☆ 4.6 Review

Unraveling the fundamentals of pulsed laser-assisted synthesis of nanomaterials in liquids: Applications in energy and the environment

APPLIED PHYSICS REVIEWS (2022)

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Article Engineering, Environmental

Time-resolved dynamics of laser-induced cavitation bubbles during production of Ni nanoparticles via pulsed laser ablation in different solvents and their electrocatalytic activity for determination of toxic nitroaromatics

Seung Jun Lee et al.

Summary: This study investigated the dynamics of laser-induced cavitation bubbles (LICBs) during pulsed laser ablation (PLA) of a nickel target in different solvents. It was found that the lifetime of LICBs depended on the liquid environment and strongly defined the phases of the Ni nanoparticles (NPs) formed. The prepared Ni NPs showed enhanced sensitivity and electrochemical performance, with the fcc/hcp Ni structure displaying the best performance.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Charge regulation engineering to suppress Jahn-Teller distortion in low crystallinity In-doping MnCo2O4 for high activity pseudocapacitors and hydrogen evolution reaction

Bang Lan et al.

Summary: The novel strategy of charge regulation engineering reduces the Jahn-Teller distortion in transition metal oxides, leading to excellent performance in supercapacitors and electrocatalysts with enhanced electrochemical activity and cycle stability.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Energy & Fuels

Multifunctional photo-electrocatalysts of copper sulfides prepared via pulsed laser ablation in liquid: Phase formation kinetics and photo-electrocatalytic activity

Talshyn Begildayeva et al.

Summary: Designing efficient and cost-effective electrocatalysts is crucial for creating a sustainable future energy source. In this study, phase-engineered nanospheres were synthesized using a unique liquid-based pulsed laser ablation method, and their multifunctionality was evaluated in hydrogen evolution, oxygen evolution, and methanol oxidation reactions. The synthesized electrocatalysts exhibited low overpotentials and high activity in alkaline media.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2022)

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Article Chemistry, Physical

In situ surface reconstruction on LaCoO3-δ leads to enhanced hydrogen evolution reaction

Di Liu et al.

Summary: Perovskite oxides are ideal electrocatalysts for water electrolysis, but their application in the hydrogen evolution reaction is limited due to poor efficiency and stability. This study uses pulsed laser deposition to fabricate nanoscale LaCoO3-delta on nickel foam, enhancing HER activity through in-situ surface reconstruction and interface engineering. The catalyst shows remarkable HER activity with low overpotential and superb stability in alkaline media, suggesting potential for engineering perovskite oxides as electrocatalysts in water electrolysis.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Article Materials Science, Multidisciplinary

Novel approach for the synthesis and recovery of lithium carbonate using a pulsed laser irradiation technique

Shreyanka Shankar Naik et al.

Summary: A high crystalline lithium carbonate (Li2CO3) was synthesized using pulsed laser irradiation (PLI) technique without precipitating agents, confirming a monoclinic phase of Li2CO3 through XRD analysis. Micro-Raman, FE-SEM, and EDS mapping analyses provided further vibrational modes, surface morphology, and elemental composition, supporting the evidence of high purity Li2CO3 formation and a robust synthetic route capable of efficient lithium recovery from real samples.

MATERIALS LETTERS (2022)

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Review Thermodynamics

Laser processing of graphene and related materials for energy storage: State of the art and future prospects

Rajesh Kumar et al.

Summary: This review summarizes recent studies on laser-assisted synthesis and modification of graphene-based materials, as well as their application as electrodes for supercapacitors and batteries. It provides an overview of the physical properties of graphene and different types of laser processing operations, with a detailed discussion on the practical uses of laser techniques for fabricating electrode materials.

PROGRESS IN ENERGY AND COMBUSTION SCIENCE (2022)

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Article Engineering, Environmental

Reconciling of experimental and theoretical insights on the electroactive behavior of C/Ni nanoparticles with AuPt alloys for hydrogen evolution efficiency and Non-enzymatic sensor

Yiseul Yu et al.

Summary: This study presents a new feasible strategy for fabricating carbon-coated nickel (C/Ni) nanoparticles with a AuPt alloy system, using an integrated pulsed laser irradiation and ultrasonochemical process. The C/Ni-AuPt alloy exhibited exceptional electrocatalytic activities for the hydrogen evolution reaction (HER) in acidic media and selective detection of 1,4-benzenediol. The optimized C/Ni-AuPt electrocatalyst showed a broad dynamic linear response range and high sensitivity for sensing 1,4-benzenediol.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Implementation of novel pulsed laser ablation strategy to control the morphological growth and enrich the electrochemically active sites of multifunctional Ni-CuO electrocatalyst

Talshyn Begildayeva et al.

Summary: A laser-based synthesis method for the preparation of multifunctional Ni-CuO nanocomposites is described, and the influence of Ni nanoparticles on the growth dynamics of CuO and the electrocatalytic activity is investigated. The prepared electrocatalyst exhibits excellent catalytic activity in methanol oxidation, oxygen evolution, and hydrogen evolution reactions.

JOURNAL OF ALLOYS AND COMPOUNDS (2022)

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Editorial Material Physics, Multidisciplinary

Freezing crystallographic defects into nanoparticles: The development of pulsed laser defect engineering in liquid (PUDEL)

S. Reichenberger

SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY (2022)

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Article Energy & Fuels

Cation modulation in dual-phase nickel sulfide nanospheres by pulsed laser irradiation for overall water splitting and methanol oxidation reaction

Deviprasath Chinnadurai et al.

Summary: This study focused on fabricating dual-phase nickel sulfide using pulsed laser irradiation technique and studying cation modulation for improved catalytic performance in various reactions. The Cu-Ni-S sample showed better performance in HER and OER compared to the Co-Ni-S sample, exhibiting excellent bifunctional activity and enhancing overall water splitting efficiency and methanol oxidation activity. The report highlights the efficiency and simplicity of fabricating transition metal derivatives and cation modulation using superficial laser methods.

FUEL (2022)

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Review Optics

Fundamentals and comprehensive insights on pulsed laser synthesis of advanced materials for diverse photo-and electrocatalytic applications

Jayaraman Theerthagiri et al.

Summary: This review presents the importance of pulsed laser synthesis technology in the production of nanomaterials and its application in the field of photo- and electrocatalysis. By analyzing the mechanisms and optimizing the structures, along with evaluating the catalytic performances in energy and environmental remediation processes, future directions and challenges of pulsed laser techniques are discussed.

LIGHT-SCIENCE & APPLICATIONS (2022)

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Article Chemistry, Physical

Architecting the AuPt alloys for hydrazine oxidation as an anolyte in fuel cell: Comparative analysis of hydrazine splitting and water splitting for energy-saving H2 generation

Yiseul Yu et al.

Summary: The study demonstrates that AuPt alloys have high activity for the hydrazine oxidation reaction in a water electrolyzer system, and exhibit excellent stability and electrocatalytic activity. This is significant for achieving high-rate hydrogen fuel generation and the advancement of hydrazine fuel cells.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Engineering, Environmental

Multiscale design of 3D metal-organic frameworks (M-BTC, M: Cu, Co, Ni) via PLAL enabling bifunctional electrocatalysts for robust overall water splitting

Shankar Naik Shreyanka et al.

Summary: This study successfully designed a new strategy and synthesized transition-metal-based 3D metal-organic framework (MOF) materials for the preparation of high-performance bifunctional electrocatalysts. The structural, morphological, and stability properties of the materials were characterized, and their performance in hydrogen and oxygen evolution reactions was studied using electrocatalytic reactions. The Co-BTC material exhibited excellent activity and stability.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Ceramics

Fabrication of g-C3N4/Au nanocomposite using laser ablation and its application as an effective catalyst in the reduction of organic pollutants in water

Atefeh Nasri et al.

Summary: Gold nanoparticles were fabricated on graphitic carbon nitride using laser ablation in liquid and ultrasonication. The prepared nanocomposite was characterized and used as an efficient catalyst for the reduction of 4-nitrophenol and methyl orange at room temperature. The recyclability of the catalyst was also examined.

CERAMICS INTERNATIONAL (2021)

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Review Materials Science, Ceramics

Recent progress on synthetic strategies and applications of transition metal phosphides in energy storage and conversion

Jayaraman Theerthagiri et al.

Summary: Transition metal phosphides (TMPs) have emerged as excellent energy conversion and storage materials due to their highly active surface sites and desirable properties. Comprehensive research has been conducted on TMPs and their applications in various energy conversion and storage technologies, with a focus on their unique electrochemical behavior and potential for improvement in multifunctional applications.

CERAMICS INTERNATIONAL (2021)

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Article Chemistry, Physical

General fabrication of metal oxide nanoparticles modified graphene for supercapacitors by laser ablation

Chenguang Zhu et al.

Summary: Metal oxide nanoparticles (MONPs)-graphene composites fabricated by a versatile approach show excellent performance as electrode materials for supercapacitors, with high specific capacitance, long-life cycling stability, and good mechanical flexibility. The simple and straightforward method used in this study provides a highly operable solution for large-scale preparation of micro-supercapacitors.

APPLIED SURFACE SCIENCE (2021)

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Review Materials Science, Ceramics

State-of-the-art technology: Recent investigations on laser-mediated synthesis of nanocomposites for environmental remediation

Babak Jaleh et al.

Summary: The pollution of hazardous/toxic environmental pollutants in water bodies is a global concern, impacting human health and economic development. Treatment of water/wastewater through photocatalytic processes, especially using laser ablation, has shown promising results in reducing/degrading organic and inorganic pollutants, highlighting the importance of this approach in environmental remediation.

CERAMICS INTERNATIONAL (2021)

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Article Environmental Sciences

Pulsed laser-assisted synthesis of metal and nonmetal-codoped ZnO for efficient photocatalytic degradation of Rhodamine B under solar light irradiation

Shreyanka Shankar Naik et al.

Summary: In this study, solar light-active ZnO:N/Ag nanocomposites were successfully fabricated and characterized. The optimized ZnO:N/Ag-2 nanocomposite showed efficient photocatalytic degradation of Rh.B under sunlight. Effective charge separation was achieved through the formation of a Schottky junction, and the presence of O-2(-) radicals contributed to the degradation of Rh.B.

CHEMOSPHERE (2021)

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Article Environmental Sciences

Efficient recovery of palladium nanoparticles from industrial wastewater and their catalytic activity toward reduction of 4-nitrophenol

Seung Jun Lee et al.

Summary: This study successfully recovered palladium nanoparticles from industrial wastewater using a pulsed laser ablation process without the need for additives or reducing agents. The recovered materials showed remarkable potential for application in the degradation of toxic aromatic nitro compounds in the environment.

CHEMOSPHERE (2021)

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Article Environmental Sciences

Plasmonic ZnO/Au/g-C3N4 nanocomposites as solar light active photocatalysts for degradation of organic contaminants in wastewater

Seung Jun Lee et al.

Summary: In this study, novel ZnO/Au/graphitic carbon nitride (g-C3N4) nanocomposites were fabricated using a liquid phase pulsed laser process, resulting in enhanced catalytic activity for methylene blue degradation. The synergistic effects between ZnO and g-C3N4, along with the surface plasmon resonance of Au nanoparticles, contribute to the improved photocatalytic performance of the ZnO/Au/g-C3N4 composite.

CHEMOSPHERE (2021)

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Article Chemistry, Physical

ZnO nanoparticles decorated carbon nanotubes via pulsed laser ablation method for degradation of methylene blue dyes

Ayman M. Mostafa et al.

Summary: ZnO nanoparticles were generated by laser ablation in liquid media to decorate carbon nanotubes in a one-step process. The amount of ZnO nanoparticles on the CNTs was controlled by optimizing the laser ablation time. The presence of CNTs was found to enhance the catalytic efficiency compared to pristine ZnO.

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2021)

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Article Chemistry, Physical

Synthesis of multi-walled carbon nanotubes decorated with silver metallic nanoparticles as a catalytic degradable material via pulsed laser ablation in liquid media

Ayman M. Mostafa et al.

Summary: In this research, a silver nanoparticle-decorated multi-walled carbon nanotube (MWCNTs/Ag nanocomposite) was prepared as a catalytic material for degrading nitro compounds and dyes. The method used for synthesis was clean, simple, and cost-effective. The nanocomposite showed promising catalytic activity for reducing hazardous materials and dyes, making it a potentially environmentally safe route for degradation.

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2021)

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Article Engineering, Environmental

Application of advanced materials in sonophotocatalytic processes for the remediation of environmental pollutants

Jayaraman Theerthagiri et al.

Summary: Significant industrial advancements have led to the release of toxic pollutants into the environment, necessitating efficient wastewater treatment processes to reduce contamination. Photocatalytic degradation is considered effective, but has limitations. Combining sonolysis with photocatalysis shows benefits for environmental remediation by utilizing more active radicals to degrade organic pollutants.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Physical

Enhanced photocatalytic degradation of rhodamine 6G (R6G) using ZnO-Ag nanoparticles synthesized by pulsed laser ablation in liquid (PLAL)

Nurfina Yudasari et al.

Summary: The photocatalytic degradation of Rhodamine 6G was enhanced by applying silver nanoparticles on a zinc oxide nanoparticle structure using a pulsed laser ablation in liquid technique. The inclusion of silver increased the photocatalytic ability of zinc oxide and facilitated a higher degradation rate of Rhodamine 6G. This research highlights the potential of hybrid nanomaterials developed through laser ablation technique for environmental protections.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Engineering, Environmental

Fabrication strategies and surface tuning of hierarchical gold nanostructures for electrochemical detection and removal of toxic pollutants

Jayaraman Theerthagiri et al.

Summary: The research on gold nanostructures has been extensively documented over the last few decades, focusing on synthesizing and characterizing these structures for applications in environmental remediation and electrochemical sensing. Current studies are mainly centered on the utilization of gold nanostructures in these areas, as well as the detection methods for various target analytes and degradation of toxic contaminants.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Catalytic activity of multi-walled carbon nanotubes decorated with tungsten trioxides nanoparticles against 4-nitrophenol

Eman A. Mwafy et al.

Summary: This study enhances catalytic reduction activity by utilizing multi-walled carbon nanotubes decorated with tungsten trioxide nanoparticles. The one-step preparation of the nanocomposite structure through infrared pulsed laser ablation demonstrates its potential large-scale applications in organic catalytic oxidation and wastewater treatment.

JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS (2021)

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Article Materials Science, Ceramics

Synthesis of manganese (IV) oxide at activated carbon on reduced graphene oxide sheets via laser irradiation technique for organic binder-free electrodes in flexible supercapacitors

Talal F. Qahtan et al.

Summary: A novel and green technique involving laser-induced photocatalytic reduction was developed to synthesize binder-free composite materials based on reduced graphene oxide (rGO) for flexible supercapacitors. The resulting supercapacitors demonstrated significant improvement in electrochemical performance due to the intrinsic characteristics of rGO such as high surface area, excellent electrical conductivity, and mechanical flexibility. The method is scalable, cost-effective, and can be used to produce all binder-free AC/rGO based composites for flexible energy-storage devices.

CERAMICS INTERNATIONAL (2021)

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Article Materials Science, Multidisciplinary

Novel laser-assisted method for synthesis of SnO2/MWCNTs nanocomposite for water treatment from Cu (II)

Eman A. Mwafy et al.

Summary: A novel multiwalled carbon nanotubes/SnO2 nanocomposite was synthesized using pulsed laser ablation in liquid media with sonication process for Cu(II) sorption in water treatment. The adsorbent was characterized using various techniques, and the impact of different variables on adsorption efficiency was studied.

DIAMOND AND RELATED MATERIALS (2021)

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Article Chemistry, Physical

Ni-doped carbon nanotubes fabricated by pulsed laser ablation in liquid as efficient electrocatalysts for oxygen evolution reaction

Sukhyun Kang et al.

Summary: Transition-metal-doped carbon-based electrocatalysts have been studied as alternatives to noble metal electrocatalysts for OER, and a simple technique using pulsed laser ablation for preparing Ni-doped multi-walled carbon nanotubes as OER catalysts was reported. The Ni-MWCNTs showed excellent OER catalytic performance, initial electrocatalytic activity, and good electrochemical durability.

APPLIED SURFACE SCIENCE (2021)

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Article Engineering, Environmental

Integrated technique of pulsed laser irradiation and sonochemical processes for the production of highly surface-active NiPd spheres

Yiseul Yu et al.

Summary: This study developed a new hybrid technique for producing highly surface-active NiPd alloy, which exhibited higher activity in the hydrogen evolution reaction and could be used as electrocatalysts.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Production of copper nanoparticles exhibiting various morphologies via pulsed laser ablation in different solvents and their catalytic activity for reduction of toxic nitroaromatic compounds

Talshyn Begildayeva et al.

Summary: Comparative experiments were carried out to study the effects of different solvents on the synthesis of copper-based nanoparticles. It was found that the copper NPs produced in methanol exhibited high catalytic activity. Particles with graphitic carbon layers showed superior catalytic performance in reducing nitrobenzene.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Article Chemistry, Physical

Zinc oxide/carbon nanotubes nanocomposite: Synthesis, characterization and catalytic reduction of 4-nitrophenol via laser assistant method

Fowzia S. Alamro et al.

Summary: In this study, ZnO nanoparticles were successfully prepared and decorated on the surface of carbon nanotubes through pulsed laser ablation method for the removal of 4-nitrophenol. The complete interaction between ZnO nanoparticles and carbon nanotubes was found to significantly enhance the catalytic efficiency against hazardous compounds.

SURFACES AND INTERFACES (2021)

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Article Chemistry, Physical

Rational synthesis of ZnO decorated Fe hierarchical nanostructures for enhanced photocatalytic performance by long-pulse-width laser ablation of binary alloys target

Xi Wang et al.

Summary: A facile approach was presented for the controllable synthesis of multifunctional ZnO decorated Fe hierarchical nanostructures, which showed promising potential in the photocatalytic degradation of aromatic dye Rhodamine B. The Fe@ZnO CSNSs displayed good performance under natural light irradiation and had effective separation of photogenerated carriers, enhancing their photocatalytic activity.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Engineering, Environmental

Rapid and highly selective electrochemical sensor based on ZnS/ Au-decorated f-multi-walled carbon nanotube nanocomposites produced via pulsed laser technique for detection of toxic nitro compounds

Shreyanka Shankar Naik et al.

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JOURNAL OF HAZARDOUS MATERIALS (2021)

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Review Green & Sustainable Science & Technology

Heteroatom-doped graphene-based materials for sustainable energy applications: A review

Seung Jun Lee et al.

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Facile one-pot synthesis of CuCN by pulsed laser ablation in nitrile solvents and mechanistic studies using quantum chemical calculations

Talshyn Begildayeva et al.

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Recent progress and emerging challenges of transition metal sulfides based composite electrodes for electrochemical supercapacitive energy storage

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Nickel sulfide nanostructures prepared by laser irradiation for efficient electrocatalytic hydrogen evolution reaction and supercapacitors

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Directed Synthesis of Mesoporous TiO2 Microspheres: Catalysts and Their Photocatalysis for Bisphenol A Degradation

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Hollow Nanoparticles of Metal Oxides and Sulfides: Fast Preparation via Laser Ablation in Liquid

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Comparison of the top-down and bottom-up approach to fabricate nanowire-based Silicon/Germanium heterostructures

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Microstructured Arrays of TiO2 Nanotubes for Improved Photo-Electrocatalysis and Mechanical Stability

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Process development for the removal of copper from wastewater using ferric/limestone treatment

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Synthesis of p-aminophenol by catalytic hydrogenation of p-nitrophenol

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