A low-temperature hydrothermal cutoff: plagioclase 40Ar/39Ar thermochronology of the Rustenburg Layered Suite, Bushveld complex

The mid-low-temperature thermal history of layered mafic intrusions is crucial to understanding the duration of hydrothermal systems and the formation of economically viable ore deposits within the large thermal anomaly of these magma bodies. Due to a lack of low-temperature chronometry, the mid-low-temperature thermal evolution of the world's largest layered intrusion, the Bushveld Complex, remains relatively unknown. We provide a comprehensive plagioclase 40Ar/39Ar thermochronologic study throughout the Rustenburg Layered Suite (RLS) of the Bushveld Complex in South Africa. 40Ar/39Ar step-heating analyses were applied to 20 plagioclase grains that encompass 12 stratigraphic levels and the entire similar to 7 km thickness of the Eastern Limb of the RLS. Individual plagioclase grains yield 40Ar/39Ar plateau ages ranging from 1997.9 +/- 5.0 Ma to 2051.4 +/- 5.3 Ma, and closure temperatures of 151 +/- 15 degrees C to 310 +/- 12 degrees C (assuming a 10 degrees C -Ma(-1) cooling rate). Plagioclase 40Ar/39Ar ages and closure temperatures, combined with 40Ar/39Ar biotite ages from the same samples, suggest that RLS cooling rates decrease abruptly (from similar to 1000 degrees C -Ma(-1) to similar to 10 degrees C -Ma(-1)) near the 40Ar/39Ar closure temperature of biotite. The decrease in cooling rate is a product of the cessation of hydrothermal circulation (within < 1 Ma of zircon crystallization) associated with the emplacement of the RLS and is supported by numerical heat-loss simulations that produce the observed geochronology. The duration of hydrothermal circulation places age constraints on hydrothermal ore deposits within the host rocks (Transvaal and Witwatersrand Supergroups), as any ore deposits related to emplacement of the RLS must be coeval with 40Ar/39Ar biotite ages.

Automated summary

By studying the 40Ar/39Ar thermochronology of plagioclase in the Rustenburg Layered Suite of the Bushveld Complex, South Africa, we gained insights into the mid-low-temperature thermal evolution of the region. The variations in 40Ar/39Ar plateau ages and closure temperatures of plagioclase suggest a sudden decrease in cooling rate near the closure temperature of biotite, indicating the cessation of hydrothermal circulation within a million years of zircon crystallization. These findings have important implications for understanding the duration of hydrothermal systems and the formation of economically viable ore deposits.