☆ 4.6 Review

Molecular and colloidal self-assembly at the oil-water interface

CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2022)

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Biophysical properties of tear film lipid layer II. Polymorphism of FAHFA

Xiaojie Xu et al.

Summary: Fatty acid esters of hydroxy fatty acids (FAHFAs) are a newly discovered class of lipids that include (O-acyl)-w-hydroxy fatty acids (OAHFAs). OAHFAs have been found to be an important component of the tear film lipid layer (TFLL), but their biophysical function in TFLL is still poorly understood. This study investigated the molecular biophysical mechanisms of OAHFAs using PAHSA as a model and found unique polymorphic behaviors and configurational transitions of PAHSA molecules under various lateral pressures.

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Biophysical properties of tear film lipid layer I. Surface tension and surface rheology

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Summary: The tear film lipid layer (TFLL) plays a crucial role in stabilizing the tear film and dysfunction can lead to dry eye disease. Understanding the properties of TFLL is important for developing treatments for dry eye disease.

BIOPHYSICAL JOURNAL (2022)

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Article Chemistry, Physical

Ion Pairing and Molecular Orientation at Liquid/Liquid Interfaces: Self-Assembly and Function

Lu Lin et al.

Summary: This study investigates the molecular orientation at buried oil/aqueous interfaces using vibrational sum-frequency generation spectroscopy, numerical polarization analysis, and atomistic molecular dynamics simulations. The results show that the orientation of self-assembled oligomers changes upon the addition of salts in the aqueous phase, attributed to competitive ion effects altering the orientations of the tails extending into the oil phase. These specific anionic effects occur via interfacial ion pairing and associated changes in interfacial solvation and hydrogen-bonding networks. These findings offer quantitative insight into orientational changes during self-assembly, facilitating the design of functional interfaces for various applications.

JOURNAL OF PHYSICAL CHEMISTRY B (2022)

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Article Chemistry, Physical

Squeezing Out Interfacial Solvation: The Role of Hydrogen-Bonding in the Structural and Orientational Freedom of Molecular Self-Assembly

Zening Liu et al.

Summary: Bioinspired membrane molecules with improved physical properties and enhanced stability can serve as functional models for conventional lipid or amphiphilic species. The self-assembly of amphiphilic, charged oligodimethylsiloxane imidazolium cation at the air-aqueous interface is elucidated using Langmuir trough methods and surface-specific vibrational sum-frequency generation spectroscopy. A compression-induced desolvation step is found to precede phase transitions, and atomistic molecular dynamics simulations support the experimental data. The understanding of hydrophobic tail conformations offers new strategies for interface design in developing soft-matter electronics and low-dimensional materials.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2022)

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Disentangling Memristive and Memcapacitive Effects in Droplet Interface Bilayers Using Dynamic Impedance Spectroscopy

Robert L. Sacci et al.

Summary: This study investigates biomimetic neuromorphic equivalents based on biological membranes using dynamic electrochemical impedance spectroscopy (dEIS) to explore the molecular-level structural and dynamic differences that give rise to memristive and memcapacitive behaviors in response to electrical biasing. The research findings show that the system's memristive and memcapacitive properties originate from different molecular restructuring processes, and can be simultaneously achieved in a single device.

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Elanna B. Stephenson et al.

Summary: Model membranes, especially droplet interface bilayers, have the potential to mimic cell membranes and enable quantification of membrane processes. They can be used for electrophysiological measurements and biological analysis.

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Emulsion stability and dilatational rheological properties of soy/whey protein isolate complexes at the oil-water interface: Influence of pH

Xiaoying Zhang et al.

Summary: At pH 2.0-8.0, the interaction between SPI and WPI at the interface resulted in unstable emulsions, while at pH 8.0-11.0, electrostatic repulsion between the proteins led to stable emulsions. This study provides insights for pH treatment selection of SPI-WPI composite emulsions with different stabilities and rheological behaviors, and potential applications for bioactive compound delivery systems.

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Functional nanoparticles through π-conjugated polymer self-assembly

Liam R. MacFarlane et al.

Summary: pi-Conjugated polymers exhibit diverse electronic and optical properties. This review discusses the preparation of self-assembled nanoparticles from these polymers and their applications in optoelectronics, biomedical imaging and therapy, photocatalysis, and sensing. The development of pi-conjugated polymers has opened up new possibilities for functional organic materials similar to inorganic semiconductors, with nanoparticles based on these polymers showing promise in various emerging applications.

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Article Chemistry, Multidisciplinary

Responsive Interfacial Assemblies Based on Charge-Transfer Interactions

Shuyi Sun et al.

Summary: Charge transfer interactions are commonly used in constructing supramolecular systems, but the formation of CT complexes at the liquid-liquid interface has not been reported until now. By utilizing electron-deficient acceptors in water and electron-rich donors in oil, CT complex surfactants can be formed and assembled at the oil-water interface, ultimately leading to the creation of higher-order nanofilms with exceptional mechanical properties. The redox-responsiveness of the electron-deficient acceptor allows for reversible manipulation of the assembly and disassembly of CTCSs, offering the potential for switchable structures in liquids.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Template-mediated self-assembly of magnetite-gold nanoparticle superstructures at the water-oil interface of AOT reverse microemulsions

Rebeca Fortes Martin et al.

Summary: In this study, bimetallic magnetite-gold nanostructures were synthesized using microemulsions, with different types of nanoparticles modulating the morphology and surfactant film properties. Phase separation into Winsor phases allowed the formation of micrometer-scale bimetallic heterostructures upon solvent evaporation.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Mechanics

Effect of nanoparticle surfactants on droplet formation in a flow-focusing microchannel

Jie Qi et al.

Summary: Nanoparticle surfactants formed by interactions between nanoparticles and complementary polymers have been proposed as excellent stabilizers for liquid droplets in substance encapsulation and delivery applications. This study found that adding carboxylated nanoparticles to the dispersed phase and amino-terminated polymers to the continuous phases significantly reduces droplet size while increasing production rate. The combined effect of nanoparticles and polymers is greater than the sum of their individual effects due to the reduction of oil-water interfacial tension by nanoparticle surfactants.

PHYSICS OF FLUIDS (2021)

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Electrophoretic concentration and production of conductive coatings from silver nanoparticles stabilized with non-ionic surfactant Span 80

Pavel Sergeevich Popovetskiy et al.

Summary: This study demonstrated the synthesis of spherical silver nanoparticles with a diameter of 9.4 nm stabilized by a non-ionic surfactant, and their high electrokinetic potential allowing for the concentration of silver organosols through non-aqueous electrophoresis. Mirror-like silver films with high silver content (up to 96%) and varying thicknesses were successfully produced by heat treatment of the concentrates at specific temperatures.

COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS (2021)

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Article Chemistry, Multidisciplinary

From Nanoparticle Heteroclusters to Filament Networks by Self-Assembly at the Water-Oil Interface of Reverse Microemulsions

Rebeca Fortes Martin et al.

Summary: Surface self-assembly of spherical nanoparticles into hierarchical heterostructures is developing, with template-mediated interactions and the use of specific surfactants playing key roles in forming complex nanostructured films and filament-like networks.

LANGMUIR (2021)

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Article Chemistry, Multidisciplinary

Growth of Au nanoparticles on phosphorylated zein protein particles for use as biomimetic catalysts for cascade reactions at the oil-water interface

Yongkang Xi et al.

Summary: This study introduces a novel strategy based on Pickering interfacial catalysis (PIC) to address the downside of traditional chemo-enzymatic cascade processes. The protein-stabilized Pickering system for biphasic cascade catalysis, enabled by phosphorylated zein nanoparticles (ZCPOPs) immobilized in gold nanoparticles (Au NCs), demonstrates excellent catalytic activity and mimicking properties of horseradish peroxidase, achieving a significant improvement in catalytic yield compared to sole metal catalysis.

CHEMICAL SCIENCE (2021)

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Temperature-sensitive soft microgels at interfaces: air-water versus oil-water

Steffen Bochenek et al.

Summary: The study investigates the behavior of microgels at different interfaces, finding that the total in-plane size of microgels increases with increasing interfacial tension, but the portion of microgels in the aqueous phase remains unchanged.

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Interfacial Assembly and Jamming of Polyelectrolyte Surfactants: A Simple Route To Print Liquids in Low-Viscosity Solution

Ruiyan Xu et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Insight into the Mechanisms Driving the Self-Assembly of Functional Interfaces: Moving from Lipids to Charged Amphiphilic Oligomers

Azhad U. Chowdhury et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Photoresponsive Structured Liquids Enabled by Molecular Recognition at Liquid-Liquid Interfaces

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JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Atomic Force Microscopy Imaging of Adsorbed Pulmonary Surfactant Films

Lu Xu et al.

BIOPHYSICAL JOURNAL (2020)

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Pickering emulsions: Versatility of colloidal particles and recent applications

Hang Jiang et al.

CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2020)

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Influence of Charges on the Behavior of Polyelectrolyte Microgels Confined to Oil-Water Interfaces

Maximilian M. Schmidt et al.

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Article Mechanics

Retardation of droplet transport in confined microchannel by interfacial jamming of nanoparticles

Zheng Yuan Luo et al.

PHYSICS OF FLUIDS (2020)

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Determining the surface dilational rheology of surfactant and protein films with a droplet waveform generator

Jinlong Yang et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2019)

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Exploring the colloid-to-polymer transition for ultra-low crosslinked microgels from three to two dimensions

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Self-Assembly of Nanoparticles in 2D and 3D: Recent Advances and Future Trends

Sujit Kumar Ghosh et al.

MACROMOLECULAR CHEMISTRY AND PHYSICS (2019)

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Capsules from Pickering emulsion templates

Ana Maria Bago Rodriguez et al.

CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2019)

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Molecular Assembly of Rotary and Linear Motor Proteins

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Solid-liquid-liquid wettability and its prediction with surface free energy models

A. Stammitti-Scarpone et al.

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Interfacial self-assembly of amphiphilic conjugated block copolymer into 2D nanotapes

Xiao-Shuai Guo et al.

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Effect of Oil Hydrophobicity on the Adsorption and Rheology of β-Lactoglobulin at Oil-Water Interfaces

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Nanoscopic Visualization of Cross-Linking Density in Polymer Networks with Diarylethene Photoswitches

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Accuracy of Axisymmetric Drop Shape Analysis in Determining Surface and Interfacial Tensions

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Fine-Tuning Nanoparticle Packing at Water-Oil Interfaces Using Ionic Strength

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Self-Assembly of Colloidal Nanocrystals: From Intricate Structures to Functional Materials

Michael A. Boles et al.

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Phospholipid adsorption at oil in water versus water in oil interfaces: Implications for interfacial densities and bulk solubilities

Ellen Hidebrandt et al.

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Supracrystalline Colloidal Eggs: Epitaxial Growth and Freestanding Three-Dimensional Supracrystals in Nanoscaled Colloidosomes

Zhijie Yang et al.

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Phase Transitions in Dipalmitoylphosphatidylcholine Monolayers

Yi Y. Zuo et al.

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Assembly of Nanoscale Objects at the Liquid/Liquid Interface

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Interfacial self-assembly of a bacterial hydrophobin

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Mechanical properties of protein adsorption layers at the air/water and oil/water interface: A comparison in light of the thermodynamical stability of proteins

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The Compressibility of pH- Sensitive Microgels at the Oil- Water Interface: Higher Charge Leads to Less Repulsion

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Conformational changes of globular proteins adsorbed at oil-in-water emulsion interfaces examined by Synchrotron Radiation Circular Dichroism

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Ordered polyelectrolyte assembly at the oil-water interface

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PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2012)

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Bappaditya Samanta et al.

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Edgar Acosta

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Yi Y. Zuo et al.

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William L. Hwang et al.

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Screening Blockers Against a Potassium Channel with a Droplet Interface Bilayer Array

Ruhma Syeda et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2008)

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Hagan Bayley et al.

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Yong-Kyun Park et al.

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Yousung Jung et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2007)

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Lipid bilayer formation by contacting monolayers in a microfluidic device for membrane protein analysis

Kei Funakoshi et al.

ANALYTICAL CHEMISTRY (2006)

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Stepwise directing of nanocrystals to self-assemble at water/oil interfaces

Jing Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2006)

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Article Multidisciplinary Sciences

Colloidal jamming at interfaces: A route to fluid-bicontinuous gels

K Stratford et al.

SCIENCE (2005)

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Spontaneous assembly of a monolayer of charged gold nanocrystals at the water/oil interface

F Reincke et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2004)

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HW Duan et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2004)

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Article Multidisciplinary Sciences

Nanoparticle assembly and transport at liquid-liquid interfaces

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SCIENCE (2003)

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Article Multidisciplinary Sciences

Colloidosomes: Selectively permeable capsules composed of colloidal particles

AD Dinsmore et al.

SCIENCE (2002)

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Review Chemistry, Physical

Particles as surfactants - similarities and differences

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CURRENT OPINION IN COLLOID & INTERFACE SCIENCE (2002)

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Review Pharmacology & Pharmacy

Microemulsion-based media as novel drug delivery systems

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ADVANCED DRUG DELIVERY REVIEWS (2000)

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