☆ 4.5 Review

Lignin-First Biorefinery for Converting Lignocellulosic Biomass into Fuels and Chemicals

ENERGIES (2023)

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Article Energy & Fuels

Valorization of jute (Corchorussp.) biomass for bioethanol production

Jyoti Singh et al.

Summary: This study highlights the potential use of jute biomass for the production of second-generation bioethanol. By subjecting the biomass to physical and chemical pretreatments, enzymatic saccharification and fermentation, high yields of ethanol can be obtained. In addition, valuable platform chemicals can be recovered from the by-products of alkali pretreatment.

BIOMASS CONVERSION AND BIOREFINERY (2022)

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Article Agricultural Engineering

Mild fractionation of poplar into reactive lignin via lignin-first strategy and its enhancement on cellulose saccharification

Zhenying Pan et al.

Summary: In this study, a mild lignin-first strategy was developed to extract reactive lignin with high yield and purity, as well as significantly increase the glucose yield of cellulose-rich residue. This approach shows promise for achieving full utilization of lignocellulosic biomass.

BIORESOURCE TECHNOLOGY (2022)

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Article Thermodynamics

Understanding cellulose pyrolysis under hydrogen atmosphere

Tan Li et al.

Summary: The distribution of cellulose pyrolysis products under different conditions was investigated using a high-pressure micropyrolyzer. The results showed that hydrogen pressure had an effect on the duration and composition of cellulose pyrolysis products. The formation mechanisms of various compounds under hydrogen atmosphere were discussed.

ENERGY CONVERSION AND MANAGEMENT (2022)

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Article Chemistry, Physical

Reductive Catalytic Fractionation of Spruce Wood over Ru/C Bifunctional Catalyst in the Medium of Ethanol and Molecular Hydrogen

Oxana P. Taran et al.

Summary: This study investigates the performance of Ru/C bifunctional catalysts in RCF for the catalytic separation of spruce wood. It is found that catalysts with acidic oxidized graphite-like carbon support, appropriate Ru content and dispersion can efficiently extract lignin and hemicelluloses, yielding high amounts of monomeric phenolic compounds and polyols.

CATALYSTS (2022)

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Article Green & Sustainable Science & Technology

Efficient sugar production from plant biomass: Current status, challenges, and future directions

J. Y. Zhu et al.

Summary: Lignocellulosic plant biomass is a sustainable alternative resource for the production of fuels and chemicals. The sugar platform is a promising approach for converting cellulose and hemicelluloses in plant biomass into targeted products. However, the natural recalcitrance of lignocellulose makes efficient and sustainable sugar production a challenge.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2022)

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Article Multidisciplinary Sciences

Rational highly dispersed ruthenium for reductive catalytic fractionation of lignocellulose

Zhenzhen Liu et al.

Summary: Producing monomeric phenols from lignin biopolymer depolymerization in a detachable and efficient manner has attracted significant attention for the fullest utilization of sustainable lignocellulosic biomass. In this study, a low-loaded and highly dispersed Ru anchored on a chitosan-derived N-doped carbon catalyst (RuN/ZnO/C) is reported. This catalyst exhibits outstanding performance in the reductive catalytic fractionation of lignocellulose, achieving nearly theoretical maximum yields of phenolic monomers from lignin. The selectivity towards propyl end-chained guaiacol and syringol allows for easy purification, and the process leaves high retention of (hemi)cellulose for enzymatic hydrolysis. The good stability and transformation of Ru species contribute to the effectiveness of the catalyst. Time-course experiments and reactivity screening shed light on the mechanism. Overall, this work opens up new possibilities for the valorization of lignin and the economic feasibility of lignocellulosic biomass.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

Multi-pass flow-through reductive catalytic fractionation

Jun Hee Jang et al.

Summary: Reductive catalytic fractionation (RCF) is an effective method for selectively extracting and depolymerizing lignin from biomass. Multi-pass flow-through RCF reduces solvent demand without compromising delignification and monomer yield.

JOULE (2022)

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Article Engineering, Chemical

Comparative Evaluation of Pyrolysis and Hydrothermal Liquefaction for Obtaining Biofuel from a Sustainable Consortium of Microalgae Arthrospira platensis with Heterotrophic Bacteria

Nadezhda Chernova et al.

Summary: This study compared the effectiveness of pyrolysis and hydrothermal liquefaction in obtaining biofuel from microalgal biomass, with hydrothermal liquefaction showing higher bio-oil yield. Both technologies produced similar bio-coal yields, which can serve as an alternative strategy for CO2 absorption and storage.

PROCESSES (2022)

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Article Chemistry, Physical

Continuous hydrodeoxygenation of lignin to jet-range aromatic hydrocarbons

Michael L. Stone et al.

Summary: This study reports a continuous, two-stage catalytic process using molybdenum carbide to convert lignin into aromatic hydrocarbons. The results show high selectivity and carbon recovery. Tier a fuel property testing indicates that the lignin-derived aromatic compounds may have performance advantages over conventional jet fuel aromatic compounds.

JOULE (2022)

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Article Chemistry, Multidisciplinary

Catalyst choice impacts aromatic monomer yields and selectivity in hydrogen-free reductive catalytic fractionation

Jacob K. Kenny et al.

Summary: Hydrogen-free reductive catalytic fractionation (RCF) is a promising method to extract and depolymerize lignin from native biomass. Pt/C and Pd/C achieve comparable monomer yields regardless of hydrogen pressure, while Ru/C and Ni/C show lower yields under H-2-free conditions. Pt/C and Pd/C can form ethyl and propanol products through dehydrogenation and hydrogenation reactions. Adding water increases the selectivity of propyl products. Similar trends in yield and selectivity are observed for poplar RCF and reactions with coniferyl alcohol, indicating the importance of stabilization rate of reactive monomer intermediates in H-2-free RCF.

REACTION CHEMISTRY & ENGINEERING (2022)

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Article Green & Sustainable Science & Technology

Environmental impact and cost assessment of a novel lignin production method

Pooja Yadav et al.

Summary: The study focuses on life cycle and cost assessment of novel organosolv lignin production process from spruce bark, comparing different scenarios to identify the most environmentally and economically suitable option. Results show that the baseline scenario has higher global warming potential and total cost compared to other scenarios, with scenario S2 being the most optimal choice.

JOURNAL OF CLEANER PRODUCTION (2021)

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Article Agricultural Engineering

Catalytic hydrogenolysis of lignin in ethanol/isopropanol over an activated carbon supported nickel-copper catalyst

Chongbo Cheng et al.

Summary: In this study, catalytic hydrogenolysis of organosolv poplar lignin was conducted using NiCu/C catalysts in ethanol/isopropanol solvent, achieving high yields of phenolic monomers. The introduction of Cu in catalysts promoted the hydrogen donor process of the solvent and facilitated the cleavage of lignin linkages, resulting in decreased molecular weight of bio-oil. The possible lignin dimer type structures were proposed and identified by MALDI-TOF MS, providing a better understanding of NiCu/C catalyzed lignin depolymerization.

BIORESOURCE TECHNOLOGY (2021)

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Article Chemistry, Physical

Reductive Catalytic Fractionation of Flax Shive over Ru/C Catalysts

Aleksandr S. Kazachenko et al.

Summary: This study presents reductive catalytic fractionation (RCF) of flax shive in ethanol and isopropanol using a bifunctional catalyst (Ru/C) and molecular hydrogen at elevated temperatures, resulting in solvolytic depolymerization of lignin and hemicelluloses. The catalytic hydrogenation effectively stabilizes lignin intermediates, preventing repolymerization reactions and producing a lignin fraction with high depolymerization degree. Bifunctional catalysts Ru/C significantly increase the conversion and yield of monophenolic compounds in the hydrogenation of flax shive.

CATALYSTS (2021)

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Review Chemistry, Physical

A review of bio-oil upgrading by catalytic hydrotreatment: Advances, challenges, and prospects

Mingyuan Zhang et al.

Summary: Fast pyrolysis and hydrothermal liquefaction are considered promising technologies for liquid bio-fuel production, but the poor quality of crude bio-oils has limited their direct applications. Hydrotreatment such as hydrodeoxygenation is a common upgrading technique, and this review explores the effects of different reaction conditions on the HDO treatment of real bio-oil. The underlying mechanisms for bio-oil HDO, technical challenges, and potential solutions are discussed, along with knowledge gaps and future research directions.

MOLECULAR CATALYSIS (2021)

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Article Energy & Fuels

Catalytic hydrotreatment of lignin-derived pyrolysis bio-oils using Cu/γ-Al2O3 catalyst: Reaction network development and kinetic study of anisole upgrading

Majid Saidi et al.

Summary: The kinetic study of upgrading anisole to jet-grade fuels via catalytic hydrotreatment process reveals that benzene is formed as the primary product through demethoxylation of anisole, with phenol showing the highest selectivity and activation energy in the hydrogenolysis reaction. The comprehensive quantitative reaction network for anisole catalytic hydrotreatment over Cu/gamma-Al2O3 catalyst is consistent with previous studies.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Highly Efficient Semi-Continuous Extraction and In-Line Purification of High β-O-4 Butanosolv Lignin

Douwe Sjirk Zijlstra et al.

Summary: The study demonstrated a method for obtaining high-quality lignin through organic solvent flow extraction, showing that the efficiency of lignin extraction under different conditions is crucial to yield and lignin quality.

FRONTIERS IN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Organosolv Fractionation of Walnut Shell Biomass to Isolate Lignocellulosic Components for Chemical Upgrading of Lignin to Aromatics

Rebecca N. Nishide et al.

Summary: Research on utilizing lignocellulosic biomass, such as walnut shell, for renewable carbon sources is rapidly growing. By isolating protected walnut shell lignin using methanol and dilute sulfuric acid with formaldehyde as a protecting group at 170 degrees C, a 64% yield was achieved, showing potential for high value product production.

ACS OMEGA (2021)

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Article Chemistry, Physical

Metal-support cooperation in Al(PO3)3-supported platinum nanoparticles for the selective hydrogenolysis of phenols to arenes

Xiongjie Jin et al.

Summary: A heterogeneous catalyst consisting of Al(PO3)(3)-supported platinum nanoparticles has been reported for the selective hydrogenolysis of a wide range of phenols to yield arenes under relatively mild reaction conditions. This catalyst is expected to have broad applications in fine chemical synthesis and biorefinery.

NATURE CATALYSIS (2021)

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Article Agricultural Engineering

Molybdenum-catalyzed hydrogenolysis of herbaceous biomass: A procedure integrated lignin fragmentation and components fractionation

Xue Gong et al.

Summary: The study demonstrated the successful utilization of a low-cost MoO2/C catalyst for reductive catalytic fractionation of various herbaceous biomass feedstocks, resulting in high yields and selectivity of phenolic monomers, along with the production of solid carbohydrate pulps suitable for enzymatic hydrolysis.

BIORESOURCE TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Techno-economic analysis and life cycle assessment of a biorefinery utilizing reductive catalytic fractionation

Andrew W. Bartling et al.

Summary: Reductive catalytic fractionation (RCF) is a promising method to fractionate lignocellulose and convert lignin to a narrow product slate. Analyses of techno-economic, life cycle assessment, and air emissions are crucial for guiding research towards commercialization, with a focus on cost and sustainability considerations.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Flow-through solvolysis enables production of native-like lignin from biomass

David G. Brandner et al.

Summary: In this study, flow-through solvolysis with methanol at 225 degrees C was used to produce native-like lignin from poplar, enabling the study of intrinsic lignin properties and evaluation of steady-state lignin depolymerization processes.

GREEN CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Guidelines for performing lignin-first biorefining

Mahdi M. Abu-Omar et al.

Summary: The valorisation of lignin is crucial for the economic viability of the lignocellulosic biorefining industry. The lignin-first biorefining approach, which considers lignin valorisation in the design phase, has been shown to make the fullest use of lignocellulose. Despite the diverse approaches to reporting and analyzing results from lignin-first methods, we propose guidelines for analyzing critical data in order to facilitate direct comparisons between studies.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Continuous hydrogenolysis of acetal-stabilized lignin in flow

Wu Lan et al.

Summary: Using acetal-stabilized lignin, researchers achieved a continuous high-yielding lignin depolymerization, showcasing both challenges and opportunities in processing this feedstock. High yields could be partially recovered through high temperature regeneration, despite rapid catalyst deactivation with insufficient loading.

GREEN CHEMISTRY (2021)

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Catalytic routes for the conversion of lignocellulosic biomass to aviation fuel range hydrocarbons

Hongliang Wang et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2020)

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Article Chemistry, Physical

Selective production of ethylbenzene from lignin oil over FeOx modified Ru/Nb2O5 catalyst

Lingxiao Li et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Agricultural Engineering

Catalytic hydrotreatment of kraft lignin into aromatic alcohols over nickel-rhenium supported on niobium oxide catalyst

Liping Kong et al.

BIORESOURCE TECHNOLOGY (2020)

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Article Biotechnology & Applied Microbiology

Total utilization of lignin and carbohydrates in Eucalyptus grandis: an integrated biorefinery strategy towards phenolics, levulinic acid, and furfural

Xue Chen et al.

BIOTECHNOLOGY FOR BIOFUELS (2020)

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Article Chemistry, Multidisciplinary

Lignin-First Fractionation of Softwood Lignocellulose Using a Mild Dimethyl Carbonate and Ethylene Glycol Organosolv Process

Alessandra De Santi et al.

CHEMSUSCHEM (2020)

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Article Chemistry, Multidisciplinary

One-Pot Conversion of Lignin into Naphthenes Catalyzed by a Heterogeneous Rhenium Oxide-Modified Iridium Compound

Xinxin Li et al.

CHEMSUSCHEM (2020)

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A sustainable wood biorefinery for low-carbon footprint chemicals production

Yuhe Liao et al.

SCIENCE (2020)

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Tanglei Sun et al.

BIORESOURCE TECHNOLOGY (2020)

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Review Chemistry, Multidisciplinary

Product-oriented Direct Cleavage of Chemical Linkages in Lignin

Xiaojun Shen et al.

CHEMSUSCHEM (2020)

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Article Chemistry, Physical

Novel Micro-Mesoporous Composite ZSM-5 Catalyst for Aromatics Production by Catalytic Fast Pyrolysis of Lignin Residues

Wenbo Wang et al.

CATALYSTS (2020)

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Review Chemistry, Multidisciplinary

Stabilization strategies in biomass depolymerization using chemical functionalization

Ydna M. Questell-Santiago et al.

NATURE REVIEWS CHEMISTRY (2020)

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Review Chemistry, Multidisciplinary

Downstream Processing Strategies for Lignin-First Biorefinery

Zhuohua Sun et al.

CHEMSUSCHEM (2020)

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Article Agricultural Engineering

A lignin -first strategy to recover hydroxycinnamic acids and improve cellulosic ethanol production from corn stover

Patrick A. Johnston et al.

BIOMASS & BIOENERGY (2020)

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Article Engineering, Chemical

Toward Alkylphenols Production: Lignin Depolymerization Coupling with Methoxy Removal over Supported MoS2 Catalyst

Na Ji et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Perspective on Overcoming Scale-Up Hurdles for the Reductive Catalytic Fractionation of Lignocellulose Biomass

Elias Cooreman et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Editorial Material Chemistry, Multidisciplinary

The rise of lignin biorefinery

Emilia Paone et al.

CURRENT OPINION IN GREEN AND SUSTAINABLE CHEMISTRY (2020)

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Review Biochemistry & Molecular Biology

Development of 'Lignin-First' Approaches for the Valorization of Lignocellulosic Biomass

Tamas I. Koranyi et al.

MOLECULES (2020)

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Article Chemistry, Physical

Atomically Dispersed Co Catalyst for Efficient Hydrodeoxygenation of Lignin-Derived Species and Hydrogenation of Nitroaromatics

Longkang Zhang et al.

ACS CATALYSIS (2020)

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Article Agricultural Engineering

Catalytic fast pyrolysis of enzymatic hydrolysis lignin over Lewis-acid catalyst niobium pentoxide and mechanism study

Simin Li et al.

BIORESOURCE TECHNOLOGY (2020)

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Review Agricultural Engineering

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Hongliang Wang et al.

BIORESOURCE TECHNOLOGY (2019)

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Article Biochemical Research Methods

Fractionation of lignocellulosic biomass to produce uncondensed aldehyde-stabilized lignin

Masoud Talebi Amiri et al.

NATURE PROTOCOLS (2019)

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Article Chemistry, Multidisciplinary

Fragmentation of Woody Lignocellulose into Primary Monolignols and Their Derivatives

Jiankui Sun et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2019)

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Review Biochemical Research Methods

Reductive catalytic fractionation: state of the art of the lignin-first biorefinery

Tom Renders et al.

CURRENT OPINION IN BIOTECHNOLOGY (2019)

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Article Energy & Fuels

Aromatics from Beechwood Organosolv Lignin through Thermal and Catalytic Pyrolysis

Konstantinos G. Kalogiannis et al.

ENERGIES (2019)

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Article Energy & Fuels

Unveiling the Pyrolysis Mechanisms of Hemicellulose: Experimental and Theoretical Studies

Xiaoxiao Yang et al.

ENERGY & FUELS (2019)

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Differences in S/G ratio in natural poplar variants do not predict catalytic depolymerization monomer yields

Eric M. Anderson et al.

NATURE COMMUNICATIONS (2019)

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Sequential utilization of bamboo biomass through reductive catalytic fractionation of lignin

Kaili Zhang et al.

BIORESOURCE TECHNOLOGY (2019)

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Article Energy & Fuels

Bioethanol production from cellulose obtained from the catalytic hydro-deoxygenation (lignin-first refined to aviation fuel) of apple wood

Jingzhi Zhang et al.

FUEL (2019)

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Review Thermodynamics

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Meng Wang et al.

PROGRESS IN ENERGY AND COMBUSTION SCIENCE (2019)

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Article Engineering, Environmental

Catalytic pyrolysis of lignin using low-cost materials with different acidities and textural properties as catalysts

Tong Han et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Multidisciplinary Sciences

Design of Nickel Supported on Water-Tolerant Nb2O5 Catalysts for the Hydrotreating of Lignin Streams Obtained from Lignin-First Biorefining

Glauco F. Leal et al.

ISCIENCE (2019)

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Article Chemistry, Physical

Visualization of Structural Changes During Deactivation and Regeneration of FAU Zeolite for Catalytic Fast Pyrolysis of Lignin Using NMR and Electron Microscopy Techniques

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CHEMCATCHEM (2018)

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Review Chemistry, Multidisciplinary

Bright Side of Lignin Depolymerization: Toward New Platform Chemicals

Zhuohua Sun et al.

CHEMICAL REVIEWS (2018)

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Review Chemistry, Multidisciplinary

Chemicals from lignin: an interplay of lignocellulose fractionation, depolymerisation, and upgrading

W. Schutyser et al.

CHEMICAL SOCIETY REVIEWS (2018)

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Catalytic Transformation of Lignocellulosic Biomass into Arenes, 5-Hydroxymethylfurfural, and Furfural

Tianye Guo et al.

CHEMSUSCHEM (2018)

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Article Chemistry, Multidisciplinary

Coupling organosolv fractionation and reductive depolymerization of woody biomass in a two-step catalytic process

Xianhong Ouyang et al.

GREEN CHEMISTRY (2018)

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Article Chemistry, Multidisciplinary

Lignin extraction and catalytic upgrading from genetically modified poplar

Hao Luo et al.

GREEN CHEMISTRY (2018)

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Article Biochemistry & Molecular Biology

Acid Assisted Organosolv Delignification of Beechwood and Pulp Conversion towards High Concentrated Cellulosic Ethanol via High Gravity Enzymatic Hydrolysis and Fermentation

Konstantinos G. Kalogiannis et al.

MOLECULES (2018)

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A. R. K. Gollakota et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2018)

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Article Chemistry, Multidisciplinary

Kinetic Studies of Lignin Solvolysis and Reduction by Reductive Catalytic Fractionation Decoupled in Flow-Through Reactors

Eric M. Anderson et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Article Chemistry, Physical

Lignin-first biorefinery: a reusable catalyst for lignin depolymerization and application of lignin oil to jet fuel aromatics and polyurethane feedstock

Yong Huang et al.

SUSTAINABLE ENERGY & FUELS (2018)

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Article Energy & Fuels

Production of bio-jet fuel from corncob by hydrothermal decomposition and catalytic hydrogenation: Lab analysis of process and techno-economics of a pilot-scale facility

Yuping Li et al.

APPLIED ENERGY (2018)

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Article Chemistry, Multidisciplinary

Catalytic lignocellulose biorefining in n-butanol/water: a one-pot approach toward phenolics, polyols, and cellulose

T. Renders et al.

GREEN CHEMISTRY (2018)

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Article Chemistry, Physical

Selective Production of Biobased Phenol from Lignocellulose-Derived Alkylmethoxyphenols

Xiaoming Huang et al.

ACS CATALYSIS (2018)

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Article Chemistry, Physical

A Convergent Approach for a Deep Converting Lignin-First Biorefinery Rendering High-Energy-Density Drop-in Fuels

Zhengwen Cao et al.

JOULE (2018)

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Article Chemistry, Physical

Complete lignocellulose conversion with integrated catalyst recycling yielding valuable aromatics and fuels

Zhuohua Sun et al.

NATURE CATALYSIS (2018)

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Review Energy & Fuels

A Critical Review on Hemicellulose Pyrolysis

Xiaowei Zhou et al.

ENERGY TECHNOLOGY (2017)

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Editorial Material Chemistry, Multidisciplinary

Lignin-first biomass fractionation: the advent of active stabilisation strategies

T. Renders et al.

ENERGY & ENVIRONMENTAL SCIENCE (2017)

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Article Chemistry, Multidisciplinary

Pre-treatment of lignocellulosic feedstocks using biorenewable alcohols: towards complete biomass valorisation

Christopher S. Lancefield et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Lignin depolymerization to monophenolic compounds in a flow-through system

Ivan Kumaniaev et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Phenolic acetals from lignins of varying compositions via iron(III) triflate catalysed depolymerisation

Peter J. Deuss et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Integrating lignin valorization and bio-ethanol production: on the role of Ni-Al2O3 catalyst pellets during lignin-first fractionation

S. Van den Bosch et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Depolymerization of lignin via a non-precious Ni-Fe alloy catalyst supported on activated carbon

Yongxiang Zhai et al.

GREEN CHEMISTRY (2017)

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Article Multidisciplinary Sciences

Selective production of arenes via direct lignin upgrading over a niobium-based catalyst

Yi Shao et al.

NATURE COMMUNICATIONS (2017)

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Article Multidisciplinary Sciences

Understanding the mechanism of catalytic fast pyrolysis by unveiling reactive intermediates in heterogeneous catalysis

Patrick Hemberger et al.

NATURE COMMUNICATIONS (2017)

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Article Chemistry, Multidisciplinary

Structural changes of poplar wood lignin after supercritical pretreatment using carbon dioxide and ethanol-water as co-solvents

Xing Wang et al.

RSC ADVANCES (2017)

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Increasing the revenue from lignocellulosic biomass: Maximizing feedstock utilization

David Martin Alonso et al.

SCIENCE ADVANCES (2017)

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Flowthrough Reductive Catalytic Fractionation of Biomass

Eric M. Anderson et al.

JOULE (2017)

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Effects of indium on Ni/SiO2 catalytic performance in hydrodeoxygenation of anisole as model bio-oil compound: Suppression of benzene ring hydrogenation and C-C bond hydrogenolysis

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Article Agricultural Engineering

Depolymerization of lignin by microwave-assisted methylation of benzylic alcohols

Guodian Zhu et al.

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Article Chemistry, Applied

Recent advances on fast hydropyrolysis of biomass

Fernando L. P. Resende

CATALYSIS TODAY (2016)

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Article Chemistry, Applied

Bifunctional Ni catalysts for the one-pot conversion of Organosolv lignin into cycloalkanes

Xingyu Wang et al.

CATALYSIS TODAY (2016)

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Article Chemistry, Multidisciplinary

Hydrogen-free catalytic fractionation of woody biomass

Maxim V. Galkin et al.

CHEMSUSCHEM (2016)

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Article Chemistry, Multidisciplinary

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Paola Ferrini et al.

CHEMSUSCHEM (2016)

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Article Chemistry, Multidisciplinary

High Yield Production of Natural Phenolic Alcohols from Woody Biomass Using a Nickel-Based Catalyst

Jiazhi Chen et al.

CHEMSUSCHEM (2016)

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Review Chemistry, Multidisciplinary

Lignin Valorization through Catalytic Lignocellulose Fractionation: A Fundamental Platform for the Future Biorefinery

Maxim V. Galkin et al.

CHEMSUSCHEM (2016)

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Review Chemistry, Multidisciplinary

Furfural: a renewable and versatile platform molecule for the synthesis of chemicals and fuels

R. Mariscal et al.

ENERGY & ENVIRONMENTAL SCIENCE (2016)

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Article Chemistry, Multidisciplinary

Mechanistic investigation of the Zn/Pd/C catalyzed cleavage and hydrodeoxygenation of lignin

Ian Klein et al.

GREEN CHEMISTRY (2016)

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Article Chemistry, Multidisciplinary

New insights into the structure and composition of technical lignins: a comparative characterisation study

Sandra Constant et al.

GREEN CHEMISTRY (2016)

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Article Chemistry, Analytical

Structural characterization and pyrolysis behavior of holocellulose obtained from lignin-first biorefinery

Yalun Hu et al.

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS (2016)

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Review Green & Sustainable Science & Technology

Production of renewable diesel through the hydroprocessing of lignocellulosic biomass-derived bio-oil: A review

Madhumita Patel et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2016)

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Article Multidisciplinary Sciences

Formaldehyde stabilization facilitates lignin monomer production during biomass depolymerization

Li Shuai et al.

SCIENCE (2016)

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Article Chemistry, Multidisciplinary

Total Utilization of Miscanthus Biomass, Lignin and Carbohydrates, Using Earth Abundant Nickel Catalyst

Hao Luo et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2016)

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Article Chemistry, Multidisciplinary

Synergetic Effects of Alcohol/Water Mixing on the Catalytic Reductive Fractionation of Poplar Wood

Tom Renders et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2016)

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Article Chemistry, Multidisciplinary

Reductive Catalytic Fractionation of Corn Stover Lignin

Eric M. Anderson et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2016)

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Article Materials Science, Paper & Wood

Degradation and Redeposition of the Chemical Components of Aspen Wood during Hot Water Extraction

Haiyan Chen et al.

BIORESOURCES (2015)

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Article Chemistry, Multidisciplinary

Direct production of naphthenes and paraffins from lignin

Jiechen Kong et al.

CHEMICAL COMMUNICATIONS (2015)

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Article Chemistry, Multidisciplinary

Tuning the lignin oil OH-content with Ru and Pd catalysts during lignin hydrogenolysis on birch wood

S. Van den Bosch et al.

CHEMICAL COMMUNICATIONS (2015)

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Review Chemistry, Multidisciplinary

Catalytic Transformation of Lignin for the Production of Chemicals and Fuels

Changzhi Li et al.

CHEMICAL REVIEWS (2015)

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Article Chemistry, Multidisciplinary

Reductive lignocellulose fractionation into soluble lignin-derived phenolic monomers and dimers and processable carbohydrate pulps

S. Van den Bosch et al.

ENERGY & ENVIRONMENTAL SCIENCE (2015)

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Article Chemistry, Multidisciplinary

Direct catalytic conversion of cellulose to liquid straight-chain alkanes

Beau Op de Beeck et al.

ENERGY & ENVIRONMENTAL SCIENCE (2015)

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Article Chemistry, Multidisciplinary

In situ trapping of enol intermediates with alcohol during acid-catalysed de-polymerisation of lignin in a nonpolar solvent

Atsushi Kaiho et al.

GREEN CHEMISTRY (2015)

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Article Chemistry, Multidisciplinary

Influence of bio-based solvents on the catalytic reductive fractionation of birch wood

W. Schutyser et al.

GREEN CHEMISTRY (2015)

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Article Chemistry, Multidisciplinary

Biomass-derived lignin to jet fuel range hydrocarbons via aqueous phase hydrodeoxygenation

Hongliang Wang et al.

GREEN CHEMISTRY (2015)

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Article Chemistry, Multidisciplinary

A synergistic biorefinery based on catalytic conversion of lignin prior to cellulose starting from lignocellulosic biomass

Trenton Parsell et al.

GREEN CHEMISTRY (2015)

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Article Chemistry, Analytical

Catalytic pyrolysis of lignin over HZSM-5 catalysts: Effect of various parameters on the production of aromatic hydrocarbon

Jae-Young Kim et al.

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS (2015)

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Article Chemistry, Multidisciplinary

Aromatic Monomers by in Situ Conversion of Reactive Intermediates in the Acid-Catalyzed Depolymerization of Lignin

Peter J. Deuss et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Review Thermodynamics

Recent progress in the direct liquefaction of typical biomass

Hua-jun Huang et al.

PROGRESS IN ENERGY AND COMBUSTION SCIENCE (2015)

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Article Chemistry, Multidisciplinary

Catalytic Biorefining of Plant Biomass to Non-Pyrolytic Lignin Bio-Oil and Carbohydrates through Hydrogen Transfer Reactions

Paola Ferrini et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2014)

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Article Agricultural Engineering

Catalytic fast pyrolysis of cellulose and biomass to produce levoglucosenone using magnetic SO42-/TiO2-Fe3O4

Qiang Lu et al.

BIORESOURCE TECHNOLOGY (2014)

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Article Chemistry, Multidisciplinary

Fractionation of Hemp Hurds by Organosolv Pretreatment and its Effect on Production of Lignin and Sugars

Stefano Gandolfi et al.

CHEMSUSCHEM (2014)

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Article Energy & Fuels

Upgrading of Bio-Oil in a Continuous Process with Dolomite Catalyst

Beatriz Valle et al.

ENERGY & FUELS (2014)

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Article Energy & Fuels

Contribution of dehydration and depolymerization reactions during the fast pyrolysis of various salt-loaded celluloses at low temperatures

Dawei Liu et al.

FUEL (2014)

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Review Chemistry, Multidisciplinary

Conversion of biomass platform molecules into fuel additives and liquid hydrocarbon fuels

Maria J. Climent et al.

GREEN CHEMISTRY (2014)

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Article Chemistry, Multidisciplinary

Catalytic pyrolysis of individual components of lignocellulosic biomass

Kaige Wang et al.

GREEN CHEMISTRY (2014)

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Review Multidisciplinary Sciences

Lignin Valorization: Improving Lignin Processing in the Biorefinery

Arthur J. Ragauskas et al.

SCIENCE (2014)

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Article Chemistry, Multidisciplinary

Hydrodeoxygenation of Lignin-Derived Phenolic Monomers and Dimers to Alkane Fuels over Bifunctional Zeolite-Supported Metal Catalysts

Wei Zhang et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2014)

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Article Chemistry, Multidisciplinary

A Route for Lignin and Bio-Oil Conversion: Dehydroxylation of Phenols into Arenes by Catalytic Tandem Reactions

Xingyu Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2013)

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Article Agricultural Engineering

Direct hydrodeoxygenation of cellulose and xylan to lower alkanes on ruthenium catalysts in subcritical water

Yuriko Osaka et al.

BIOMASS & BIOENERGY (2013)

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Article Agricultural Engineering

Bioethanol production, using carbohydrate-rich microalgae biomass as feedstock

Shih-Hsin Ho et al.

BIORESOURCE TECHNOLOGY (2013)

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Review Energy & Fuels

Catalytic Fast Pyrolysis: A Review

Theodore Dickerson et al.

ENERGIES (2013)

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Article Chemistry, Multidisciplinary

Lignin depolymerization (LDP) in alcohol over nickel-based catalysts via a fragmentation-hydrogenolysis process

Qi Song et al.

ENERGY & ENVIRONMENTAL SCIENCE (2013)

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Article Chemistry, Multidisciplinary

Cleavage and hydrodeoxygenation (HDO) of C-O bonds relevant to lignin conversion using Pd/Zn synergistic catalysis

Trenton H. Parsell et al.

CHEMICAL SCIENCE (2013)

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Article Chemistry, Physical

Controlling the selectivity to chemicals from lignin via catalytic fast pyrolysis

Zhiqiang Ma et al.

APPLIED CATALYSIS A-GENERAL (2012)

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Article Chemistry, Physical

Gas-phase hydrodeoxygenation of guaiacol over Fe/SiO2 catalyst

R. N. Olcese et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2012)

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Review Agricultural Engineering

Review of fast pyrolysis of biomass and product upgrading

A. V. Bridgwater

BIOMASS & BIOENERGY (2012)

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Article Chemistry, Physical

Deactivation and Regeneration of H-USY Zeolite during Lignin Catalytic Fast Pyrolysis

Zhiqiang Ma et al.

CHEMCATCHEM (2012)

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Article Chemistry, Multidisciplinary

One-pot catalytic hydrocracking of raw woody biomass into chemicals over supported carbide catalysts: simultaneous conversion of cellulose, hemicellulose and lignin

Changzhi Li et al.

ENERGY & ENVIRONMENTAL SCIENCE (2012)

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Article Energy & Fuels

Structural Characterization of Switchgrass Lignin after Ethanol Organosolv Pretreatment

Gang Hu et al.

ENERGY & FUELS (2012)

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Review Multidisciplinary Sciences

Valorization of Biomass: Deriving More Value from Waste

Christopher O. Tuck et al.

SCIENCE (2012)

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Article Chemistry, Physical

Novel Hierarchical Cerium-Incorporated MFI Zeolite Catalysts for the Catalytic Fast Pyrolysis of Lignocellulosic Biomass

Gregory T. Neumann et al.

ACS CATALYSIS (2012)

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Article Biotechnology & Applied Microbiology

Chemicals from lignocellulosic biomass: opportunities, perspectives, and potential of biorefinery systems

Francesco Cherubini et al.

BIOFUELS BIOPRODUCTS & BIOREFINING-BIOFPR (2011)

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Article Chemistry, Multidisciplinary

Effective Production of Octane from Biomass Derivatives under Mild Conditions

Wenjie Xu et al.

CHEMSUSCHEM (2011)

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Article Chemistry, Multidisciplinary

Product Distribution from the Fast Pyrolysis of Hemicellulose

Pushkaraj R. Patwardhan et al.

CHEMSUSCHEM (2011)

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Article Chemistry, Physical

Aqueous-phase hydrodeoxygenation of bio-derived phenols to cycloalkanes

Chen Zhao et al.

JOURNAL OF CATALYSIS (2011)

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Article Agricultural Engineering

The direct pyrolysis and catalytic pyrolysis of Nannochloropsis sp residue for renewable bio-oils

Pan Pan et al.

BIORESOURCE TECHNOLOGY (2010)

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Article Chemistry, Multidisciplinary

Hydrodeoxygenation of bio-derived phenols to hydrocarbons using RANEY (R) Ni and Nafion/SiO2 catalysts

Chen Zhao et al.

CHEMICAL COMMUNICATIONS (2010)

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Review Chemistry, Multidisciplinary

The Catalytic Valorization of Lignin for the Production of Renewable Chemicals

Joseph Zakzeski et al.

CHEMICAL REVIEWS (2010)

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Article Thermodynamics

The biorefinery concept: Using biomass instead of oil for producing energy and chemicals

Francesco Cherubini

ENERGY CONVERSION AND MANAGEMENT (2010)

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Article Energy & Fuels

Catalytic upgrading of biomass fast pyrolysis vapors with titania and zirconia/titania based catalysts

Qiang Lu et al.

FUEL (2010)

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Article Chemistry, Applied

Catalytic pyrolysis-GC/MS of lignin from several sources

Charles A. Mullen et al.

FUEL PROCESSING TECHNOLOGY (2010)

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Article Chemistry, Physical

Stability of Zeolites in Hot Liquid Water

Ryan M. Ravenelle et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2010)

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Review Thermodynamics

Main routes for the thermo-conversion of biomass into fuels and chemicals. Part 1: Pyrolysis systems

Mustafa Balat et al.

ENERGY CONVERSION AND MANAGEMENT (2009)

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Review Green & Sustainable Science & Technology

Biomass-based energy fuel through biochemical routes: A review

R. C. Saxena et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2009)

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Article Chemistry, Multidisciplinary

Selective Degradation of Wood Lignin over Noble-Metal Catalysts in a Two-Step Process

Ning Yan et al.

CHEMSUSCHEM (2008)

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Article Chemistry, Analytical

Fast pyrolysis of cassava rhizome in the presence of catalysts

Adisak Pattiya et al.

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS (2008)

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Article Chemistry, Analytical

Effect of zeolites and nanopowder metal oxides on the distribution of chiral anhydrosugars evolved from pyrolysis of cellulose: An analytical study

Daniele Fabbri et al.

JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS (2007)

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Review Thermodynamics

Review of biomass pyrolysis oil properties and upgrading research

Zhang Qi et al.

ENERGY CONVERSION AND MANAGEMENT (2007)

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Review Agricultural Engineering

Features of promising technologies for pretreatment of lignocellulosic biomass

N Mosier et al.

BIORESOURCE TECHNOLOGY (2005)

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Review Multidisciplinary Sciences

Stabilization wedges: Solving the climate problem for the next 50 years with current technologies

S Pacala et al.

SCIENCE (2004)

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Article Energy & Fuels

An overview of Biomass pyrolysis

A Demirbas et al.

ENERGY SOURCES (2002)

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Article Thermodynamics

Mechanisms of liquefaction and pyrolysis reactions of biomass

A Demirbas

ENERGY CONVERSION AND MANAGEMENT (2000)

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