期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 7, 期 10, 页码 1845-1851出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpclett.6b00295
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类别
资金
- National Research Foundation of Korea (NRF) - Ministry of Science, ICT AMP
- Future Planning (MSIP) of Korea [NRF-2007-00091, NRF-2011-0031565, NRF-2015M1A2A2056542]
- KRICT core program [KK1602-A01]
- KRICT-SKKU DRC program
Low-temperature-processed perovskite solar cells (PSCs), especially those fabricated on flexible substrates, exhibit device performance that is worse than that of high-temperature-processed PSCs. One of the main reasons for the inferior performance of low-temperature-processed PSCs is the loss of photogenerated electrons in the electron collection layer (ECL) or related interfaces, i.e., indium tin oxide/ECL and ECL/perovskite. Here, we report that tailoring of the energy level and electron transporting ability in oxide ECLs using Zn2SnO4 nanoparticles and quantum dots notably minimizes the loss of photogenerated electrons in the low-temperature-fabricated flexible PSC. The proposed ECL with methylammonium lead halide [MAPb-(I0.9Br0.1)(3)] leads to fabrication of significantly improved flexible PSCs with steady-state power conversion efficiency of 16.0% under AM 1.5G illumination of 100 mW cm(-2) intensity. These results provide an effective method for fabricating high-performance, low-temperature solution-processed flexible PSCs.
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