期刊
CATALYSIS COMMUNICATIONS
卷 69, 期 -, 页码 86-91出版社
ELSEVIER
DOI: 10.1016/j.catcom.2015.05.016
关键词
Hierarchical zeolite; Reductive amination; Nickel nanoparticles; Acid-metal bi-functional catalyst; One-pot reaction
In this paper, we wish to report the synthesis and characterization of nickel nanoparticles supported on acidic form of ZSM-5 zeolite (Ni/H-mZSM-5) with microporous/mesoporous hierarchical structure. This catalyst was effectively employed as novel acid-metal hi-functional heterogeneous catalyst for direct one-pot reductive amination of aldehydes with nitroarenes in the presence of NaBH4 as a mild reducing agent. Excellent yields at room temperature and short reaction time in aqueous media conditions were obtained. (C) 2015 Elsevier B.V. All rights reserved.
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