期刊
INTERNATIONAL JOURNAL OF MINERALS METALLURGY AND MATERIALS
卷 30, 期 3, 页码 581-590出版社
SPRINGER
DOI: 10.1007/s12613-022-2556-7
关键词
BaTiO3/TiO2@polypyrrole composites; hollow multishelled structure; electromagnetic wave absorbing
Researchers constructed BaTiO3/TiO2@polypyrrole (PPy) composites with hollow multishelled structure (HoMS) to enhance the electromagnetic wave absorbing properties of BaTiO3-based absorbing material. BaTiO3/TiO2 HoMSs were prepared using TiO2 HoMSs as a template. FeCl3 was then introduced to initiate the oxidative polymerization of pyrrole monomer, successfully forming BaTiO3/TiO2@PPy HoMSs. The electromagnetic wave absorbing properties of BaTiO3/TiO2 HoMSs and BaTiO3/TiO2@PPy HoMSs with different shell numbers were investigated. The results show that BaTiO3/TiO2@PPy HoMSs exhibit improved microwave absorption, with tripled-shelled BaTiO3/TiO2@PPy HoMS having the most excellent absorbing performance.
BaTiO3/TiO2@polypyrrole (PPy) composites with hollow multishelled structure (HoMS) were constructed to enhance the electromagnetic wave absorbing properties of BaTiO3-based absorbing material. BaTiO3/TiO2 HoMSs were prepared by hydrothermal crystallization using TiO2 HoMSs as template. Then, FeCl3 was introduced to initiate the oxidative polymerization of pyrrole monomer, forming BaTiO3/TiO2@PPy HoMSs successfully. The electromagnetic wave absorbing properties of BaTiO3/TiO2 HoMSs and BaTiO3/TiO2@PPy HoMSs with different shell number were investigated using a vector network analyzer. The results indicate that BaTiO3/TiO2@PPy HoMSs exhibit improved microwave absorption compared with BaTiO3/TiO2 HoMSs. In particular, tripled-shelled BaTiO3/TiO2@PPy HoMS has the most excellent absorbing performance. The best reflection loss can reach up to -21.80 dB at 13.34 GHz with a corresponding absorber thickness of only 1.3 mm, and the qualified absorption bandwidth of tripled-shelled BaTiO3/TiO2@PPy HoMS is up to 4.2 GHz. This work paves a new way for the development of high-performance composite microwave absorbing materials.
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