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Article
Chemistry, Multidisciplinary
Junjie Zhou et al.
Summary: Transient devices are an emerging type of electronics characterized by the dissolution or disintegration of their constituent materials after completing their missions. Research on transient devices is still in its infancy, with a relatively slow development in transient energy devices. In this study, a biodegradable zinc ion battery with a carefully designed cellulose aerogel-gelatin solid electrolyte was developed, demonstrating excellent electrochemical performance and controlled degradation.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Jiahui Zhou et al.
Summary: The flexible MXene/graphene scaffold created through an oriented freezing process can effectively inhibit dendritic growth of the zinc-metal anode and form a solid electrolyte interface at the electrode/electrolyte interface, improving battery stability and cycling life.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Guojin Liang et al.
Summary: The article introduces a method to solve the irreversibility issue of zinc metal anodes through a solution-dipping approach that constructs a protective coating. The synergistic combination of electric conductive coatings, insulating coatings, and 3D structural frameworks enables highly reversible zinc metal anode chemistry with suppressed gas production and dendrite growth.
ENERGY & ENVIRONMENTAL SCIENCE
(2022)
Editorial Material
Materials Science, Multidisciplinary
Ming Song et al.
Summary: This study introduces a method of using glucose as an electrolyte additive to improve the performance of aqueous Zn-ion batteries, enabling the zinc anode to have higher reversibility and stability.
Article
Chemistry, Multidisciplinary
Zefang Yang et al.
Summary: A protective copper nitride layer is constructed on the zinc metal anode to inhibit zinc dendrite growth effectively. By restricting the 2D atomic surface diffusion mechanism, stable zinc deposition with enhanced electrochemical stability is achieved.
Article
Chemistry, Physical
Kailin Guan et al.
Summary: By assembling a self-consistent hydrophobic interface, water erosion can be blocked and the deposition process of zinc ions can be regulated, thereby improving the stability of the zinc metal anode.
ADVANCED ENERGY MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Shiyin Xie et al.
Summary: This article reports a novel strategy of using zincophilic Cu nanowire networks to stabilize zinc anodes. The Cu nanowire networks can homogenize the surface electric field and Zn2+ concentration field, and inhibit side reactions through their hydrophobic feature. The facets and edge sites of the Cu nanowires, especially the latter ones, are highly zincophilic, which promotes uniform zinc nucleation/deposition. The protected zinc anodes exhibit an ultralong cycle life and rapid charge/discharge ability.
NANO-MICRO LETTERS
(2022)
Review
Nanoscience & Nanotechnology
Bin Li et al.
Summary: This article reviews the role of interfacial engineering in inhibiting the growth of Zn dendrites and the occurrence of side reactions. Researchers have regulated the deposition behavior of Zn ions through surface modification and the addition of electrolyte additives to achieve uniform Zn nucleation and flat Zn deposition, improving the cycling stability of Zn anodes.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Applied
Shizhe Gao et al.
Summary: Researchers reported a nanoflower vanadium tetrasulfide/carbon nanotubes cathode material with high Zn storage performance, which has great application potential in large-scale energy storage.
JOURNAL OF ENERGY CHEMISTRY
(2022)
Article
Multidisciplinary Sciences
Bingyao Zhang et al.
Summary: This study effectively addresses the issues of dendrite growth and side reactions in zinc-ion batteries by using a highly-confined tannic acid modified sodium alginate composite gel electrolyte. The modified electrolyte guides and regulates zinc deposition, resulting in steady zinc plating/stripping behavior and high cycle stability.
Editorial Material
Chemistry, Physical
Qing Li et al.
Article
Chemistry, Physical
Weijun Zhou et al.
Summary: This study utilizes a cotton-derived cellulose film as a separator for AZIBs, which effectively inhibits zinc dendritic growth and harmful side reactions due to its excellent mechanical properties and ionic conductivity. Batteries with this separator show stability and high capacity, as well as improved rate capability and cyclability.
ENERGY STORAGE MATERIALS
(2022)
Review
Chemistry, Applied
Aruuhan Bayaguud et al.
Summary: Rechargeable aqueous zinc-ion batteries have high power density and low cost, but face challenges such as dendrite formation and interfacial parasitic reactions at the zinc anode, leading to low zinc reversibility and hindering commercialization. Thorough understanding and development of inhibition strategies, including electrode design and electrolyte modification, are crucial for addressing these issues.
JOURNAL OF ENERGY CHEMISTRY
(2022)
Article
Chemistry, Multidisciplinary
Fangwang Ming et al.
Summary: This work proposes a hybrid electrolyte induced by the salting-in effect as an effective strategy to achieve a highly reversible zinc anode with good stability and compatibility. By altering the solvation structure and reducing parasitic side reactions, this electrolyte ensures a stable zinc anode with excellent cycling stability.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Materials Science, Multidisciplinary
Chao Guan et al.
Summary: By using Zn(CF3SO3)(2) as an electrolyte, the electrode of zinc ion battery shows high cycle stability and capacity retention at high rates. Compared to ZnSO4 electrolyte, the electrode operates under different electrochemical mechanisms, transforming the HNaV6O16·4H2O electrode in-situ to ZnxV2O5·nH2O.
Article
Multidisciplinary Sciences
Canpeng Li et al.
Summary: An 'all-in-one' (AIO) electrode was developed by combining structural design, interface modification, and electrolyte optimization, which can effectively improve the stability and performance of zinc-ion batteries.
NATIONAL SCIENCE REVIEW
(2022)
Article
Nanoscience & Nanotechnology
Huan Meng et al.
Summary: The in situ surface alloying of Cu and Zn with the assistance of anionic surfactant has been found to significantly improve the reversibility of 3D nanoporous Zn electrodes, leading to enhanced performance of aqueous rechargeable zinc-metal batteries. The self-supported nanoporous ZnxCuy/Zn electrodes exhibit superior dendrite-free Zn stripping/plating behaviors, high Zn utilization, and long-term stability.
NANO-MICRO LETTERS
(2022)
Article
Electrochemistry
Mingming Wang et al.
Summary: This study constructs a Zn/Bi electrode by in-situ growth of a Bi-based energizer upon the Zn metal surface using a replacement reaction. Experimental and theoretical calculations demonstrate that the Bi-based energizer composed of metallic Bi and ZnBi alloy contributes significantly to Zn plating/stripping due to strong adsorption energy and fast ion transport rates. The Zn/Bi electrode not only avoids Zn dendrite growth but also improves Zn anode anti-corrosion performance.
Article
Chemistry, Multidisciplinary
Huanyan Liu et al.
Summary: This research proposes a novel metal-organic complex interphase strategy to address the corrosion and dendrite issues in aqueous Zn metal batteries. By forming complex interphases between metal Zn and phytic acid, the deposition of Zn is made more uniform and the Coulombic efficiency is significantly improved, leading to enhanced stability and cycling lifetime of Zn metal batteries.
ENERGY & ENVIRONMENTAL SCIENCE
(2022)
Article
Chemistry, Multidisciplinary
Ruirui Zhao et al.
Summary: An anti-corrosion elastic constraint (AEC) consisting of nanosized TiO2 and polyvinylidene fluoride (PVDF) matrix was introduced to address the issues of dendrite formation and sustained corrosion in Zn metal anodes for aqueous batteries. This coating significantly improved the electrodeposition consistency and thermodynamic stability of the Zn anode, enabling long-term stable plating/stripping performance with high efficiency and no dendrite formation.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Yunpei Zhu et al.
Summary: Aqueous Zn-based batteries are promising due to their low cost and high capacity, but existing designs use excess Zn which reduces energy density. A new anode-free design utilizing nanocarbon nucleation layer enables uniform Zn electrodeposition with high efficiency and stability across various current densities. This innovation opens up new possibilities for implementing Zn-based batteries in energy storage systems.
Article
Chemistry, Physical
Tianjiao Li et al.
Summary: The oxygen-containing carbonized coconut framework (O-CCF) with a 3D tubular structure is designed to inhibit dendrite growth, enabling stable Na stripping/plating over 10,000 cycles. The oxygen functional groups contribute to the adsorption of Na+ and reduce the Na nucleation energy on the surface of O-CCF.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Physical
Liangdong Lin et al.
Summary: The lifespan of an anode-free Li metal battery has been prolonged by applying an epitaxial induced plating current-collector (E-Cu) in this study, promoting Li storage and forming a LiF-rich solid electrolyte interphase (SEI) beneficial for uniform Li plating. This strategy has increased the initial coulombic efficiency and capacity retention of the battery, achieving a remarkable energy density under limited electrolyte addition conditions.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Physical
Fangxi Xie et al.
Summary: The bonding between zinc ions and zincophilic sites is revealed as the mechanism for suppressing zinc-dendrite formation in the ZMA host, leading to enhanced electrochemical performance. This study highlights the importance of nitrogen zincophilic sites in inhibiting zinc-dendrite growth.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Physical
Yamin Zhang et al.
Summary: Rechargeable aqueous zinc anodes are attracting attention for their safety, low cost, and high theoretical volumetric capacity. Zinc anodes in aqueous electrolytes often suffer from dendritic metal deposition, with the regulation of Zn using Zn-alloying metals as a reported solution. By introducing Ag on Zn anodes, uniform Zn deposition was achieved, leading to improved cycling performance. This alloy-seeding design principle could potentially enhance the rechargeability of other metal anodes.
ACS ENERGY LETTERS
(2021)
Article
Nanoscience & Nanotechnology
Ziqi Wang et al.
Summary: This study presents a Janus separator based on a Zn-ion conductive metal-organic framework (MOF) and reduced graphene oxide (rGO), which can simultaneously regulate uniform Zn2+ flux and electron conduction during battery operation, effectively improving the stability and corrosion issues of Zn anodes.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Yongling An et al.
Summary: Anode-free zinc batteries (AFZBs) have great potential as energy storage systems due to their high energy density, inherent safety, low cost, and simplified fabrication process. However, rapid capacity fading caused by side reactions hinders their practical applications. Aqueous AFZBs enabled by electrolyte engineering with a stable interphase are designed to address these issues. Introducing a multifunctional zinc fluoride (ZnF2) additive into the electrolyte helps to form a stable F-rich interfacial layer, improving cycling performance and longevity of AFZBs.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Shiying Li et al.
Summary: The research investigates the influence of surface structure on the nucleation and deposition of Zn by reconstructing the surface structure of a Zn-metal anode with Sn crystal textures. The high-affinity Zn binding sites of Sn and the high surface energy ensure better wettability from the deposits and promote the lateral growth of Zn crystals, leading to improved stability and cycling performance of the Zn-metal anode.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Miao Zhou et al.
Summary: This study investigates a novel zinc anode with a surface-preferred (002) crystal plane, revealing its characteristics of fewer dendrites, no by-products, and weak hydrogen evolution. This leads to improved stability and reversibility of the battery system.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Physical
Yingchang Jiang et al.
Summary: The study demonstrates a novel self-grown strategy for binder-free, freestanding electrodes on Zn2+ ion storage using thin, flexible ammonium vanadates nanostructures. The resulting paper cathode exhibits high reversible capacity and specific energy, outperforming most zinc-ion batteries based on powder form cathodes. The design of the paper electrode with binder-free and porous architecture shows great potential in Zn2+ ion storage.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Physical
Jian Wu et al.
Summary: This study introduces spinel Zn3V3O8 as a high-capacity zinc supplied cathode in vanadium family for AZIBs, achieving a discharge capacity of 285 mA.h g(-1) and excellent capacity retention. Additionally, a novel Zn-metal free AZIBs using Zn3V3O8 parallel to carbon paper battery has been designed, aiming to promote the practical application of rechargeable AZIBs.
ENERGY STORAGE MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Longsheng Cao et al.
Summary: The study introduces an aqueous zinc battery with a solid-electrolyte interphase that enables excellent performance in various tests, demonstrating its potential for practical applications in energy storage.
NATURE NANOTECHNOLOGY
(2021)
Article
Chemistry, Multidisciplinary
Shuang Zhou et al.
Summary: The study introduces an elastic and anti-corrosive interlayer (PSN-Zn) to address dendrite formation and complex side reactions of Zn metal anodes in aqueous Zn batteries. The interlayer improves the electrochemical stability and lifespan of Zn anodes, even under harsh conditions, and has been proven to be effective in full cells as well.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Huaizhi Liu et al.
Summary: By combining photolithography with electrochemical machining, a flexible ultrathin and ultralight Zn micromesh is fabricated for high-performance aqueous Zn-ion batteries, demonstrating excellent flexibility and mechanical strength.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Pan Xue et al.
Summary: A 3D porous hollow fiber scaffold with well-dispersed TiO2, SiO2, and carbon is utilized as the superzincophilic host materials for zinc anodes to address the uncontrolled dendrite formation issue, resulting in enhanced cycling lifespan and coulombic efficiency.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Engineering, Chemical
Yang Li et al.
Journal of Energy Chemistry
(2021)
Article
Chemistry, Multidisciplinary
Ze Chen et al.
Summary: In this study, the issues faced by the zinc metal anodes in aqueous zinc ion batteries (ZIBs) were addressed using a solid polymer electrolyte, resulting in the development of all-solid-state ZIBs with superior stability and reliability. By effectively suppressing dendrites and side reactions, excellent cycling performance of up to 10,000 cycles was achieved, with the batteries able to function normally in temperatures ranging from -35 degrees Celsius to 100 degrees Celsius.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Yihu Li et al.
Summary: This study demonstrates a new nucleation mechanism in aqueous zinc-ion batteries by introducing high-valence cations into the electrolyte to regulate zinc deposition behavior, resulting in more stable and long-lasting cycling performance. The effects of cation adsorption on zinc nucleation are deeply explored, leading to higher capacity retention and longer cycling life compared to additive-free electrolytes.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
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Longtao Ma et al.
ADVANCED MATERIALS
(2020)
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Sheng-Bo Wang et al.
NATURE COMMUNICATIONS
(2020)
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ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2019)
Review
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Boya Tang et al.
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ENERGY & ENVIRONMENTAL SCIENCE
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Jianhang Huang et al.
NATURE COMMUNICATIONS
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Litao Kang et al.
ADVANCED ENERGY MATERIALS
(2018)
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Dipan Kundu et al.
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Chengjun Xu et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2012)
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Salim Derrouiche et al.
CHEMISTRY OF MATERIALS
(2012)
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S Funk et al.
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G Trejo et al.
JOURNAL OF APPLIED ELECTROCHEMISTRY
(2001)
