期刊
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS
卷 50, 期 1, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/1361-6455/50/1/013002
关键词
photoelectron spectra; ab initio calculations; above-threshold ionization; electron correlations; giant dipole resonance; multiphoton ionization
资金
- Hamburg Centre of Ultrafast Imaging through the Louise-Johnson Fellowship
The present tutorial provides an overview of the time-dependent configuration interaction singles scheme applied to nonlinear ionization over a broad photon-energy range. The efficient propagation of the wave function and the calculation of photoelectron spectra within this approach are described and demonstrated in various applications. Above-threshold ionization of argon and xenon in the extreme ultraviolet energy range is investigated as an example. A particular focus is put on the xenon 4d giant dipole resonance and the information that nonlinear ionization can provide about resonance substructure. Furthermore, above-threshold ionization is studied in the x-ray regime and the intensity regime, at which multiphoton ionization starts to play a role at hard x-ray photon energies, is identified.
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