期刊
FRONTIERS IN CHEMISTRY
卷 10, 期 -, 页码 -出版社
FRONTIERS MEDIA SA
DOI: 10.3389/fchem.2022.995063
关键词
metal-organic frameworks; ionic liquid; electrolyte; battery; lithium; sodium
资金
- Ministerio de Ciencia, Innovacion y Universidades [PID 2019-107468RB-C21]
- BIDEKO project - MCIN/AEI
- NextGenerationEU
- PRTR
- Gobierno Vasco/Eusko Jaurlaritza [IT1546-22]
- ELKARTEK program
- FCT (Fundacao para a Ciencia e Tecnologia) [UIDB/4650/2020, UID/CTM/50025/2021, UID/FIS/04650/2021, UID/EEA/04436/2021]
- FEDER funds through the COMPETE 2020 Program [PTDC/FIS-MAC/28157/2017, POCI-01-0145-FEDER-007688]
- European Commission [778412]
- [2020.04028 CEECIND]
This review focuses on the combination of metal-organic frameworks (MOFs) and ionic liquids (ILs) for the development of solid electrolytes. MOFs offer great opportunities for synthesizing high-performance electrolytes due to their controllable chemical composition and tunable pore structure. Encapsulating ILs into porous materials provides environmentally friendly solid-state electrolytes. The review also discusses the use of MOFs as anodes and cathodes in Li- and Na-ion batteries.
This review focuses on the combination of metal-organic frameworks (MOFs) and ionic liquids (ILs) to obtain composite materials to be used as solid electrolytes in metal-ion battery applications. Benefiting from the controllable chemical composition, tunable pore structure and surface functionality, MOFs offer great opportunities for synthesizing high-performance electrolytes. Moreover, the encapsulation of ILs into porous materials can provide environmentally benign solid-state electrolytes for electrochemical devices. Due to the versatility of MOF-based materials, in this review we also explore their use as anodes and cathodes in Li- and Na-ion batteries. Finally, solid IL@MOF electrolytes and their implementation into Li and Na batteries have been analyzed, as well as the design and advanced manufacturing of solid IL@MOF electrolytes embedded on polymeric matrices.
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