On-line measurement for velocity and particle size distribution of flowing aerosol by dynamic light scattering

In the dynamic light scattering (DLS) measurement for a flowing aerosol, an anemometer, is needed to measure the flow velocity to invert the aerosol particle size. In this work, a cumulative analysis method has been used to obtain the aerosol velocity through the light intensity autocorrelation function (ACF) based on the relation between the particle velocity and the second cumulant of the electric field ACF of flowing aerosol particles. Additionally, the particle size distribution (PSD) has been inversed by the regularization method, which enables the online measurement of flowing aerosol to be realized. The simulation results at different noise levels show that the accurate velocity and PSD for flowing aerosols can be obtained by the proposed method at low noise levels and high noise levels. It has been observed that higher noise causes the PSD broadening and the peak offset. For aerosol particles with a bimodal distribution, the increase of noise leads to the increase of peak height ratio and peak of small particles in bimodal distribution disappears, leaving only unimodal distribution. Furthermore, the increase of noise has no significant effect on the calculated velocity value both for unimodal and bimodal aerosol distributions. The experimental results of DLS measurements on unimodal and bimodal aerosols verified the above statements.

Automated summary

In this study, a method has been proposed to obtain the velocity and particle size distribution of flowing aerosols through the analysis of light intensity autocorrelation function (ACF) and the application of regularization method. The results from simulations and experiments demonstrate that the proposed method can accurately measure the velocity and particle size distribution of flowing aerosols under different noise levels.