☆ 4.6 Review

Profitable Fischer Tropsch realization via CO2-CH4 reforming; an overview of nickel-promoter-support interactions

RSC ADVANCES (2023)

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Production of hydrogen via methanol steam reforming over mesoporous CeO2-Cu/KIT-6 nanocatalyst: Effects of polar aprotic tetrahydrofuran solvent and ZrO2 promoter on catalytic performance

Majid Taghizadeh et al.

Summary: CeO2-Cu/KIT-6 catalysts were prepared using conventional impregnation method and ethylene glycol-assisted impregnation method. The impact of the zirconium promoter on the catalytic activity of the catalyst in methanol steam reforming was evaluated. The results showed that the use of THF solvent and incorporation of ZrO2 significantly improved the performance of the catalyst.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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The Effect of Calcination Temperature on Various Sources of ZrO2 Supported Ni Catalyst for Dry Reforming of Methane

Ahmed Aidid Ibrahim et al.

Summary: The performance of dry reforming catalysts is influenced by the source of ZrO2 support and calcination temperature. Increasing the calcination temperature decreases the activity of the catalysts when the average conversion is higher than 40%. However, the impact of calcination temperature does not constantly decrease for low activity catalysts with an average conversion of less than 40%.

CATALYSTS (2022)

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Article Chemistry, Physical

Sustainable Synthesis of a Highly Stable and Coke-Free Ni@CeO2 Catalyst for the Efficient Carbon Dioxide Reforming of Methane

Seung Bo Kim et al.

Summary: A facile and green synthetic strategy was developed to construct an efficient Ni@CeO2 catalyst for the dry reforming of methane. The catalyst showed superb syngas production efficiency and stability, with resistance to carbon deposits and sintering. It exhibited high catalytic activity and durability during the DRM reaction.

CATALYSTS (2022)

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Article Chemistry, Multidisciplinary

Calculation of absolute Raman scattering cross-sections using vibrational self-consistent field/vibrational configuration interaction wave functions

Jhonatas R. Carvalho et al.

Summary: In this study, the scattering cross-sections, depolarization ratios, and Raman shifts of small molecular systems were analyzed using VSCF and VCI methods. It was found that the VCI method showed larger deviations from experimental values for Raman transition wave-numbers, with better accuracy for C2H2 and C2HD.

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Emerging high-prospect applications in photothermal catalysis

Ana Iglesias-Juez et al.

Current Opinion in Green and Sustainable Chemistry (2022)

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Article Chemistry, Applied

Dry reforming of methane over Pt-Ni/CeO2 catalysts: Effect of the metal composition on the stability

Daniel G. Araiza et al.

Summary: The addition of Pt improved the catalytic activity and stability of nickel-ceria catalysts, while bimetallic Pt-Ni/CeO2 catalysts showed stable performance and higher H-2/CO ratio compared to monometallic samples.

CATALYSIS TODAY (2021)

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Article Energy & Fuels

Valuation of catalytic activity of nickel-zirconia-based catalysts using lanthanum co-support for dry reforming of methane

Radwa A. El-Salamony et al.

Summary: This research investigated the impact of incorporating lanthanum metal in different percentages as a catalytic promoter or cosupport for methane dry reforming. The results showed that using lanthanum as a cosupport had a positive effect on reactants' conversions and H-2 yield, while using it as a promoter led to decreased catalytic performance and H-2/CO ratio.

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Catalytic systems for enhanced carbon dioxide reforming of methane: a review

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Summary: By selecting the active metal, supporting materials, promoters and preparation techniques, improved catalysts of high catalytic performance and stability can be obtained for dry reforming of methane. There is a strong correlation between the support morphology, physicochemical properties and catalytic performances, with fibrous structures showing optimal metal-support interaction and high performance.

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Article Energy & Fuels

Enhanced activity and stability of MgO-promoted Ni/Al2O3 catalyst for dry reforming of methane: Role of MgO

Baitang Jin et al.

Summary: The study deposited highly dispersed nickel nanoparticles on aluminum oxide using atomic layer deposition, and found that the addition of MgO increased the basicity of catalyst surfaces, assisting CO2 adsorption and activation. Although the formation of NiO-MgO solid solution did not improve overall reducibility, the interaction between reduced Ni nanoparticles and MgO inhibited sintering and provided sufficient metal-support interface for CO2 activation, leading to higher methane reforming rates.

FUEL (2021)

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Article Chemistry, Physical

Ni/La2O3 catalysts for dry reforming of methane: Effect of La2O3 synthesis conditions on the structural properties and catalytic performances

M. Grabchenko et al.

Summary: 10 wt% Ni/La2O3 catalysts for dry reforming of methane were synthesized by wetness impregnation of lanthana supports prepared using sol-gel citric method with and without NH3 addition. The Ni-La CA catalyst showed higher catalytic activity at 650 degrees Celsius, while Ni-La CA-NH3 exhibited higher stability under the same temperature and time conditions. After long run tests, both catalysts formed La2O2CO3 phase, but Ni-La CA showed more severe deactivation.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Chemistry, Physical

Recent advances during CH4 dry reforming for syngas production: A mini review

Chunsheng Wang et al.

Summary: This review discusses recent advances in the development of efficient and stable catalysts for methane dry reforming, with a focus on novel materials, advanced characterizations, and improved reaction system compatibility. Crystalline oxide catalysts and new materials demonstrate superior reactivity and stability, while progress in advanced characterizations has led to the establishment of reaction mechanisms. Efforts are also being made to upgrade reaction systems for higher efficiency and milder conditions.

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Enhanced carbon resistance and regenerability in methane partial oxidation to syngas using oxygen vacancy-rich fibrous Pd, Ru and Rh/KCC-1 catalysts

Tan Ji Siang et al.

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Zhige Zhang et al.

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Summary: In this study, a series of Ni/SBA-16-MgO catalysts with varying promoters were tested in the reforming of CH4 with CO2 process. The results showed that the addition of Y and Ce promoters had a positive effect on catalytic activity and stability, while the addition of La had a negative influence.

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Dry reforming of methane for syngas production: A review and assessment of catalyst development and efficacy

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Dry reforming of methane over Ni/MgO-Al2O3 catalysts: Thermodynamic equilibrium analysis and experimental application

Vanessa Rossato Bach et al.

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Dry Reforming of Methane over Ni-Al2O3 and Ni-SiO2 Catalysts: Role of Preparation Methods

S. Dekkar et al.

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Carbon dioxide reforming of methane over MgO-promoted Ni/SiO2 catalysts with tunable Ni particle size

Jie-ying Jing et al.

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Article Chemistry, Physical

Effect of O2 and temperature on the catalytic performance of Ni/Al2O3 and Ni/MgAl2O4 for the dry reforming of methane (DRM)

Puneet Kumar Chaudhary et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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Article Chemistry, Physical

Dry reforming of methane on Ni-Fe-MgO catalysts: Influence of Fe on carbon-resistant property and kinetics

Tingting Zhang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Dry reforming of methane over La2O2CO3-modified Ni/Al2O3 catalysts with moderate metal support interaction

Kang Li et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Thermodynamics

Thermodynamic equilibrium study of altering methane partial oxidation for Fischer-Tropsch synfuel production

T. J. Siang et al.

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Effect of spinel inversion and metal-support interaction on the site activity of Mg-Al-Ox supported Co catalyst for CO2 reforming of CH4

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Effect of Ni-Ta ratio on the catalytic selectivity of fibrous Ni-Ta/ZSM-5 for dry reforming of methane

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C. C. Chong et al.

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APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Nur Fajrina et al.

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