4.6 Article

Full-color Persistent Room-temperature Phosphorescence from Carbon Dot Composites Based on a Single Nonaromatic Carbon Source

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CHEMISTRY-AN ASIAN JOURNAL
卷 18, 期 2, 页码 -

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WILEY-V C H VERLAG GMBH
DOI: 10.1002/asia.202201027

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room temperature phosphorescence; full-color; afterglow; carbon dots; white light

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A series of carbon dot composites with full-color and long-lived room-temperature phosphorescence have been prepared using a simple solid-phase one-step method. The emission wavelength can be adjusted by changing the feeding ratio and reaction temperature. These composites exhibit huge application potential in the field of anti-counterfeiting, fingerprint identification, and optoelectronic devices.
Herein, a series of carbon dot composites (CDC) with full-color and long-lived room-temperature phosphorescence (RTP) are prepared by a simple solid-phase one-step method from a single non-conjugated and non-aromatic carbon source. The RTP emission wavelength can be adjusted from 462 to 623 nm by changing the feeding ratio and reaction temperature. The luminescent lifetime and quantum yield of a green emissive CDC (AB-CDC-3) reach 1.1 s and 39%, respectively, because of the close interaction between carbon dots and inorganic matrix. Due to the existence of multiple luminescent centers, these CDC exhibit excitation wavelength-dependent RTP and a white emission when excited at a specific wavelength. A single-component afterglow luminescent diode based on AB-CDC-4 shows a high-quality white emission with CIE of (0.30, 0.33) and color-rendering index of 88. Based on the unique photophysical properties of the composites, they exhibit huge application potential in the field of multilevel anti-counterfeiting, fingerprint identification, and optoelectronic devices.

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