期刊
JOURNAL OF PHYSICS-CONDENSED MATTER
卷 28, 期 32, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-8984/28/32/32LT01
关键词
iridates; spin-orbit coupling materials; free-electron laser science; resonant diffraction; ultra-fast x-ray studies; magnetism
资金
- U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]
- DOE Office of Science [DE-AC02-06CH11357]
We report a time-resolved study of the ultrafast dynamics of the magnetic moments formed by the J(eff) = 1/2 states in Sr2IrO4 by directly probing the localized iridium 5d magnetic state through resonant x-ray diffraction. Using optical pump-hard x-ray probe measurements, two relaxation time scales were determined: a fast fluence-independent relaxation is found to take place on a time scale of 1.5 ps, followed by a slower relaxation on a time scale of 500 ps-1.5 ns.
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