Low-threshold green and red random lasing emission in inorganic halide lead perovskite microcrystals with plasmonic and interferential enhancement

Herein, low-threshold green and red random lasing actions were investigated in inorganic caesium lead bromide (CsPbBr3) and caesium lead iodide (CsPbI3) perovskite microcrystals, which were grown using metal organic chemical vapor deposition. Sharp random lasing emission peaks were visible on the right side of the broad photoluminescence emission spectra. Interferential patterned sapphire substrates and novel metal nanoparticles were used to enhance the lasing emission intensity and reduce the lasing emission thresholds. Fast-decayed random lasing oscillation dynamics and backscattering angular distribution of light confirmed that the multi-scattering of light was important in the reduction of the threshold in thin films on patterned sapphire sub-strates. Plasmonic enhancement between gold or silver nanoparticles and the perovskite microcrystals contrib-uted similarly to low threshold random lasing emission, which was verified using the simulation result from the finite difference time domain (FDTD) method. This work has a wide range of applications in sensing, speckle-free imaging, illumination, and medical diagnosis.

Automated summary

In this study, low-threshold green and red random lasing actions were investigated in inorganic caesium lead bromide and caesium lead iodide perovskite microcrystals. The use of interferential patterned sapphire substrates and novel metal nanoparticles enhanced the lasing emission intensity and reduced the lasing emission thresholds. The multi-scattering of light and plasmonic enhancement were important in reducing the threshold and contributing to low threshold random lasing emission, as confirmed by experimental and simulation results using the FDTD method.