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Hui Ouyang et al.
Summary: A study on the preparation and application of yolk-shell Co SASCs highlights the potential of direct chemical interactions for the formation of highly active catalysts and their use in catalysis and chemiluminescence.
ANALYTICAL CHEMISTRY
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Mylena Lemes Cunha et al.
Summary: Rapid and low-cost molecular analysis is crucial for early and specific diagnostics. Automated molecular diagnostic devices, such as sample-to-answer microfluidic devices, promise a complete molecular diagnosis system. The extraction process in such devices is laborious but important for sensitive and specific detection. Thus, researching automated or semiautomated extraction methodologies is beneficial for improving extraction procedures.
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Yanmei Yang et al.
Summary: This study presents a multi-amplification strategy based on paper-spray mass spectrometry for the analysis of miRNAs in blood. A toehold-mediated DNA-strand-displacement reaction is used to amplify the signal chain and ensure specificity. The paper spray method efficiently filters out interfering substances and enhances detection sensitivity.
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Chemistry, Multidisciplinary
Anna C. Closs et al.
Summary: Evolutionary biological processes lead to changes in heritable traits, where the responsible genetic information in DNA is altered, selected, and inherited through the mutation of the base sequence. Evolutionary changes at the molecular level of small organic molecules are unknown but represent an important prerequisite for the emergence of life, where catalysts can exhibit different selectivity during formation.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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Oncology
Cuiliu Liu et al.
Summary: This article discusses the importance of liquid biopsies in the discovery of lung cancer biomarkers, introduces emerging blood-based minimally invasive biomarkers, and discusses their advantages and limitations. It also summarizes the progress of identified biomarkers for clinical management of lung cancer, and proposes a potential strategy for early detection of lung cancer using a combination of LDCT scans and biomarkers.
Review
Chemistry, Multidisciplinary
Vasile I. Parvulescu et al.
Summary: This review examines the use of catalytic processes in water treatment, exploring their advantages in terms of kinetics of transformation, selectivity, and energy saving. However, implementing these technologies at an industrial scale still faces controversies and limitations. The focus is on solar-driven catalytic technologies and other emerging processes, while also identifying the challenges involved, such as the complexity of systems and the coexistence of various interfaces.
Review
Chemistry, Multidisciplinary
Hari Krishna Bisoyi et al.
Summary: Smart soft materials play a critical role in advanced devices and digitally augmented technologies. Liquid crystals, with their responsive and adaptive attributes, have promising potential as smart soft materials. In the 20th century, liquid crystals revolutionized the information display industry, and in the 21st century, they have demonstrated numerous beyond-display applications.
Review
Medical Laboratory Technology
Steve Miller et al.
Summary: Majority of studies show that mNGS has similar sensitivity to specific PCR assays and can identify more potential pathogens than conventional methods. Concerns remain about contamination and detection of nonclinically significant organisms, highlighting the importance of careful interpretation of pathogenicity and potential association with clinical syndromes. Further research is needed to evaluate the improvement in clinical outcomes and cost-effectiveness of mNGS testing.
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Haiping Wu et al.
Summary: This article presents an alternative analysis platform, dNASA, which is based on digital nucleic acid signal amplification in droplets. By using a bead-based controllable extension bridged cascade signal amplification reaction, the platform achieves highly efficient and specific nucleic acid signal amplification. The feasibility of the platform was demonstrated in single-base DNA mutation analysis.
ANALYTICAL CHEMISTRY
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Chemistry, Analytical
Jie Wang et al.
Summary: In this study, a miRNA-21-responsive G-quadruplex-embedded self-quenching probe was designed for regulating single probe-based multiplex amplifications. The method allows for the detection of miRNA-21 in a range from 1 fM to 1 nM with a limit of detection of 0.86 fM, and was successfully applied to serum samples.
ANALYTICAL CHEMISTRY
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Biophysics
Lei Wu et al.
Summary: Cancer is the second leading cause of death worldwide, making early diagnosis and personalized treatment crucial. Surface enhanced Raman spectroscopy (SERS) has emerged as an effective biosensing technique in cancer theranostics, allowing ultra-sensitive and multiplex detection of tumor nucleic acids. It has great potential for clinical cancer detection and subtyping.
BIOSENSORS & BIOELECTRONICS
(2022)
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Chemistry, Analytical
Haimei Li et al.
Summary: Under the interference of complex and diverse tumor microenvironments, accurate diagnosis and effective treatment of malignant tumors have become the focus of research. In this study, a novel biomimetic nanocatalyst with quad-modal imaging capabilities was developed for self-enhanced photothermal/chemodynamic synergistic therapy. This nanocatalyst showed excellent tumor-targeting ability and biocompatibility, and enabled TME-responsive tumor visualization.
ANALYTICAL CHEMISTRY
(2022)
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Chemistry, Analytical
Liqin Chen et al.
Summary: A new center dot OH-specific fluorescent probe RH-EDA was developed based on the scavenging mechanism of a neuroprotective drug edaravone. RH-EDA showed high sensitivity and selectivity for center dot OH, allowing imaging of endogenous center dot OH production in living cells and zebrafishes, as well as discrimination of cancer cells from normal ones based on different center dot OH levels.
ANALYTICAL CHEMISTRY
(2021)
Review
Environmental Sciences
Jiebin Duan et al.
Summary: This review summarizes the effectiveness of hydroxylamine-driven advanced oxidation processes (HAOPs) for water treatment and categorizes them into different types, discussing their reaction mechanisms and advantages. Additionally, the application prospects and challenges of HAOPs in pollutant degradation are also discussed.
Review
Biochemical Research Methods
Yan Cao et al.
Summary: This review examines a wide range of methods for detecting DNA and RNA at single-digit attomolar concentrations without the need for nucleic acid amplification. These methods correspond to the clinically desirable detection range for pathogen-specific nucleic acid and are close to the detection limits of commercially available nucleic acid amplification tests based on PCR. With the ongoing pandemic, the demand for faster, more cost-effective, yet highly accurate tests has become increasingly evident.
CURRENT OPINION IN BIOTECHNOLOGY
(2021)
Review
Chemistry, Analytical
Changjing Yuan et al.
Summary: The combination of SERS and NAIA provides researchers with more sensitive and precise analysis in biological samples, covering various techniques such as HCR, CHA, EDR, SDA, RPA, EXPAR, RCA, and LAMP. Challenges and prospective opinions of SERS in application are also discussed.
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(2021)
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Environmental Sciences
Chao Wang et al.
Summary: This study demonstrated a fast and efficient degradation of the antibiotic norfloxacin in a hydroxylamine enhanced Fenton system, proposing three main degradation steps including defluorination, quinolone group transformation, and defluorination and piperazinyl ring opening. The crucial degradation step was identified as the defluorination process.
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Engineering, Environmental
Zhuo-Yu Li et al.
Summary: This study compared the degradation efficiency of two hydroxylamine salts on dimethyl phthalate and found that Cl- significantly improved the production of hydroxyl radicals, affecting the oxidation intermediates. It was revealed for the first time that Cl- could shift reactive species from Fe(IV) to radicals in the PMS/Fe(II) system.
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Chemistry, Analytical
Wenzhi Zhang et al.
Summary: This method achieves ultrasensitive gene sensing through electrochemical-chemical-cyclic amplification and fluorescence detection, amplifying the signal while reducing noise, reliably quantifying Fe3+ and detecting HBV and p53 genes in blood samples.
ANALYTICAL CHEMISTRY
(2021)
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Chemistry, Analytical
Riham Zayani et al.
Summary: The study developed a magnetofluorescent bioplatform for the direct and specific detection of SARS-CoV-2 viral RNA in COVID-19-positive patients' nasopharyngeal swabs with high selectivity and sensitivity. It was able to differentiate SARS-CoV-2 RNA from other related viruses and demonstrated 100% sensitivity and specificity in clinical samples.
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Zijie Zhang et al.
Summary: This study developed a simple and rapid saliva-based SARS-CoV-2 antigen test using a newly developed DNA aptamer, which showed high sensitivity and specificity in detecting the wildtype virus and its Alpha and Delta variants.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
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Chemistry, Physical
Hongyu Zhou et al.
Summary: This review systematically summarized the origins, development, basic mechanism, and limits of reductant-enhanced iron-based peroxide activation processes. It was found that the use of reductants could accelerate the reduction of Fe3+ and quench the production of reactive species, with the trade-off determined by intrinsic chemical properties and experimental conditions. Additionally, practical application potential of different reductants based on toxicity, costs, and self-transformation products was evaluated, and new enhancement strategies were proposed for future research needs.
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Min Li et al.
Summary: Nucleic acids, such as DNA and RNA, play crucial roles in storing, transmitting, and expressing genetic information. Nucleic acid tests are essential for clinical diagnosis and infectious disease prevention, and have made significant advancements in recent years.
Review
Chemistry, Multidisciplinary
Jianzhi Huang et al.
Summary: This review focuses on the redox reactivity of four types of Fe(II) species and discusses their formation pathways, factors governing the reactivity, potential mechanisms, reactivity comparison, and characterization techniques. It also covers the roles of Fe(II) species in environmental applications and abiotic oxidation related processes in natural and engineered systems.
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Yufan Chen et al.
Summary: The study found that the adsorption and decomposition of formate and H2O2 in the presence of freshly formed ferrihydrite are controlled by surface-initiated reactions, affecting the surface Fenton reactions. Oxidation mainly occurs in the solid-liquid boundary layer, rather than in bulk or on the surface.
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Erik E. Augspurger et al.
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Krzysztof Zamojc et al.
CRITICAL REVIEWS IN ANALYTICAL CHEMISTRY
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(2011)
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(2011)
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Anna Maria Nowicka et al.
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Benoit D'Autreaux et al.
NATURE REVIEWS MOLECULAR CELL BIOLOGY
(2007)
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G Bengtsson et al.
JOURNAL OF THE CHEMICAL SOCIETY-DALTON TRANSACTIONS
(2002)
