☆ 4.6 Review

Cocatalysts for Photocatalytic Overall Water Splitting: A Mini Review

CATALYSTS (2023)

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Summary: Production of hydrogen fuel from sunlight and water is a promising pathway for carbon neutrality. A strategy using pure water, concentrated solar light, and an indium gallium nitride photocatalyst has achieved a solar-to-hydrogen efficiency of 9.2%. The strategy promotes forward hydrogen-oxygen evolution and inhibits reverse hydrogen-oxygen recombination by operating at an optimal reaction temperature, which can be achieved by harvesting infrared light in sunlight.

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Photocatalytic water splitting on BiVO4: Balanced charge-carrier consumption and selective redox reaction

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Summary: The interrelationship between photocatalytic activity and surficial reaction sites on BiVO4 photocatalyst was investigated by controlling the ratio of reductive and oxidative sites. The results showed that BiVO4 with a medium ratio of reductive/oxidative sites exhibited superior photocatalytic water oxidation and further modification with appropriate cocatalysts achieved efficient overall water splitting. The excellent photocatalytic performance was attributed to balanced charge-carrier consumption.

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Photocatalytic overall water splitting without noble-metal: Decorating CoP on Al-doped SrTiO3

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Summary: In this study, CoP was introduced onto the surface of Al-doped SrTiO3 through an in situ photodeposition-phosphorization method for photocatalytic overall water splitting. The POWS activity was significantly enhanced by CoP, which acted as reactive sites for H2 evolution reaction and facilitated surface reduction reaction. Further improvement was achieved by photodepositing Cr2O3 on the composite surface to suppress undesired reverse reaction. This work presents a new avenue for designing noble-metal-free cocatalyst system for photocatalytic overall water splitting.

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Pd single-atom decorated CdS nanocatalyst for highly efficient overall water splitting under simulated solar light

Wei Li et al.

Summary: This study presents a CdS-Pd nanocatalyst with improved stability and activity for solar-induced overall water splitting. The CdS-Pd nanocatalyst showed 110-fold higher activity than pristine CdS. It also demonstrated high apparent quantum yields under broadband light illumination. The findings provide important insights for the development of stable and efficient CdS-based photocatalysts for hydrogen production.

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Construction of Ag decorated 2D rGO/SnS2 nanostructure towards synergistically enabling overall water splitting

Yue Liu et al.

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Summary: This study investigates the role of RhCrOx cocatalyst in photo-catalytic water splitting, revealing its ability to promote the desired hydrogen evolution reaction while inhibiting the formation of harmful ROS. This suggests that regulation of ROS should be considered for designing a more efficient cocatalyst for photo-catalytic water splitting.

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Homojunction photocatalysts for water splitting

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Advances and challenges in developing cocatalysts for photocatalytic conversion of carbon dioxide to fuels

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Transition-Metal-Based Cocatalysts for Photocatalytic Water Splitting

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Summary: This review summarizes recent advances in transition-metal-based cocatalysts for photocatalytic water splitting. The fundamentals, including classification, function mechanisms, loading methods, modification strategies, and design considerations, are presented. The cases of reduction cocatalysts, oxidation cocatalysts, and reduction-oxidation dual cocatalysts for water splitting are further discussed. The challenges and possible research directions of transition-metal-based cocatalysts for photocatalytic water splitting are proposed.

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A Yin-Yang hybrid co-catalyst (CoOx-Mo2N) for photocatalytic overall water splitting

Baojun Ma et al.

Summary: A new Yin-Yang hybrid co-catalyst has been proposed for efficient water splitting, showing higher activity compared to traditional spatially separated dual co-catalysts. The superior performance is attributed to the adjacent spatial configuration, extra use of surface excitons, and more favorable water molecular absorption.

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Strategies and Challenges on Selectivity of Photocatalytic Oxidation of Organic Substances

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Summary: This review provides an overview of the fundamentals of reactive oxygen species in photocatalytic organic oxidations and discusses strategies to improve the selectivity of high value chemicals. Difficulties and challenges in developing highly selective oxidation photocatalysts are comprehensively discussed to guide future research focus.

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Summary: This review summarizes the basic concepts and synthetic methods of utilizing particulate semiconductor catalysts for water splitting to produce hydrogen, focusing on the role of co-catalysts and improving light absorption. It also discusses reactor design, overall technology costs, the potential for commercial-scale deployment of different technologies, and the significant challenges ahead. The highest reported efficiency of these systems to date is at least one order of magnitude lower than what is suitable for practical applications.

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Silver cocatalyst-concentration dependence of overall water splitting performance over silver-inserted solid-state heterojunction photocatalyst composed of zinc rhodium oxide and bismuth vanadium oxide

Hiroshi Irie et al.

Summary: The study achieved selective loading of Ag cocatalyst between ZRO and BVO via photodeposition method, with controlled Ag deposition which led to overall water splitting and increased generation of hydrogen and oxygen.

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The overall water splitting of CdS/Ti3+-SrTiO3 core-shell heterojunction via OER enhancement of MnOx nanoparticles

Jiaqi Pan et al.

Summary: This study enhanced the water splitting performance by fabricating MnOx/CdS/Ti3+-SrTiO3 core-shell heterojunction, achieving a well-matched HER/OER process and decent photocatalytic activity.

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Recent Advances in Noncontact External-Field-Assisted Photocatalysis: From Fundamentals to Applications

Xibao Li et al.

Summary: Effective separation of photogenerated carriers plays a crucial role in photocatalytic reactions, and the enhancement effect generated by an external field can provide extra energy to improve catalytic efficiency. Noncontact external fields, such as thermal, magnetic, microwave, and ultrasonic fields, have been found to broaden the applications of photocatalysis technology by improving the performance of catalytic systems.

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Boron-doped nitrogen-deficient carbon nitride-based Z-scheme heterostructures for photocatalytic overall water splitting

Daming Zhao et al.

Summary: Researchers have successfully used doped carbon nitride-based Z-scheme heterostructures to split water and produce hydrogen, but coupling suitable H-2 and O-2 evolution components remains challenging.

NATURE ENERGY (2021)

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Surface Modifications of (ZnSe)0.5(CuGa2.5Se4.25)0.5 to Promote Photocatalytic Z-Scheme Overall Water Splitting

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CrOx-Mediated Performance Enhancement of Ni/NiO-Mg:SrTiO3 in Photocatalytic Water Splitting

Kai Han et al.

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Structural Evolution during Photocorrosion of Ni/NiO Core/Shell Cocatalyst on TiO2

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Earth-abundant cocatalysts for semiconductor-based photocatalytic water splitting

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Cobalt-Oxide-Based Materials as Water Oxidation Catalyst: Recent Progress and Challenges

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Roles of Cocatalysts in Photocatalysis and Photoelectrocatalysis

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ACCOUNTS OF CHEMICAL RESEARCH (2013)

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One-Step Overall Water Splitting under Visible Light Using Multiband InGaN/GaN Nanowire Heterostructures

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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The effect of Au cocatalyst loaded on La-doped NaTaO3 on photocatalytic water splitting and O2 photoreduction

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Direct Water Splitting into Hydrogen and Oxygen under Visible Light by using Modified TaON Photocatalysts with d0 Electronic Configuration

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Tungsten Carbide Nanoparticles as Efficient Cocatalysts for Photocatalytic Overall Water Splitting

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Assembling graphitic-carbon-nitride with cobalt-oxide-phosphate to construct an efficient hybrid photocatalyst for water splitting application

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Nanoscale Strontium Titanate Photocatalysts for Overall Water Splitting

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Enhanced performance of NaTaO3 using molecular co-catalyst [Mo3S4](4+) for water splitting into H-2 and O-2

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Overall photocatalytic water splitting with NiOx-SrTiO3 - a revised mechanism

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Photocatalytic Water Splitting Using Modified GaN:ZnO Solid Solution under Visible Light: Long-Time Operation and Regeneration of Activity

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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Gas phase photocatalytic water splitting with Rh2-yCryO3/GaN:ZnO in μ-reactors

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Photocatalytic Overall Water Splitting Promoted by Two Different Cocatalysts for Hydrogen and Oxygen Evolution under Visible Light

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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2010)

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CHEMICAL REVIEWS (2010)

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Simultaneous photodeposition of rhodium-chromium nanoparticles on a semiconductor powder: structural characterization and application to photocatalytic overall water splitting

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Direct deposition of nanoparticulate rhodium-chromium mixed-oxides on a semiconductor powder by band-gap irradiation

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RuO2-loaded β-Ge3N4 as a non-oxide photocatalyst for overall water splitting

J Sato et al.

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New photocatalyst group for water decomposition of RuO2-loaded p-block metal (In, Sn, and Sb) oxides with d10 configuration

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Effect of chromium addition for photocatalytic overall water splitting on Ni-K2La2Ti3O10

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