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Article
Engineering, Environmental
Yanyi Wang et al.
Summary: This work presents an in-situ formation strategy of V2O5/C composite nanosheets derived from V4AlC3 MAX, as an efficient Zn2+ storage host, through electrochemically etching-induced phase transition. The V4AlC3 MAX electrode conversion mechanism is studied systematically. The results demonstrate that the derived electrode exhibits high specific capacity, superior rate capability, and cycling stability, providing an effective strategy for green and advanced cathode material design.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Chemistry, Multidisciplinary
Aosai Chen et al.
Summary: The researchers developed a multifunctional coating called PVA@SR-ZnMoO4 on the Zn anode, which consists of an outer layer PVA@SR to enhance flexibility and Zn2+ mobility, and an inner layer ZnMoO4 to inhibit dendrite growth and side reactions. The cooperation between these layers improved the performance of the Zn anode.
ENERGY & ENVIRONMENTAL SCIENCE
(2023)
Article
Chemistry, Multidisciplinary
Xinliang Li et al.
Summary: Using MXene materials as an artificial layer can induce uniform zinc deposition, leading to an extended lifespan of the zinc anode. Among different terminations, Cl termination is found to be more effective in regulating zinc ion diffusion.
Article
Chemistry, Multidisciplinary
Kefeng Ouyang et al.
Summary: A strategy to build an indium metal interphase on the zinc anode surface is proposed, preventing hydrogen evolution reaction and zinc corrosion, guiding smooth zinc deposition. This approach achieves ultrahigh cumulative capacities and stable plating/stripping behavior, with encouraging rate performance and cyclic stability for Zn-V2O5 batteries.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Xuemei Ma et al.
Summary: This work introduces organic-inorganic hybrid cathodes with a dual energy-storage mechanism for aqueous zinc-ion batteries, providing high specific capacity, elevated voltage, and excellent long-term cycle stability. Density functional theory calculations show remarkable electronic conductivity with an ultralow diffusion barrier, opening new research directions in high-energy secondary batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Jiahui Zhou et al.
Summary: The flexible MXene/graphene scaffold created through an oriented freezing process can effectively inhibit dendritic growth of the zinc-metal anode and form a solid electrolyte interface at the electrode/electrolyte interface, improving battery stability and cycling life.
ADVANCED MATERIALS
(2022)
Review
Nanoscience & Nanotechnology
Bin Li et al.
Summary: This article reviews the role of interfacial engineering in inhibiting the growth of Zn dendrites and the occurrence of side reactions. Researchers have regulated the deposition behavior of Zn ions through surface modification and the addition of electrolyte additives to achieve uniform Zn nucleation and flat Zn deposition, improving the cycling stability of Zn anodes.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Multidisciplinary
Dao-Sheng Liu et al.
Summary: A novel 3 m Zn(CF3SO3)2 electrolyte was used to improve the cycling performance and specific capacity of aqueous vanadium-based zinc-ion batteries. By manipulating the solvation structure of the electrolyte, the batteries showed super-stable cycling performance and high specific capacity.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yongchang Liang et al.
Summary: This study developed a unique dual-interface engineering strategy to design an efficient ion transport modulator separator for Zn metal batteries. By decorating BaTiO3 (BTO) on glass fiber, the modified separator can capture and accelerate ion transport, and distribute it homogenously, resulting in highly reversible Zn plating/stripping in the anode and improved battery performance.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Physical
Hao Zhang et al.
Summary: High yield carbon dots (CDs) with abundant polar functional groups are used to optimize the electrolyte/Zn interfaces, effectively preventing dendritic growth and parasitic reactions. The CDs also improve the reaction kinetics and lifespan of the Zn anode.
ADVANCED ENERGY MATERIALS
(2022)
Article
Multidisciplinary Sciences
Canpeng Li et al.
Summary: An 'all-in-one' (AIO) electrode was developed by combining structural design, interface modification, and electrolyte optimization, which can effectively improve the stability and performance of zinc-ion batteries.
NATIONAL SCIENCE REVIEW
(2022)
Article
Chemistry, Physical
Yajun Zhao et al.
Summary: This study proposes sulfur doped MnO2 nanosheets as a high-performance cathode material for zinc-ion batteries, exhibiting large discharge capacity, high rate performance, and long cycle life. The incorporation of sulfur improves the intrinsic electronic conductivity of MnO2 and accelerates reaction kinetics by weakening the electrostatic interactions with Zn(2+) cations. The sulfur doping also induces an amorphous surface with abundant oxygen defects, contributing to additional Zn storage sites with pseudocapacitive behavior.
ENERGY STORAGE MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Yang Song et al.
Summary: In this study, a metal-organic framework modified separator is proposed for robust aqueous zinc-ion batteries. The modified separator enhances the transport ability of charge carriers and corrosion resistance, resulting in dendrite-free zinc deposition. Experimental results show excellent performance in terms of cycle life and capacity retention.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Physical
Xiaobin Hui et al.
Summary: In this study, an optimized electrode-electrolyte integrated MXene/Zn-layered double hydroxides (LDH)-array@PVA structure is developed to improve the working life and energy density of flexible zinc-air batteries (ZABs).
ADVANCED ENERGY MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Yangwu Chen et al.
Summary: A multifunctional anti-proton electrolyte is proposed to address multiple issues in aqueous Zn-vanadium oxide battery. The electrolyte can regulate solvation structure, inhibit ionization of free water molecules, achieve smaller lattice expansion and reduce by-product formation. It also helps guide uniform Zn deposition and suppress hydrogen evolution side reactions.
NANO-MICRO LETTERS
(2022)
Article
Chemistry, Physical
Xiujuan Chen et al.
Summary: The application of a polyvinyl alcohol coating on the zinc anode has successfully achieved dendrite-free and long-life aqueous zinc batteries, demonstrating superior cyclability and durability. The insights gained from this research shed light on the future development of stable zinc anodes.
Article
Chemistry, Physical
Meijia Qiu et al.
Summary: This article introduces a method to improve the long-term reversible plating/stripping of zinc anodes by introducing sorbitol as an additive. The research found that sorbitol can promote the preferred (002) orientation growth on the zinc anode surface, which facilitates stable inversion of the zinc deposition. Additionally, sorbitol modulates the solvation structure of Zn2+ and reduces common side reactions. Experimental results demonstrate the excellent stability of the zinc anode in zinc-zinc symmetric cells and other types of full cells.
ENERGY STORAGE MATERIALS
(2022)
Article
Nanoscience & Nanotechnology
Jinxin Xu et al.
Summary: MXenes have shown potential applications in electrochemical energy storage due to their high electrical conductivity, pseudocapacitance, and two-dimensional layered structures with a regulatable interlayer spacing. Intercalation strategy can greatly influence the properties and electrochemical performance of MXenes.
ACS APPLIED NANO MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Juan Feng et al.
Summary: The concept of multifunctional MXene bonded transport network-embedded poly(vinylidene fluoride co-hexafluoropropylene)/Zn(OTf)(2) solid polymer electrolyte (PH/MXene SPE) is proposed as an all-in-one strategy for designing robust solid polymer electrolyte. Through comprehensive research including density functional theory calculation, simulation, and multiple characterization techniques, the mechanism of the rational designed solid polymer electrolyte on regulating ion transport, interphase chemistry, and zinc deposition is uncovered. The PH/MXene SPE enables ultrastable zinc plating/stripping behavior and demonstrates significantly improved rate performance and cyclic stability in solid-state Zn/VO2 batteries. The unique strategy proposed in this work offers a new insight into solid polymer electrolyte design and the development of high-performance solid-state Zn metal batteries.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Boyu Li et al.
Summary: By constructing a Cu-Zn alloy interlayer on Zn foil, researchers successfully fabricated an ultra-stable Zn metal anode, which effectively suppresses dendrite growth and side reactions, leading to improved electrochemical performance.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Multidisciplinary
Xu Liu et al.
Summary: The study demonstrates the effectiveness of ion-affiliative cellulose acetate (CA) coating with Zn(CF3SO3)(2) on Zn anode in suppressing zinc dendrite formation and growth in aqueous electrolytes. The symmetric CAZ@Zn//CAZ@Zn battery shows significantly improved reversible plating/stripping performance compared to bare Zn, while the full cell with optimized Zn anode and NH4V4O10 cathode achieves substantially stable performance, outperforming bare Zn.
Article
Chemistry, Physical
Qiuju Xu et al.
Summary: By preparing a Ti-MOF derived nanocomposite coating, researchers have successfully improved the anode performance of aqueous Zn-based batteries, including corrosion resistance, cycle life, and the reduction of dendrite growth and hydrogen gas evolution. When combined with a MnO2 cathode, this anode exhibits higher and more stable capacity.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Review
Chemistry, Multidisciplinary
Jing Zou et al.
Summary: 2D carbides and nitrides of transition metals, known as MXenes, are a new class of 2D nanomaterials that show excellent performance and broad application prospects in various fields. However, their surface functional groups are difficult to control due to the exposure of metal atoms and implanted ions during the extraction process. By adding synergistic additives under non-hazardous conditions, stable and efficient MXene-based materials with exceptional optical, electrical, and magnetic properties can be obtained.
CHEMICAL SOCIETY REVIEWS
(2022)
Article
Chemistry, Multidisciplinary
Shengwei Li et al.
Summary: The research successfully increased the MoS2 interlayer spacing and enhanced hydrophilicity by innovatively intercalating graphene into MoS2 layers, forming MoS2/graphene nanocomposites with flower-like structures. These composites showed exceptional high-rate capability and long-term cycling stability, paving a new direction for high-performance cathodes in aqueous zinc-ion batteries.
ADVANCED MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Chuang Sun et al.
Summary: Well-dispersed MXene nanosheets in the electrolyte facilitate Zn2+ migration and deposition, while the MXene interfacial layer induces uniform nucleation. The MXene-containing electrolyte enables dendrite-free Zn plating/striping with high efficiency and superior reversibility.
NANO-MICRO LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Miao Zhou et al.
Summary: This study investigates a novel zinc anode with a surface-preferred (002) crystal plane, revealing its characteristics of fewer dendrites, no by-products, and weak hydrogen evolution. This leads to improved stability and reversibility of the battery system.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Physical
Yuan Tian et al.
Summary: By designing and growing multifunctional uniform antimony nanoarrays on Ti3C2Tx MXene paper, this study demonstrates the feasibility of antimony as an alloying-type Zn storage anode and provides an effective approach to suppress Zn dendrites.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Physical
Jian Wu et al.
Summary: This study introduces spinel Zn3V3O8 as a high-capacity zinc supplied cathode in vanadium family for AZIBs, achieving a discharge capacity of 285 mA.h g(-1) and excellent capacity retention. Additionally, a novel Zn-metal free AZIBs using Zn3V3O8 parallel to carbon paper battery has been designed, aiming to promote the practical application of rechargeable AZIBs.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Xinliang Li et al.
Summary: The study focuses on utilizing Ti(3)C(2)Tx MXene as a redistributor for zinc powder anodes, constructing a stable and highly reversible zinc powder anode to address dendrite growth and polarization issues, improving the cycle life and rate capability of zinc-based full batteries.
Article
Chemistry, Multidisciplinary
Jiahui Zhou et al.
Summary: By synthesizing a nitrogen-doped graphene oxide film on zinc foil, this study effectively suppresses hydrogen evolution reactions and passivation, improving the electrochemical performance of aqueous Zn-ion batteries. This research provides a new method for enhancing the application of high-specific-energy AZIBs.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Shengwei Li et al.
Summary: The study introduces a molecular engineering strategy for MoS2 cathodes, involving the manufacturing of structure defects and O-doping to unlock the inactive basal plane and increase the interlayer spacing, leading to the production of abundant 1T-phase for enhanced Zn2+ transport. The tailored D-MoS2-O material exhibits excellent hydrophilicity and high conductivity, allowing for high-rate capability and stable performance in a wearable rechargeable Zn battery, showcasing great application potential for aqueous Zn-ion batteries.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Physical
Yingjie Gao et al.
Summary: Despite challenges in the field, the organic cathode material TAPQ, with its easily-synthesized nature and novel structure, demonstrated excellent electrochemical performance and a clear H+/Zn2+ co-insertion mechanism. This provides important insights for further development of organic cathode materials for ARZBs towards practical applications.
ENERGY STORAGE MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Yongling An et al.
Summary: By designing and constructing a protective heterogeneous layer composed of sulfur-doped three-dimensional (3D) MXene and ionic conductive ZnS on the zinc anode, the issues of dendrite growth and side reactions hindering the practical applications of zinc anode in aqueous batteries have been successfully addressed. This results in a stable and dendrite-free zinc anode with notable cycling stability and high-rate performance.
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JOURNAL OF ENERGY STORAGE
(2019)
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Qian Pan et al.
ACS APPLIED ENERGY MATERIALS
(2019)
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David B. Lioi et al.
ACS APPLIED NANO MATERIALS
(2019)
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Tao Hu et al.
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(2018)
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Tian Zhang et al.
JOURNAL OF ALLOYS AND COMPOUNDS
(2017)
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Pan He et al.
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(2017)
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APPLIED SURFACE SCIENCE
(2016)
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PHYSICAL CHEMISTRY CHEMICAL PHYSICS
(2015)
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CERAMICS INTERNATIONAL
(2013)
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ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2012)
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