期刊
CHEMICAL SOCIETY REVIEWS
卷 52, 期 4, 页码 1428-1455出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cs00785a
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Since the successful separation of different cucurbit[n]uril homologues in 2001, the field of cucurbit[n]uril supramolecular chemistry has rapidly developed. The combination of Q[n] cavity size and various external stimuli has led to the creation of various Q[n]-based mechanically interlocked molecules (MIMs), including (pseudo)rotaxanes, catenanes, dendrimers, and poly(pseudo)rotaxanes. This review article highlights the important advancements in the field of Q[n]-based MIMs over the past two decades, discusses examples of heterowheel (pseudo)rotaxanes and poly(pseudo)rotaxanes involving Q[n]s, and reflects on the opportunities and challenges of constructing Q[n]-based stimuli-responsive MIMs.
Cucurbit[n]uril supramolecular chemistry has developed rapidly since 2001 when different cucurbit[n]uril homologues (Q[n]) were successfully separated in pure form. The combination of Q[n] cavity size and various types of external stimuli has given birth to numerous types of Q[n]-based mechanically interlocked molecules (MIMs), including (pseudo)rotaxanes, catenanes, dendrimers and poly(pseudo)rotaxanes. In this review article, the important advances in the field of Q[n]-based MIMs over the past two decades are highlighted. This review also describes examples of heterowheel (pseudo)rotaxanes and poly(pseudo)rotaxanes involving Q[n]s, and reflects on the opportunities and challenges of constructing Q[n]-based stimuli-responsive MIMs.
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