期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 -, 期 -, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202217565
关键词
Advanced Characterizations; CO2 Reduction; Metal-Organic Frameworks; Photocatalysis; Water Splitting
Photocatalytic water splitting and CO2 reduction using metal-organic frameworks (MOFs) have great potential for addressing energy and environmental issues. This review discusses the semiconductor-like behavior of MOFs and summarizes recent advances in photocatalytic water splitting and CO2 reduction using MOF-based materials. The unique advantage of MOFs in elucidating the structure-property relationship in photocatalysis is highlighted, along with representative characterization techniques for studying the kinetics and reaction intermediates. The challenges and future directions are also proposed.
Photocatalytic water splitting and carbon dioxide (CO2) reduction provide promising solutions to global energy and environmental issues. In recent years, metal-organic frameworks (MOFs), a class of crystalline porous solids featuring well-defined and tailorable structures as well as high surface areas, have captured great interest toward photocatalytic water splitting and CO2 reduction. In this review, the semiconductor-like behavior of MOFs is first discussed. We then summarize the recent advances in photocatalytic water splitting and CO2 reduction over MOF-based materials and focus on the unique advantage of MOFs for clarifying the structure-property relationship in photocatalysis. In addition, some representative characterization techniques have been presented to unveil the photocatalytic kinetics and reaction intermediates in MOF-based systems. Finally, the challenges, and perspectives for future directions are proposed.
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