☆ 4.8 Review

Designing better electrolytes

SCIENCE (2022)

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Article Chemistry, Physical

Suspension electrolyte with modified Li+ solvation environment for lithium metal batteries

Mun Sek Kim et al.

Summary: Designing a suspension electrolyte that modifies the Li+ solvation environment and creates inorganic-rich solid-electrolyte interphases on a Li anode has been achieved in this study. By investigating Li2O nanoparticles suspended in liquid electrolytes, the roles of Li2O in the electrolyte and interphases have been elucidated. The application of the suspension electrolyte design in conventional and advanced electrolytes has demonstrated improved performance and stability.

NATURE MATERIALS (2022)

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Article Chemistry, Multidisciplinary

A sobering examination of the feasibility of aqueous aluminum batteries

Glenn R. Pastel et al.

Summary: This study provides a rigorous examination of aqueous aluminum electrolytes and reveals a dynamic solvation structure around Al3+ cations. However, practical concerns related to the corrosiveness of acidic solutions and the inadequate reductive stability of the proposed electrolytes limit the feasibility of rechargeable aqueous aluminum batteries.

ENERGY & ENVIRONMENTAL SCIENCE (2022)

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Article Materials Science, Multidisciplinary

Solvation Structure and Dynamics of Mg(TFSI)2 Aqueous Electrolyte

Zhou Yu et al.

Summary: Through various simulations and experiments, the study investigates the solvation structure and ion dynamics of magnesium bis(trifluoromethanesulfonyl)imide aqueous electrolyte at different concentrations. The research finds that the first solvation shell of an Mg2+ ion is composed of six water molecules and the ion dynamics and diffusion coefficients are mainly influenced by the formation of ion complexes.

ENERGY & ENVIRONMENTAL MATERIALS (2022)

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Article Multidisciplinary Sciences

A rechargeable zinc-air battery based on zinc peroxide chemistry

Wei Sun et al.

Summary: The study presents a zinc-O-2/zinc peroxide chemistry that operates through a 2e(-)/O-2 process in nonalkaline aqueous electrolytes, allowing highly reversible redox reactions in zinc-air batteries. This innovative ZnO2 chemistry, enabled by water-poor and zinc ion (Zn2+)-rich inner Helmholtz layer, shows superior reversibility and stability compared to alkaline zinc-air batteries.

SCIENCE (2021)

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Editorial Material Chemistry, Physical

Standardized Battery Reporting Guidelines

Alexandra K. Stephan

JOULE (2021)

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Article Chemistry, Physical

High Performance Printed AgO-Zn Rechargeable Battery for Flexible Electronics

Lu Yin et al.

Summary: The study developed printable polymer-based flexible batteries with features such as flexibility, rechargeability, and high capacity, demonstrating superior performance through detailed testing and analysis. These batteries are suitable for various electronic devices and have significant implications for the future development of high-performance flexible batteries.

JOULE (2021)

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Article Multidisciplinary Sciences

Copper-coordinated cellulose ion conductors for solid-state batteries

Chunpeng Yang et al.

Summary: By coordinating copper ions with cellulose nanofibrils, this study has developed a high-performance solid polymer ion conductor with molecular channels that enable rapid lithium ion transport, showing promise for safe, high-performance solid-state batteries. This molecular-channel engineering approach shows high lithium ion conductivity, high transference number, and wide electrochemical stability, with implications for applications beyond batteries.

NATURE (2021)

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Article Nanoscience & Nanotechnology

Identification of LiH and nanocrystalline LiF in the solid-electrolyte interphase of lithium metal anodes

Zulipiya Shadike et al.

Summary: A comprehensive understanding of the solid-electrolyte interphase (SEI) composition is crucial for developing high-energy batteries based on lithium metal anodes. This study used synchrotron-based X-ray diffraction and pair distribution function analysis to identify and differentiate two elusive components, LiH and LiF, in the SEI of lithium metal anodes. The presence of LiH in the SEI was confirmed, with discussion on the possibility of its misidentification as LiF in the literature. The study also found that LiF in the SEI has different structural features from LiF in the bulk phase, which favor Li+ transport and make it a favored component for the SEI.

NATURE NANOTECHNOLOGY (2021)

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Article Multidisciplinary Sciences

Solvation sheath reorganization enables divalent metal batteries with fast interfacial charge transfer kinetics

Singyuk Hou et al.

Summary: Rechargeable magnesium and calcium metal batteries show promise as alternatives to lithium-ion batteries due to their high crustal abundance and capacity. By using a specific family of chelants, researchers were able to greatly improve the interfacial charge transfer kinetics and suppress side reactions, resulting in stable and highly reversible cycling performance for the batteries. This work provides a versatile electrolyte design strategy for divalent metal batteries.

SCIENCE (2021)

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Article Chemistry, Physical

Understanding the Outstanding High-Voltage Performance of NCM523||Graphite Lithium Ion Cells after Elimination of Ethylene Carbonate Solvent from Conventional Electrolyte

Sven Klein et al.

Summary: Increasing the specific energy of lithium ion batteries by raising the cell voltage can lead to rapid capacity fade, which can be prevented by removing ethylene carbonate from the electrolyte. This change in electrolyte composition results in a decrease in transition metal deposits and lithium dendrites, ultimately ensuring a rollover-free performance at high voltage conditions.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

High-Efficiency Zinc-Metal Anode Enabled by Liquefied Gas Electrolytes

Lin Ma et al.

Summary: The use of a liquefied gas electrolyte has shown to improve the performance of rechargeable zinc metal batteries, allowing for highly reversible Zn cycling across a wide temperature range. Furthermore, the formation of a ZnF2-enriched interphase on the anode, resulting from electrolyte decomposition, plays a key role in enhancing battery performance.

ACS ENERGY LETTERS (2021)

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Article Energy & Fuels

Pressure-tailored lithium deposition and dissolution in lithium metal batteries

Chengcheng Fang et al.

Summary: This study presents a high-density Li deposition technique achieved by controlling uniaxial stack pressure to improve the performance of lithium metal batteries, along with proposing a Li morphology testing protocol to maintain the ideal Li deposition morphology. The critical role of stack pressure on Li nucleation, growth, and dissolution processes is elucidated, highlighting the importance of precise control of Li deposition and dissolution.

NATURE ENERGY (2021)

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Article Chemistry, Physical

A Safer, Wide-Temperature Liquefied Gas Electrolyte Based on Difluoromethane

Daniel M. Davies et al.

Summary: In order to address safety and practicality concerns with electrolytes, researchers have demonstrated the enhanced safety features of liquefied gas electrolytes and shown the feasibility of using difluoromethane as a solvent, providing a new direction for their use. Through custom setups and various testing methods, they have proven that this electrolyte has good conductivity over a wide temperature range and compatibility with metal anodes and high-voltage cathodes.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Insight into SEI Growth in Li-Ion Batteries using Molecular Dynamics and Accelerated Chemical Reactions

Lorena Alzate-Vargas et al.

Summary: A classical molecular dynamics simulation protocol is proposed to predict the formation of the solid electrolyte interphase (SEI) in lithium-ion batteries using organic electrolytes. By accelerating the formation of SEI components near the anode surface, the protocol can evaluate the effects of varying electrolyte compositions and additives on SEI layer structure and composition. Gases, inorganic, and organic components are observed during the SEI formation process.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Article Multidisciplinary Sciences

Carbon-free high-loading silicon anodes enabled by sulfide solid electrolytes

Darren H. S. Tan et al.

Summary: The research successfully achieved stable operation of silicon anodes by using the interface passivating properties of sulfide solid electrolytes. Analysis showed that this approach eliminates continuous interfacial growth and irreversible lithium losses. The promising performance of microsilicon full cells can be attributed to the ideal interface properties between microsilicon and sulfide electrolytes and the unique chemomechanical behavior of the lithium-silicon alloy.

SCIENCE (2021)

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Editorial Material Chemistry, Physical

An Experimental Checklist for Reporting Battery Performances

Yang-Kook Sun

ACS ENERGY LETTERS (2021)

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Editorial Material Energy & Fuels

Li-ion battery electrolytes

Kang Xu

Summary: The electrolyte plays a crucial role in any electrochemical device, especially in lithium-ion batteries where its development is closely linked to the evolution of electrode chemistries.

NATURE ENERGY (2021)

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Article Chemistry, Multidisciplinary

Single-ion conducting polymer electrolytes as a key jigsaw piece for next-generation battery applications

Jingyi Gao et al.

Summary: The development of next-generation battery technologies is driven by the increasing demand for energy storage on a larger scale. Efforts to improve safety issues in commercial liquid electrolytes have focused on developing ion-selective polymers. These polymers offer advantages in battery operation, such as minimizing cell polarization and dendrite growth.

CHEMICAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Achievements, Challenges, and Prospects of Calcium Batteries

M. Elena Arroyo-de Dompablo et al.

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Research Development on K-Ion Batteries

Tomooki Hosaka et al.

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Review Chemistry, Multidisciplinary

New Concepts in Electrolytes

Matthew Li et al.

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Review Chemistry, Multidisciplinary

Current Challenges and Routes Forward for Nonaqueous Lithium-Air Batteries

Tao Liu et al.

CHEMICAL REVIEWS (2020)

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Review Chemistry, Multidisciplinary

Mobile Ions in Composite Solids

Zheyi Zou et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Physical

Li2O Solid Electrolyte Interphase: Probing Transport Properties at the Chemical Potential of Lithium

Rui Guo et al.

CHEMISTRY OF MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Effect of Pressure on Lithium Metal Deposition and Stripping against Sulfide-Based Solid Electrolytes

Yuxing Wang et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Review Chemistry, Multidisciplinary

Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes

Abhik Banerjee et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Conventional Electrolyte and Inactive Electrode Materials in Lithium-Ion Batteries: Determining Cumulative Impact of Oxidative Decomposition at High Voltage

Benjamin Streipert et al.

CHEMSUSCHEM (2020)

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Review Energy & Fuels

Current status and future directions of multivalent metal-ion batteries

Yanliang Liang et al.

NATURE ENERGY (2020)

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Article Energy & Fuels

Diagnosing and correcting anode-free cell failure via electrolyte and morphological analysis

A. J. Louli et al.

NATURE ENERGY (2020)

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Article Chemistry, Physical

A Liquid Electrolyte with De-Solvated Lithium Ions for Lithium-Metal Battery

Zhi Chang et al.

JOULE (2020)

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Article Multidisciplinary Sciences

Energy storage emerging: A perspective from the Joint Center for Energy Storage Research

Lynn Trahey et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2020)

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Realizing high zinc reversibility in rechargeable batteries

Lin Ma et al.

NATURE ENERGY (2020)

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Autonomous Discovery of Battery Electrolytes with Robotic Experimentation and Machine Learning

Adarsh Dave et al.

CELL REPORTS PHYSICAL SCIENCE (2020)

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Concentration and velocity profiles in a polymeric lithium-ion battery electrolyte

Hans-Georg Steinruck et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Beyond the concentrated electrolyte: further depleting solvent molecules within a Li+ solvation sheath to stabilize high-energy-density lithium metal batteries

Zhi Chang et al.

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Review Chemistry, Physical

Uncharted Waters: Super-Concentrated Electrolytes

Oleg Borodin et al.

JOULE (2020)

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Review Chemistry, Physical

Mechanical vs. chemical stability of sulphide-based solid-state batteries. Which one is the biggest challenge to tackle? Overview of solid-state batteries and hybrid solid state batteries

Lea Rose Mangani et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Quantifying inactive lithium in lithium metal batteries

Chengcheng Fang et al.

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Identifying the components of the solid-electrolyte interphase in Li-ion batteries

Luning Wang et al.

NATURE CHEMISTRY (2019)

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In situ quantification of interphasial chemistry in Li-ion battery

Tongchao Liu et al.

NATURE NANOTECHNOLOGY (2019)

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Toward a Fundamental Understanding of the Lithium Metal Anode in Solid-State Batteries-An Electrochemo-Mechanical Study on the Garnet-Type Solid Electrolyte Li6.25Al0.25La3Zr3O12

Thorben Krauskopf et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Computational Screening of Cathode Coatings for Solid-State Batteries

Yihan Xiao et al.

JOULE (2019)

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High-Efficiency Lithium-Metal Anode Enabled by Liquefied Gas Electrolytes

Yangyuchen Yang et al.

JOULE (2019)

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Review Energy & Fuels

Status and challenges in enabling the lithium metal electrode for high-energy and low-cost rechargeable batteries

Paul Albertus et al.

NATURE ENERGY (2018)

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High-Voltage Lithium-Metal Batteries Enabled by Localized High-Concentration Electrolytes

Shuru Chen et al.

ADVANCED MATERIALS (2018)

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Vertically Aligned and Continuous Nanoscale Ceramic-Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity

Xiaokun Zhang et al.

NANO LETTERS (2018)

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An artificial interphase enables reversible magnesium chemistry in carbonate electrolytes

Seoung-Bum Son et al.

NATURE CHEMISTRY (2018)

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High energy-density and reversibility of iron fluoride cathode enabled via an intercalation-extrusion reaction

Xiulin Fan et al.

NATURE COMMUNICATIONS (2018)

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Cryo-STEM mapping of solid-liquid interfaces and dendrites in lithium-metal batteries

Michael J. Zachman et al.

NATURE (2018)

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Martin Winter et al.

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Fluorinating Interphases

Chunsheng Wang et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2018)

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Computation-Accelerated Design of Materials and Interfaces for All-Solid-State Lithium-Ion Batteries

Adelaide M. Nolan et al.

JOULE (2018)

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Article Polymer Science

Simulation of local ion transport in lamellar block copolymer electrolytes based on electron micrographs

Mahati Chintapalli et al.

JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS (2017)

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A Guide to Ethylene Carbonate-Free Electrolyte Making for Li-Ion Cells

Lin Ma et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2017)

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Conversion cathodes for rechargeable lithium and lithium-ion batteries

Feixiang Wu et al.

ENERGY & ENVIRONMENTAL SCIENCE (2017)

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New Insights on the Structure of Electrochemically Deposited Lithium Metal and Its Solid Electrolyte Interphases via Cryogenic TEM

Xuefeng Wang et al.

NANO LETTERS (2017)

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Atomic structure of sensitive battery materials and Interfaces revealed by cryo-electron microscopy

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Liquefied gas electrolytes for electrochemical energy storage devices

Cyrus S. Rustomji et al.

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Lithium battery chemistries enabled by solid-state electrolytes

Arumugam Manthiram et al.

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Modeling Insight into Battery Electrolyte Electrochemical Stability and Interfacial Structure Published as part of the Accounts of Chemical Research special issue Energy Storage: Complexities Among Materials and Interfaces at Multiple Length Scales

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Advanced High-Voltage Aqueous Lithium-Ion Battery Enabled by Water-in-Bisalt Electrolyte

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Synergetic Effects of Inorganic Components in Solid Electrolyte Interphase on High Cycle Efficiency of Lithium Ion Batteries

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The structural and chemical origin of the oxygen redox activity in layered and cation-disordered Li-excess cathode materials

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NATURE CHEMISTRY (2016)

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First principles study on electrochemical and chemical stability of solid electrolyte-electrode interfaces in all-solid-state Li-ion batteries

Yizhou Zhu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2016)

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Hydrate-melt electrolytes for high-energy-density aqueous batteries

Yuki Yamada et al.

NATURE ENERGY (2016)

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The Electrolyte Genome project: A big data approach in battery materials discovery

Xiaohui Qu et al.

COMPUTATIONAL MATERIALS SCIENCE (2015)

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New insights into the structure-property relationship of high-voltage electrolyte components for lithium-ion batteries using the pKa value

Dennis Roman Gallus et al.

ELECTROCHIMICA ACTA (2015)

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Accelerating Electrolyte Discovery for Energy Storage with High-Throughput Screening

Lei Cheng et al.

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An ultrafast rechargeable aluminium-ion battery

Meng-Chang Lin et al.

NATURE (2015)

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Water-in-salt electrolyte enables high-voltage aqueous lithium-ion chemistries

Liumin Suo et al.

SCIENCE (2015)

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Review Chemistry, Multidisciplinary

Recent advances in the electrolytes for interfacial stability of high-voltage cathodes in lithium-ion batteries

Nam-Soon Choi et al.

RSC ADVANCES (2015)

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Review Chemistry, Multidisciplinary

Electrolytes and Interphases in Li-Ion Batteries and Beyond

Kang Xu

CHEMICAL REVIEWS (2014)

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Alloy Negative Electrodes for Li-Ion Batteries

M. N. Obrovac et al.

CHEMICAL REVIEWS (2014)

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Review Chemistry, Multidisciplinary

Rechargeable Lithium-Sulfur Batteries

Arumugam Manthiram et al.

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Research Development on Sodium-Ion Batteries

Naoaki Yabuuchi et al.

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Lithium metal anodes for rechargeable batteries

Wu Xu et al.

ENERGY & ENVIRONMENTAL SCIENCE (2014)

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Stable lithium electrodeposition in liquid and nanoporous solid electrolytes

Yingying Lu et al.

NATURE MATERIALS (2014)

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Solvation structure and energetics of electrolytes for multivalent energy storage

Saul H. Lapidus et al.

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Understanding Li+-Solvent Interaction in Nonaqueous Carbonate Electrolytes with 17O NMR

Xavier Bogle et al.

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Electrolyte roadblocks to a magnesium rechargeable battery

John Muldoon et al.

ENERGY & ENVIRONMENTAL SCIENCE (2012)

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Nanostructured high-energy cathode materials for advanced lithium batteries

Yang-Kook Sun et al.

NATURE MATERIALS (2012)

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Preferential Solvation of Li+ Directs Formation of Interphase on Graphitic Anode

Arthur von Cresce et al.

ELECTROCHEMICAL AND SOLID STATE LETTERS (2011)

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Article Electrochemistry

Electrolyte Additive in Support of 5 V Li Ion Chemistry

Arthur von Cresce et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2011)

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Review Chemistry, Physical

Challenges for Rechargeable Li Batteries

John B. Goodenough et al.

CHEMISTRY OF MATERIALS (2010)

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Aging of the LiNi1/2Mn1/2O2 Positive Electrode Interface in Electrolyte

Nicolas Dupre et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2009)

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Article Chemistry, Physical

The Solid Electrolyte Interphase - The Most Important and the Least Understood Solid Electrolyte in Rechargeable Li Batteries

Martin Winter

ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS (2009)

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Article Electrochemistry

Identification of the source of evolved gas in Li-ion batteries using C-13-labeled solvents

Masamichi Onuki et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2008)

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High-performance lithium battery anodes using silicon nanowires

Candace K. Chan et al.

NATURE NANOTECHNOLOGY (2008)

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Solvation sheath of Li+ in nonaqueous electrolytes and its implication of graphite/electrolyte interface chemistry

Kang Xu et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2007)

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Review Chemistry, Physical

Nano- and bulk-silicon-based insertion anodes for lithium-ion secondary cells

Uday Kasavajjula et al.

JOURNAL OF POWER SOURCES (2007)

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Article Multidisciplinary Sciences

Anomalous increase in carbon capacitance at pore sizes less than 1 nanometer

J. Chmiola et al.

SCIENCE (2006)

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Article Chemistry, Physical

Lithium ethylene dicarbonate identified as the primary product of chemical and electrochemical reduction of EC in 1.2 m LiPF6/EC:EMC electrolyte

GRV Zhuang et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2005)

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Article Electrochemistry

Film formation at positive electrodes in lithium-ion batteries

A Wursig et al.

ELECTROCHEMICAL AND SOLID STATE LETTERS (2005)

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Molecular dynamics simulations of multicomponent diffusion. 1. Equilibrium method

DR Wheeler et al.

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Nonaqueous liquid electrolytes for lithium-based rechargeable batteries

K Xu

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