4.7 Article

Pre-strain accommodation enabled multi-dimensionally and hierarchically elastomeric MoSe2/MXene and AC/MXene electrodes for stretchable sodium ion capacitors

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JOURNAL OF ALLOYS AND COMPOUNDS
卷 935, 期 -, 页码 -

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ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2022.168065

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Pre-strain; Multi-dimensionally; Elastomeric composite electrode; Stretchable; Sodium ion capacitors

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In this study, stretchable sodium ion capacitors (S-SICs) based on multi-dimensionally and hierarchically elastomeric composite electrodes and stretchable high voltage gel polymer electrolyte were developed. The S-SICs demonstrated high energy/power densities, good stretchability, and stability.
Stretchable supercapacitors with simultaneously high energy/power densities and long life can enrich in-tegrated power options for ever-increasing wearable electronics. However, supercapacitors with high electrochemical performances while maintaining high stretchability are still challenging. Herein, we report stretchable sodium ion capacitors (S-SICs) based on multi-dimensionally and hierarchically elastomeric composite electrodes, and stretchable high voltage gel polymer electrolyte (3.0 V). The elastomeric com-posite electrode is constructed by stretchable 3D electrospun polyurethane (PU) fibrous mat and conductive 1D Ag nanowire network. 2D MoSe2/MXene and 3D AC/MXene as anodic and cathodic materials are em-bedded in this conductive and stretchable mat. This hierarchical structure enables multi-dimensional conductive connections under tensile condition. The pre-strain treatment on PU fibrous mat further in-creases the relatively stretching distance before losing conductive connection among hierarchical compo-nents. The electrodes exhibit superior sodium ion storage performances (420 mAh g(-1) at 5 A g(-1)), as well as good stretchability and stability (95% after 1000 cycles at 2 A g(-1)). Based on this, the S-SICs with high operating voltage demonstrate high energy/power densities (max. 5.44 mWh cm(-3), 493.55 mW cm(-3)) and good stretchability. This prototypical exhibition of S-SICs indicates a promising design direction of stretchable supercapacitors with high electrochemical performances and tolerance of stretchability. (c) 2022 Elsevier B.V. All rights reserved.

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