☆ 4.8 Article

On the Trail of Molecular Hydrophilicity and Hydrophobicity at Aqueous Interfaces

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2023)

相关参考文献

注意：仅列出部分参考文献，下载原文获取全部文献信息。

Review Chemistry, Physical

Vibrational Dynamics at Aqueous-Mineral Interfaces

Stefan M. Piontek et al.

Summary: The dynamics of water at mineral surfaces have attracted significant attention due to the differences in the ability of interfacial water populations to redistribute vibrational energy compared to the bulk water. However, there are still many unanswered questions regarding these systems. In this review, the evolution of our understanding and the current state-of-the-art interpretation for three important mineral/water interfaces are discussed. Vibrational dynamics provide unique insights into interfacial structure that may be missed by traditional static vibrational spectroscopy.

JOURNAL OF PHYSICAL CHEMISTRY C (2022)

添加到收藏夹

Article Chemistry, Physical

Mechanism and Free-Energy Landscape of Peptide Bond Formation at the Silica-Water Interface

Flavio Siro Brigiano et al.

Summary: This study investigates the mechanism of peptide bond formation over a silica surface in an aqueous environment, revealing a strong catalytic effect of the interface on the reaction.

ACS CATALYSIS (2022)

添加到收藏夹

Review Chemistry, Multidisciplinary

Probing the Mineral-Water Interface with Nonlinear Optical Spectroscopy

Ellen H. G. Backus et al.

Summary: The interaction between minerals and water is influenced by various factors, prompting researchers to conduct molecular-level studies to uncover the complexity of these processes.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

添加到收藏夹

Article Chemistry, Physical

Anomalously Low Dielectric Constant of Ordered Interfacial Water

Chonghai Qi et al.

Summary: This study reveals that the parallel dielectric constant at the solid/water interface is influenced by solid-water interactions and the water structure on different solid crystal faces. Ordered water structures can significantly reduce the parallel dielectric constant at the interface, attributed to the specific antiferroelectric ordered structure of interfacial water molecules.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

添加到收藏夹

Article Multidisciplinary Sciences

Stripping away ion hydration shells in electrical double-layer formation: Water networks matter

Serena R. Alfarano et al.

Summary: The study combines experiments and simulations to provide a molecular picture of double-layer formation under applied voltage, showing the stripping away of cation/anion hydration shells for an NaCl electrolyte at the Au surface at varying bias potentials. Results indicate that Na+ is attracted towards the electrode at the smallest negative potentials, while stripping of the Cl- hydration shell occurs only at higher potential values. The phenomena are measured directly by THz spectroscopy using ultrabright synchrotron light and rationalized by molecular dynamics simulations and electronic-structure calculations.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

添加到收藏夹

Article Multidisciplinary Sciences

Identifying hydrophobic protein patches to inform protein interaction interfaces

Nicholas B. Rego et al.

Summary: By using specialized molecular simulations, researchers have identified the most hydrophobic protein patches and found a strong correlation between these patches and regions responsible for mediating protein interactions. This study helps to better understand the functionality and interaction patterns of proteins.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

添加到收藏夹

Article Chemistry, Physical

Molecular Fingerprints of Hydrophobicity at Aqueous Interfaces from Theory and Vibrational Spectroscopies

Simone Pezzotti et al.

Summary: The hydrophobicity/hydrophilicity of aqueous interfaces is influenced by a delicate balance between water-water and water-surface interactions. Through DFT-MD, SFG, and THz-IR absorption spectroscopies, it has been shown that water at interfaces forms a two-dimensional hydrogen-bonded network, revealing the competition between water-surface and water-water interactions. Combining SFG and THz-IR spectroscopies provides a powerful tool for characterizing molecular hydrophobicity at aqueous interfaces.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

添加到收藏夹

Article Multidisciplinary Sciences

Size dependence of hydrophobic hydration at electrified gold/water interfaces

Alessandra Serva et al.

Summary: Hydrophobic hydration at the metal/water interface is studied using constant applied potential molecular dynamics in this work. The study proposes an adaptation of the Lum-Chandler-Weeks theory to describe the free energy of hydrophobic hydration at the interface, showing a preference for outer-sphere adsorption of small hydrophobic solutes at the gold surface and higher free energy cost for hydrating larger hydrophobes at the interface compared to the bulk.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2021)

添加到收藏夹

Article Chemistry, Multidisciplinary

Wettability of graphene and interfacial water structure

Donghwan Kim et al.

Summary: The study utilized vibrational sum-frequency-generation spectroscopy to elucidate the water structure at a water-graphene interface. The observation of an excellent correlation between water adhesion energy of graphene and the fraction of dangling OH groups suggests that VSFG can be an incisive technique for measuring water's adhesion energy on spatially confined interfaces. The results are anticipated to aid in understanding the wettability of low-dimensional materials.

CHEM (2021)

添加到收藏夹

Article Multidisciplinary Sciences

Asymmetric response of interfacial water to applied electric fields

Angelo Montenegro et al.

Summary: This experimental study reveals that the dielectric response of interfacial water may deviate from linear response, challenging the traditional view of treating interfacial water as a simple dielectric medium. Vibrational sum-frequency generation spectra show significant asymmetry for negative versus neutral/positive electrode charge conditions.

NATURE (2021)

添加到收藏夹

Article Chemistry, Multidisciplinary

Local Mutations Can Serve as a Game Changer for Global Protein Solvent Interaction

Ellen M. Adams et al.

Summary: Research has shown that local mutations not only affect the local properties of proteins, but also have a global impact, especially on the dynamics of water molecules near the protein surface, which in turn affects protein stability. The solvent contribution can be experimentally probed via terahertz spectroscopy, opening up new possibilities for rational protein design.

JACS AU (2021)

添加到收藏夹

Article Chemistry, Multidisciplinary

A molecular twist on hydrophobicity

Sara Gomez et al.

Summary: This study comprehensively explores the molecular basis for hydrophobicity using theoretical tools and organic solvent S/water binary systems, revealing no evidence of repulsion between water and S molecules, but rather a complex interplay of entropic, enthalpic, and dynamic factors maintaining stable water interfaces.

CHEMICAL SCIENCE (2021)

添加到收藏夹

Review Chemistry, Multidisciplinary

Recent Advances in Electrocatalytic Hydrogen Evolution Using Nanoparticles

Jing Zhu et al.

CHEMICAL REVIEWS (2020)

添加到收藏夹

Review Chemistry, Multidisciplinary

Molecular Structure and Modeling of Water-Air and Ice-Air Interfaces Monitored by Sum-Frequency Generation

Fujie Tang et al.

CHEMICAL REVIEWS (2020)

添加到收藏夹

Article Chemistry, Physical

Water Structure, Dynamics, and Sum-Frequency Generation Spectra at Electrified Graphene Interfaces

Yiwei Zhang et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

添加到收藏夹

Article Chemistry, Applied

Water Structure and Properties at Hydrophilic and Hydrophobic Surfaces

Jacob Monroe et al.

Annual Review of Chemical and Biomolecular Engineering (2020)

添加到收藏夹

Article Chemistry, Multidisciplinary

Ions Tune Interfacial Water Structure and Modulate Hydrophobic Interactions at Silica Surfaces

Aashish Tuladhar et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

添加到收藏夹

Article Chemistry, Physical

Heterodyne-detected sum frequency generation of water at surfaces with varying hydrophobicity

Stephanie E. Sanders et al.

JOURNAL OF CHEMICAL PHYSICS (2019)

添加到收藏夹

Article Chemistry, Physical

Effect of Functional and Electron Correlation on the Structure and Spectroscopy of the Al2O3(001)-H2O Interface

Mark J. DelloStritto et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

添加到收藏夹

Article Multidisciplinary Sciences

Versatile electrification of two-dimensional nanomaterials in water

Benoit Grosjean et al.

NATURE COMMUNICATIONS (2019)

添加到收藏夹

Article Chemistry, Physical

Spatially Heterogeneous Water Properties at Disordered Surfaces Decrease the Hydrophobicity of Nonpolar Self-Assembled Monolayers

Bradley C. Dallin et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

添加到收藏夹

Article Chemistry, Physical

Gate-Controlled Sum-Frequency Vibrational Spectroscopy for Probing Charged Oxide/Water Interfaces

Hongqing Wang et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2019)

添加到收藏夹

Article Multidisciplinary Sciences

Molecular hydrophobicity at a macroscopically hydrophilic surface

Jenee D. Cyran et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2019)

添加到收藏夹

Article Chemistry, Physical

Deconvolution of BIL-SFG and DL-SFG spectroscopic signals reveals order/disorder of water at the elusive aqueous silica interface

Simone Pezzotti et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2019)

添加到收藏夹

Article Chemistry, Physical

Characterizing Hydration Properties Based on the Orientational Structure of Interfacial Water Molecules

Sucheol Shin et al.

JOURNAL OF CHEMICAL THEORY AND COMPUTATION (2018)

添加到收藏夹

Article Chemistry, Physical

The Topmost Water Structure at a Charged Silica/Aqueous Interface Revealed by Heterodyne-Detected Vibrational Sum Frequency Generation Spectroscopy

Shu-hei Urashima et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2018)

添加到收藏夹

Article Chemistry, Physical

Structural definition of the BIL and DL: a new universal methodology to rationalize non-linear chi((2))(omega) SFG signals at charged interfaces, including chi((3))(omega) contributions

Simone Pezzotti et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2018)

添加到收藏夹

Article Chemistry, Physical

Effects of third-order susceptibility in sum frequency generation spectra: a molecular dynamics study in liquid water

Tatsuya Joutsuka et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2018)

添加到收藏夹

Article Chemistry, Physical

Relating Interfacial Order to Sum Frequency Generation with Ab Initio Simulations of the Aqueous Al2O3(0001) and (11(2)over-bar0) Interfaces

Mark DelloStritto et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2018)

添加到收藏夹

Article Multidisciplinary Sciences

Computational discovery of chemically patterned surfaces that effect unique hydration water dynamics

Jacob I. Monroe et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2018)

添加到收藏夹

Article Geochemistry & Geophysics

What the Diffuse Layer (DL) Reveals in Non-Linear SFG Spectroscopy

Simone Pezzotti et al.

MINERALS (2018)

添加到收藏夹

Article Environmental Sciences

Spectroscopic BIL-SFG Invariance Hides the Chaotropic Effect of Protons at the Air-Water Interface

Simone Pezzotti et al.

ATMOSPHERE (2018)

添加到收藏夹

Article Chemistry, Physical

The excess proton at the air-water interface: The role of instantaneous liquid interfaces

Federico Giberti et al.

JOURNAL OF CHEMICAL PHYSICS (2017)

添加到收藏夹

Article Chemistry, Physical

2D H-Bond Network as the Topmost Skin to the Air-Water Interface

Simone Pezzotti et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2017)

添加到收藏夹

Article Chemistry, Physical

The elusive silica/water interface: isolated silanols under water as revealed by vibrational sum frequency spectroscopy

Laetitia Dalstein et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2017)

添加到收藏夹

Article Multidisciplinary Sciences

Hydrophobicity of proteins and nanostructured solutes is governed by topographical and chemical context

Erte Xi et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2017)

添加到收藏夹

Article Physics, Multidisciplinary

Unveiling Microscopic Structures of Charged Water Interfaces by Surface-Specific Vibrational Spectroscopy

Yu-Chieh Wen et al.

PHYSICAL REVIEW LETTERS (2016)

添加到收藏夹

Article Multidisciplinary Sciences

Water orientation and hydrogen-bond structure at the fluorite/water interface

Remi Khatib et al.

SCIENTIFIC REPORTS (2016)

添加到收藏夹

Article Chemistry, Multidisciplinary

Aqueous Heterogeneity at the Air/Water Interface Revealed by 2D-HD-SFG Spectroscopy

Cho-Shuen Hsieh et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2014)

添加到收藏夹

Review Chemistry, Physical

Recent progress on sum-frequency spectroscopy

C. S. Tian et al.

SURFACE SCIENCE REPORTS (2014)

添加到收藏夹

Article Chemistry, Multidisciplinary

CP2K: atomistic simulations of condensed matter systems

Juerg Hutter et al.

WILEY INTERDISCIPLINARY REVIEWS-COMPUTATIONAL MOLECULAR SCIENCE (2014)

添加到收藏夹

Article Multidisciplinary Sciences

Hydration of metal surfaces can be dynamically heterogeneous and hydrophobic

David T. Limmer et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2013)

添加到收藏夹

Review Chemistry, Physical

Environmental Chemistry at Vapor/Water Interfaces: Insights from Vibrational Sum Frequency Generation Spectroscopy

Aaron M. Jubb et al.

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 63 (2012)

添加到收藏夹

Article Chemistry, Physical

The Silica-Water Interface: How the Silanols Determine the Surface Acidity and Modulate the Water Properties

Marialore Sulpizi et al.

JOURNAL OF CHEMICAL THEORY AND COMPUTATION (2012)

添加到收藏夹

Article Chemistry, Multidisciplinary

Ultrafast vibrational energy transfer at the water/air interface revealed by two-dimensional surface vibrational spectroscopy

Zhen Zhang et al.

NATURE CHEMISTRY (2011)

添加到收藏夹

Review Chemistry, Applied

Hydrophobicity of Proteins and Interfaces: Insights from Density Fluctuations

Sumanth N. Jamadagni et al.

ANNUAL REVIEW OF CHEMICAL AND BIOMOLECULAR ENGINEERING, VOL 2 (2011)

添加到收藏夹

Article Chemistry, Physical

Mapping hydrophobicity at the nanoscale: Applications to heterogeneous surfaces and proteins

Hari Acharya et al.

FARADAY DISCUSSIONS (2010)

添加到收藏夹

Article Chemistry, Physical

Fluctuations of Water near Extended Hydrophobic and Hydrophilic Surfaces

Amish J. Patel et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2010)

添加到收藏夹

Article Chemistry, Physical

Instantaneous Liquid Interfaces

Adam P. Willard et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2010)

添加到收藏夹

Article Chemistry, Multidisciplinary

Effect of Hydrogen-Bond Strength on the Vibrational Relaxation of Interfacial Water

Ali Eftekhari-Bafrooei et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2010)

添加到收藏夹

Article Chemistry, Physical

Probing the microscopic hydrophobicity of smectite surfaces. A vibrational spectroscopic study of dibenzo-p-dioxin sorption to smectite

Kiran Rana et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2009)

添加到收藏夹

Article Multidisciplinary Sciences

Characterizing hydrophobicity of interfaces by using cavity formation, solute binding, and water correlations

Rahul Godawat et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2009)

添加到收藏夹

Article Multidisciplinary Sciences

Structure and charging of hydrophobic material/water interfaces studied by phase-sensitive sum-frequency vibrational spectroscopy

C. S. Tian et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2009)

添加到收藏夹

Article Chemistry, Multidisciplinary

Realistic Models of Hydroxylated Amorphous Silica Surfaces and MCM-41 Mesoporous Material Simulated by Large-scale Periodic B3LYP Calculations

P. Ugliengo et al.

ADVANCED MATERIALS (2008)

添加到收藏夹

Article Chemistry, Physical

Recent progress in theoretical analysis of vibrational sum frequency generation spectroscopy

Akihiro Morita et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2008)

添加到收藏夹

Article Multidisciplinary Sciences

Hydrophobic interaction and hydrogen-bond network for a methane pair in liquid water

Je-Luen Li et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2007)

添加到收藏夹

Article Chemistry, Physical

Hydration behavior under confinement by nanoscale surfaces with patterned hydrophobicity and hydrophilicity

Nicolas Giovambattista et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2007)

添加到收藏夹

Article Chemistry, Multidisciplinary

Semiempirical GGA-type density functional constructed with a long-range dispersion correction

Stefan Grimme

JOURNAL OF COMPUTATIONAL CHEMISTRY (2006)

添加到收藏夹

Article Computer Science, Interdisciplinary Applications

QUICKSTEP: Fast and accurate density functional calculations using a mixed Gaussian and plane waves approach

J VandeVondele et al.

COMPUTER PHYSICS COMMUNICATIONS (2005)

添加到收藏夹

Article Chemistry, Multidisciplinary

Accurate description of van der Waals complexes by density functional theory including empirical corrections

S Grimme

JOURNAL OF COMPUTATIONAL CHEMISTRY (2004)

添加到收藏夹

Article Chemistry, Physical

A theoretical analysis of the sum frequency generation spectrum of the water surface. II. Time-dependent approach

A Morita et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2002)

添加到收藏夹

Article Chemistry, Physical

Sum frequency generation (SFG) study of the pH-dependent water structure on a fused quartz surface modified by an octadecyltrichlorosilane (OTS) monolayer

S Ye et al.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2001)

添加到收藏夹

Article Chemistry, Physical

The solvation of Na+ in water:: First-principles simulations

JA White et al.

JOURNAL OF CHEMICAL PHYSICS (2000)

添加到收藏夹

© Peeref 2019-2024. All rights reserved.