4.3 Article

AMS measurements of 14C, 36Cl, and 239/240Pu samples taken in a 'small facility'

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ELSEVIER
DOI: 10.1016/j.nimb.2022.10.025

关键词

Accelerator mass spectrometry; AMS; Decommissioning; 14C; 36Cl; 239Pu; 240Pu

资金

  1. German Federal Ministry for the Environment, Nature Conservation, Nuclear Safety and Consumer Protection [4719E03510]
  2. German Federal Ministry of Education and Research [15S9410B]

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In this study, a radiochemistry laboratory in Cologne, Germany was chosen as a case study to investigate the release of nuclear facilities from regulatory control. Measurements of the samples showed elevated values of C-14 and Cl-36, but below the release values. It was confirmed that these elements were openly handled in the laboratory.
The release of nuclear facilities from regulatory control is commonly addressed by demonstrating that con-taminations are below 'clearance values'. AMS is commonly too laborious for a large number of samples, especially if nuclide vectors have been established, but it might be of interest for the release of a so-called 'small facility'. For this case study, a radiochemistry laboratory in Cologne, Germany was chosen. It was known that C-14, Cl-36 as well as 240Pu had been handled openly in this lab. There were no apparent contaminations, i.e., no alpha/beta contaminations that could be detected using a hand-held radiation monitor. Elevated values of C-14 were measured in three, increased values of Cl-36 in all and Pu-239 in only one of the examined samples. All measured activities are well below the release values, but it can be proven that the elements C-14, Cl-36, Pu-239 were handled openly in the 'small facility'.

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