compared to others currently available. Density functional theory reveals the structural effects of nanocrystals on catalytic activity.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Ying Chen et al.
Summary: This study reports an air-stable Cu-based nanostructure consisting of Mn doped CuCl and CuO as a dual functional electrocatalyst for water splitting. The excellent catalytic activity and stability are found to be attributed to the main active component CuCl, along with Mn doping and the synergistic effect between CuCl and CuO, demonstrating the great potential of Cu-based non-noble metal electrocatalysts in water splitting and other renewable energy conversion technologies.
CHEMISTRY-AN ASIAN JOURNAL
(2021)
Article
Chemistry, Physical
Shuangshuang Jiang et al.
Summary: A self-supported FeNiCo-based amorphous catalyst with hierarchical micro/nanoporous structure was successfully designed, showing fast reaction kinetics, abundant active sites, and significant catalytic activity under alkaline conditions, enabling stable electrolysis apparatus for overall water splitting.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2021)
Article
Chemistry, Multidisciplinary
K. S. Aneeshkumar et al.
Summary: The Fe40Ni20Co20P15C5 metallic glass ribbons exhibit excellent electrocatalytic activity in water-splitting reactions, with low overpotentials for both hydrogen and oxygen evolution reactions under acidic and alkaline conditions. The electrochemical dealloying procedure reduces the overpotential significantly and maintains stability over 20 hours of testing. These metallic glass ribbons show promise for commercial and industrial electrocatalytic applications.
Article
Chemistry, Multidisciplinary
Jing Gao et al.
CHEMISTRY-A EUROPEAN JOURNAL
(2020)
Article
Chemistry, Multidisciplinary
Zi-Jian Wang et al.
ADVANCED MATERIALS
(2020)
Article
Chemistry, Physical
Shufang Cui et al.
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
(2020)
Article
Nanoscience & Nanotechnology
Qilong Liu et al.
ACS APPLIED NANO MATERIALS
(2019)
Article
Chemistry, Physical
Yinlong Zhu et al.
ADVANCED ENERGY MATERIALS
(2017)
Review
Chemistry, Physical
Varun Vij et al.
Article
Chemistry, Multidisciplinary
Yongwen Tan et al.
ADVANCED MATERIALS INTERFACES
(2017)
Article
Nanoscience & Nanotechnology
Fabao Zhang et al.
ACS APPLIED MATERIALS & INTERFACES
(2017)
Article
Chemistry, Multidisciplinary
Fei Hu et al.
ADVANCED MATERIALS
(2017)
Article
Chemistry, Multidisciplinary
Gustavo Doubek et al.
ADVANCED MATERIALS
(2016)
Article
Chemistry, Multidisciplinary
Yuan Chao Hu et al.
ADVANCED MATERIALS
(2016)
Article
Electrochemistry
Canbin Ouyang et al.
ELECTROCHIMICA ACTA
(2015)
Article
Chemistry, Multidisciplinary
Marcelo Carmo et al.
