4.6 Article

Two-Dimensional Structures Formed by Triblock Patchy Particles with Two Different Patches

期刊

LANGMUIR
卷 38, 期 49, 页码 15404-15412

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.2c02699

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资金

  1. JSPS KAKENHI [JP20K03782, 21K04908]
  2. Grant for Joint Research Program of the Institute of Low Temperature Science, Hokkaido University [22G015]

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We examined two-dimensional structures formed by spherical triblock patchy particles through Monte Carlo simulations. Different structures, such as kagome lattices, hexagonal structures, two-dimensional dodecagonal quasi-crystal structures, and chain-like structures, were observed by varying the patch sizes, pressure, and interaction energy.
Two-dimensional structures formed by spherical triblock patchy particles are examined by performing Monte Carlo simulations. In the model, the triblock patchy particles have two different types of patches at the polar positions. The patch sizes are different from each other, and the attractive interaction acts only between the same types of patches. The particles translate on a flat plane and rotate three-dimensionally. When varying the two patch sizes, the pressure, and interaction energy, various structures are observed. When the difference between two patch sizes is small, kagome lattices, hexagonal structures, and two-dimensional dodecagonal quasi-crystal structures are observed. When the difference between two patch sizes is large, chain-like structures are created. With lower temperature, sparse structures such as ring-like structures form.

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