Three-dimensional SnCu scaffold with layered porous structure enable dendrite-free anode of lithium metal batteries

Article Nanoscience & Nanotechnology

In Situ Constructing a Stable Solid Electrolyte Interface by Multifunctional Electrolyte Additive to Stabilize Lithium Metal Anodes for Li-S Batteries

Mou-Zhi Huang et al.

Summary: In this study, a new method is proposed to achieve a uniform and dendrite-free Li anode for improved performance of Li-S batteries.

ACS APPLIED MATERIALS & INTERFACES (2022)

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Article Materials Science, Multidisciplinary

Constructing a composite lithium anode for high-performance solid-state lithium-metal batteries via in-situ alloying reaction

Jie Wei et al.

Summary: This research proposes a method to construct a composite lithium metal anode, which effectively improves the contact issue and volume stability of solid-state lithium metal batteries, reduces the interfacial resistance, and exhibits excellent cycling and rate performance.

FUNCTIONAL MATERIALS LETTERS (2022)

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Article Chemistry, Analytical

Synthesis of 3D graphitic carbon foams via pressurized pyrolysis of Victorian brown coal as anode material for Li-ion battery

Rou Wang et al.

Summary: This study explores the use of Victorian brown coal for carbon foam preparation and its application in LIBs, showing that tailored treatment methods can significantly enhance battery performance.

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS (2022)

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Article Chemistry, Applied

Self-assembled, highly-lithiophilic and well-aligned biomass engineered MXene paper enables dendrite-free lithium metal anode in carbonate-based electrolyte

Liwen Tan et al.

Summary: A dendrite-free composite Li metal anode has been achieved using a flexible, freestanding, well-aligned, and highly-lithiophilic MXene paper. The MX@CS paper with a micro-crumpled surface effectively decreases the local current density, guides even Li plating, and suppresses dendritic Li growth. The surface-adsorbed chitosan enhances lithiophilicity and reduces Li nucleation overpotential. The dendrite-free Li morphology of the MX@CS-Li anode results in significantly improved cycling life and high Coulombic efficiency.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Engineering, Environmental

Gradient trilayer solid-state electrolyte with excellent interface compatibility for high-voltage lithium batteries

Fang Liu et al.

Summary: This study presents a novel strategy to enhance solid-state lithium-metal batteries by designing a unique gradient trilayer solid-state electrolyte. The gradient trilayer electrolyte improves the compatibility of interfaces and provides continuous Li+ transport channels, leading to stable operation and high capacity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Composites

High safety and electrochemical performance electrospun para-aramid nanofiber composite separator for lithium-ion battery

Wei Tang et al.

Summary: A porous composite membrane based on ANFs and PEO was successfully prepared and applied as a separator for LIBs. The ANFs/PEO separator exhibited excellent morphology, high porosity, thermal stability, and better electrochemical performance compared to the Celgard 2400 separator.

COMPOSITES SCIENCE AND TECHNOLOGY (2022)

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Article Electrochemistry

Flexible 3D porous boron nitride interconnected network as a high-performance Li-and Na-ion battery electrodes

Nabil Khossossi et al.

Summary: To achieve high-efficiency electrochemical energy storage, the battery anode needs to be electronically and ionically conductive. Recent research has found that three-dimensional porous materials composed of carbon and/or boron have great potential for lithium/sodium-ion batteries. This study explores the 3D porous boron nitride network, which exhibits stability, high specific capacity, fast ion diffusion, and other desirable characteristics for battery anodes.

ELECTROCHIMICA ACTA (2022)

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Review Chemistry, Multidisciplinary

Recent Developments in Dendrite-Free Lithium-Metal Deposition through Tailoring of Micro- and Nanoscale Artificial Coatings

Melissa L. Meyerson et al.

Summary: Forty years after the failed introduction of rechargeable lithium-metal batteries and 30 years after the successful commercialization of the lower capacity, graphite-anode based lithium-ion battery by Sony, demand for higher energy density batteries is leading to reinvestigation of the problem of dendrite growth that makes the metallic lithium anodes unsafe. One strategy to mitigate dendrite growth is to deposit thin, tailored, corrosion-passivating coatings on the metallic lithium, instead of allowing the metal to spontaneously react with the organic electrolyte solution to form its passivating solid electrolyte interface (SEI).

ACS NANO (2021)

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Article Chemistry, Physical

Structural Evolution upon Delithiation/Lithiation in Prelithiated Foil Anodes: A Case Study of AgLi Alloys with High Li Utilization and Marginal Volume Variation

Xuan Wu et al.

Summary: This study investigates the structural evolution and stability of nanoporous materials in lithium-ion batteries using Li-Ag composites as a case study. The results show that the rationally designed nanoporous AgLi framework can achieve dendrite-free anodes with stable electrochemical performance.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Artificial Single-Ion Conducting Polymer Solid Electrolyte Interphase Layer toward Highly Stable Lithium Anode

Jianwei Zhang et al.

Summary: By designing a single ion conducting artificial polymer SEI layer on the surface of the Li anode, this study effectively improves lithium batteries' performance, facilitates uniform Li deposition, suppresses dendrite growth, reduces side reactions, and extends battery lifespan.

ACS APPLIED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Elevated Lithium Ion Regulation by a Natural Silk Modified Separator for High-Performance Lithium Metal Anode

Xiang Li et al.

Summary: This research developed a functional modification layer from a derivant of natural silk to protect the lithium anode, offering abundant functional group sites for efficient uniform Li-ion flux and in situ formation of a Li3N-rich solid electrolyte interphase film. The high-performance lithium metal anode achieved dendrite-free morphology and significantly enhanced cycle stability, showing long-term cycling stability of 3000 cycles when paired with LiFePO4 cathodes and over 400 cycles with sulfur cathodes. This study provides a facile and practical approach for interface modification of the high-performance lithium anode and explores the application of biomass-based materials in advanced batteries.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Scalable slurry-coating induced integrated 3D lithiophilic architecture for stable lithium metal anodes

Jiaming Zhang et al.

Summary: The 3D MNCu/FC structure promotes charge transfer, inhibits Li dendrite growth, and regulates uniform Li nucleation and deposition, leading to a dendrite-free lithium metal anode with enhanced electrochemical performance.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Multidisciplinary

Design of Robust, Lithiophilic, and Flexible Inorganic-Polymer Protective Layer by Separator Engineering Enables Dendrite-Free Lithium Metal Batteries with LiNi0.8Mn0.1Co0.1O2 Cathode

Liwen Tan et al.

Summary: The development of a protective layer composed of lithiated SiO and polyacrylate acid on the Li metal anode enables dendrite-free Li deposition, leading to enhanced cycling stability and coulombic efficiency in Li||Li and Cu||Li cells. This technology also significantly extends the lifespan of full cells with a composite separator in carbonate-based electrolytes.

SMALL (2021)

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Article Energy & Fuels

Rejuvenating dead lithium supply in lithium metal anodes by iodine redox

Chengbin Jin et al.

Summary: The researchers use an iodic species to react with inactive lithium, bringing it back to life and thus making batteries last longer.

NATURE ENERGY (2021)

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Article Chemistry, Applied

Synthetic poly-dioxolane as universal solid electrolyte interphase for stable lithium metal anodes

Tao Chen et al.

Summary: A new synthetic poly-dioxolane (PDOL) approach was successfully used to construct an artificial 'elastic' solid electrolyte interface (SEI) layer, stabilizing the Li/electrolyte interface and improving Li deposition/dissolution behavior. This strategy effectively reduces dendrite formation during Li deposition, decreases interfacial side reactions, and enhances cycling performance of the batteries.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Applied

Circumventing chemo-mechanical failure of Sn foil battery anode by grain refinement and elaborate porosity design

Shuibin Tu et al.

Summary: By reducing grain size and designing elaborate porosity, a three-dimensional interconnected porous Sn (3DIP-Sn) foil was proposed to improve the electrochemical performance of Sn foil anodes. Experimental results showed enhanced structure stability of the 3DIP-Sn foil and demonstrated long cycle lifespan, high reversible capacity, and stable cycling performance.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Engineering, Environmental

Controllable lithium deposition behavior hollow of N, O co-doped carbon nanospheres for practical lithium metal batteries

Chunhui Gao et al.

Summary: The study showed that a hollow N, O co-doped carbon nanosphere (NOCS) as a current collector for Li metal anode can improve the cycling performance of Li-based batteries and reduce dendritic growth. Using N, O-doped carbon nanospheres as a current collector can enhance the uniformity of Li deposition and Coulombic efficiency, leading to longer cycle life and more stable performance. Additionally, the Li@NOCS parallel to LiFePO4 full cells demonstrated excellent cycling and rate performance compared to Li@Cu parallel to LiFePO4 full cells.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Physical

Advanced strategies for the development of porous carbon as a Li host/current collector for lithium metal batteries

Rajesh Pathak et al.

Summary: Lithium metal is promising for high-energy-density rechargeable batteries due to its high capacity and low density, but faces challenges like unstable solid electrolyte interphase formation and dendrite growth. Using a carbon-based porous matrix to host lithium deposition shows potential in addressing these issues and improving battery performance.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

Guiding lithium-ion flux to avoid cell's short circuit and extend cycle life for an anode-free lithium metal battery

Haile Hisho Weldeyohannes et al.

Summary: Guiding lithium deposition towards the backside of a gold-sputtered polyimide film in an anode-free lithium metal battery enables safer operation and improved cycling stability. This innovative approach also demonstrates the feasibility of using electrically nonconductive substrates as anode current collectors by modifying their lithiophilicity.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Applied

Structurally tunable characteristics of ionic liquids for optimizing lithium plating/stripping via electrolyte engineering

Shihan Qi et al.

Summary: Electrolyte chemistry plays a crucial role in regulating the solid electrolyte interphase (SEI) and Li+ solvation for safe lithium metal batteries (LMBs), with imidazole-based ionic liquids (ILs) as electrolyte additives showing promising potential in enhancing battery performance. The structured tunable characteristics of ILs contribute to the efficient formation of SEI, regulation of Li+ solvation sheath structure, and suppression of further Li plating, leading to improved electrochemical performance and stable battery life.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Review Materials Science, Multidisciplinary

Research progress on graphene-based materials for high-performance lithium-metal batteries

Xin Wang et al.

Summary: The practical application of lithium metal batteries is limited by safety problems and low Coulombic efficiency, but graphene-based materials have shown promise in solving these issues. Various protection strategies using GBMs are summarized and challenges and solutions for future development are discussed.

NEW CARBON MATERIALS (2021)

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Article Electrochemistry

Selective elimination of the reactive groups of porous biochar 3D host for stable lithium anodes

Tuo Zhao et al.

Summary: By designing a 3D porous biochar modified by silver nanoparticles with high lithiophilic and chemically stable surface as a host for Li anode, the generation of dead lithium and side reactions can be minimized, leading to high cycle coulombic efficiency.

ELECTROCHIMICA ACTA (2021)

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Article Nanoscience & Nanotechnology

Improving Cyclability of Lithium Metal Anode via Constructing Atomic Interlamellar Ion Channel for Lithium Sulfur Battery

Mao Yang et al.

Summary: The study focuses on constructing an atomic interlamellar ion channel by introducing layered montmorillonite on the surface of the separator to guide lithium ion flux, leading to stable lithium deposition and enhanced battery performance, with increased specific capacity observed after cycling.

NANOSCALE RESEARCH LETTERS (2021)

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Review Chemistry, Multidisciplinary

Biomass-based materials for green lithium secondary batteries

Chengbin Jin et al.

Summary: The advances in process engineering, nanotechnology, and materials science have made it possible for biomass to be used in novel energy storage technologies like lithium secondary batteries (LSBs). Biomass-derived materials can be sustainable battery components, contributing to green battery systems. This review provides a comprehensive overview of the fabrication and application of biomass and biomass-derived materials in LSBs, emphasizing the potential for high-performance green battery systems.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Physical

Stable Li Metal Anode Enabled by Space Confinement and Uniform Curvature through Lithiophilic Nanotube Arrays

Karnpiwat Tantratian et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Single Zinc Atoms Immobilized on MXene (Ti3C2Clx) Layers toward Dendrite-Free Lithium Metal Anodes

Jianan Gu et al.

ACS NANO (2020)

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Article Multidisciplinary Sciences

Mechanical rolling formation of interpenetrated lithium metal/lithium tin alloy foil for ultrahigh-rate battery anode

Mintao Wan et al.

NATURE COMMUNICATIONS (2020)

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Article Multidisciplinary Sciences

An ultrastable lithium metal anode enabled by designed metal fluoride spansules

Huadong Yuan et al.

SCIENCE ADVANCES (2020)

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Article Chemistry, Physical

Regulating the Hidden Solvation-Ion-Exchange in Concentrated Electrolytes for Stable and Safe Lithium Metal Batteries

Rachid Amine et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Soft Lithiophilic Graphene Aerogel for Stable Lithium Metal Anode

Tianyu Yang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Interfaces and Interphases in All-Solid-State Batteries with Inorganic Solid Electrolytes

Abhik Banerjee et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Physical

Freestanding agaric-like molybdenum carbide/graphene/N-doped carbon foam as effective polysulfide anchor and catalyst for high performance lithium sulfur batteries

Shuzhang Niu et al.

ENERGY STORAGE MATERIALS (2020)

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Review Chemistry, Physical

Dendrite-free lithium metal and sodium metal batteries

Lianbo Ma et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Advances in the Design of 3D-Structured Electrode Materials for Lithium-Metal Anodes

Sunwoo Park et al.

ADVANCED MATERIALS (2020)

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Sn layer decorated copper mesh with superior lithiophilicity for stable lithium metal anode

Jingyi Luan et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Chemistry, Physical

Lithiophilic Li-Zn alloy modified 3D Cu foam for dendrite-free lithium metal anode

Yu Ye et al.

JOURNAL OF POWER SOURCES (2020)

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Article Chemistry, Multidisciplinary

Hierarchically Nanoporous 3D Assembly Composed of Functionalized Onion-Like Graphitic Carbon Nanospheres for Anode-Minimized Li Metal Batteries

Son Ha et al.

SMALL (2020)

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Article Chemistry, Physical

Lithiophobic-lithiophilic composite architecture through co-deposition technology toward high-performance lithium metal batteries

Yifeng Cheng et al.

NANO ENERGY (2019)

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Strengthening dendrite suppression in lithium metal anode by in-situ construction of Li-Zn alloy layer

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ELECTROCHEMISTRY COMMUNICATIONS (2019)

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A Concentrated Ternary-Salts Electrolyte for High Reversible Li Metal Battery with Slight Excess Li

Feilong Qiu et al.

ADVANCED ENERGY MATERIALS (2019)

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Reduced graphene oxide aerogel as stable host for dendrite-free sodium metal anode

Feng Wu et al.

ENERGY STORAGE MATERIALS (2019)

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PMMA-assisted Li deposition towards 3D continuous dendrite-free lithium anode

Yanpeng Guo et al.

ENERGY STORAGE MATERIALS (2019)

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A 3D Cu current collector with a biporous structure derived by a phase inversion tape casting method for stable Li metal anodes

Li-Min Wang et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Chemistry, Physical

Oxygen and nitrogen co-doped porous carbon granules enabling dendrite-free lithium metal anode

Yuanming Liu et al.

ENERGY STORAGE MATERIALS (2019)

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Stable Lithium Electrodeposition at Ultra-High Current Densities Enabled by 3D PMF/Li Composite Anode

Lei Fan et al.

ADVANCED ENERGY MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Hierarchically Nanostructured Transition Metal Oxides for Lithium-Ion Batteries

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Polymer-Laden Composite Lignin-Based Electrolyte Membrane for High-Performance Lithium Batteries

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Dendrite-free Li metal anode by lowering deposition interface energy with Cu99Zn alloy coating

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Review Chemistry, Physical

Sustainability and in situ monitoring in battery development

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NATURE MATERIALS (2017)

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Nanosilicon anodes for high performance rechargeable batteries

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Making Li-metal electrodes rechargeable by controlling the dendrite growth direction

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Electrolyte additive enabled fast charging and stable cycling lithium metal batteries

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Ultrahigh-current density anodes with interconnected Li metal reservoir through overlithiation of mesoporous AlF3 framework

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Multi-shelled hollow micro-/nanostructures: promising platforms for lithium-ion batteries

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Dendrite-Free Lithium Deposition Induced by Uniformly Distributed Lithium Ions for Efficient Lithium Metal Batteries

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The role of nanotechnology in the development of battery materials for electric vehicles

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Three-dimensional SnCu scaffold with layered porous structure enable dendrite-free anode of lithium metal batteries

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